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Statistical, Nonlinear, and Soft Matter Physics
City University of New York (CUNY)
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Nonlinear Optical Studies Of Interfacial Ferroelectricity And Strain Distribution In Perovskite Dielectric Films, Tony Le
Dissertations, Theses, and Capstone Projects
Dielectric and ferroelectric perovskite films have been model energy storage structures for their low-dielectric loss, extremely high charge-discharge speed, and good temperature stability, yet there is still much to understand about the material’s limitations. This dissertation presents a detailed understanding of the strain-induced ferroelectricity at the boundary between a strontium titanate (SrTiO3) ultrathin film epitaxially grown on a germanium (Ge) substrate through optical second harmonic generation (SHG), and the polydomain distribution in the Zr-doped BaTiO3 (BZT) films by time-resolved pump-probe spectroscopy.
First, SHG measurements were performed to reveal interfacial ferroelectricity in the epitaxial SrTiO3/Ge (100) …