Physics Commons^™

Single-Stage Few-Cycle Pulse Amplification, Sagnik Ghosh, Nathan G. Drouillard, Tj Hammond

Physics Publications

Kerr instability can be exploited to amplify visible, near-infrared, and midinfrared ultrashort pulses. We use the results of Kerr instability amplification theory to inform our simulations amplifying few-cycle pulses. We show that the amplification angle dependence is simplified to the phase-matching condition of four-wave mixing when the intense pump is considered. Seeding with few-cycle pulses near the pump leads to broadband amplification without spatial chirp, while longer pulses undergo compression through amplification. Pumping in the midinfrared leads to multioctave spanning amplified pulses with single-cycle duration not previously predicted. We discuss limitations of the amplification process and optimizing pump and seed …

Supercontinuum Light Generation Via Non-Linear Effects In Hollow-Core Fiber, Skyler Gulati

Physics Student Works

The field of non-linear optics has gained traction in the last couple decades due to the variable generation of wavelengths which are less deterministic than within traditional optics. Using non-linear mediums, including hollow-core fibers (HCF), generation of wavelengths spanning into the vacuum ultraviolet (VUV) wavelength range is possible. These short wavelengths can be utilized within electron spectroscopy-based methods of material science like angle-resolved photoemission spectroscopy (ARPES). This technique most often uses specific photoemission lines of atoms in discharge lamps, however, with the frequency dispersion capabilities of HCF, broad band creation can allow for variable wavelength selection through filtering specific wavelengths …

Experimental Evidence That Shear Bands In Metallic Glasses Nucleate Like Cracks, Alan A. Long, Wendelin Wright, Xiaojun Gu, Anna Thackray, Mayisha Nakib, Jonathan T. Uhl, Karin A. Dahmen

Faculty Journal Articles

Highly time-resolved mechanical measurements, modeling, and simulations show that large shear bands in bulk metallic glasses nucleate in a manner similar to cracks. When small slips reach a nucleation size, the dynamics changes and the shear band rapidly grows to span the entire sample. Smaller nucleation sizes imply lower ductility. Ductility can be increased by increasing the nucleation size relative to the maximum (“cutoff”) shear band size at the upper edge of the power law scaling range of their size distribution. This can be achieved in three ways: (1) by increasing the nucleation size beyond this cutoff size of the …

A Microfluidic Approach For Synthesis And Kinetic Profiling Of Branched Gold Nanostructures, Qi Cai, Valentina Castagnola, Luca Boselli, Alirio Moura, Hender Lopez, Wei Zhang, João M. De Araújo, Kenneth A. Dawson

Articles

Automatized approaches for nanoparticle synthesis and characterization represent a great asset to their applicability in the biomedical field by improving reproducibility and standardization, which help to meet the selection criteria of regulatory authorities. The scaled-up production of nanoparticles with carefully defined characteristics, including intrinsic morphological features, and minimal intra-batch, batch-to-batch, and operator variability, is an urgent requirement to elevate nanotechnology towards more trustable biological and technological applications. In this work, microfluidic approaches were employed to achieve fast mixing and good reproducibility in synthesizing a variety of gold nanostructures. The microfluidic setup allowed exploiting spatial resolution to investigate the growth evolution …

Spectral Broadening For Pulse Compression Using Liquid Alcohols, Jacob A. Stephen, Chathurangani J. Arachchige, Tj Hammond

Physics Publications

Although gases, and more recently solids, have been used to create few-cycle pulses, we explore using liquid alcohols for spectral broadening and femtosecond pulse compression. By using a series of 1 cm cuvettes filled with 1-decanol, we have compressed a pulse from 83.6 fs down to 31.3 fs with a spectrum capable of supporting 25 fs pulses without filamentation.We measure the nonlinear index of refraction for various liquids, measuring n2 = (6.8 ± 0.5) × 10−20 m2 W−1 for 1-decanol.We demonstrate liquids to be a compact, simple, versatile, and cost-effective material to obtain broad spectra.

A Nanoscale Shape-Discovery Framework Supporting Systematic Investigations Of Shape-Dependent Biological Effects And Immunomodulation, Wei Zhang, Hender Lopez, Luca Boselli, Paolo Bigini, André Perez-Potti, Zengchun Xie, Valentina Castagnola, Qi Cai, Camila P. Silveira, Joao M. De Araujo, Laura Talamini, Nicolò Panini, Giuseppe Ristagno, Martina B. Violatto, Stéphanie Devineau, Marco P. Monopoli, Mario Salmona, Valeria A. Giannone, Sandra Lara, Kenneth A. Dawson, Yan Yan

Articles

Since it is now possible to make, in a controlled fashion, an almost unlimited variety of nanostructure shapes, it is of increasing interest to understand the forms of biological control that nanoscale shape allows. However, a priori rational investigation of such a vast universe of shapes appears to present intractable fundamental and practical challenges. This has limited the useful systematic investigation of their biological interactions and the development of innovative nanoscale shape-dependent therapies. Here, we introduce a concept of biologically relevant inductive nanoscale shape discovery and evaluation that is ideally suited to, and will ultimately become, a vehicle for machine …

Robust Method Of Determining Microfacet Brdf Parameters In The Presence Of Noise Via Recursive Optimization, Michael W. Bishop, Samuel D. Butler, Michael A. Marciniak

Faculty Publications

Accurate bidirectional reflectance distribution function (BRDF) models are essential for computer graphics and remote sensing performance. The popular microfacet class of BRDF models is geometric-optics-based and computationally inexpensive. Fitting microfacet models to scatterometry measurements is a common yet challenging requirement that can result in a model being fit as one of several unique local minima. Final model fit accuracy is therefore largely based on the quality of the initial parameter estimate. This makes for widely varying material parameter estimates and causes inconsistent performance comparisons across microfacet models, as will be shown with synthetic data. We proposed a recursive optimization method …

Nonlinear Schrödinger Equation Solitons On Quantum Droplets, A. Ludu, A.S. Carstea

Publications

Irrotational flow of a spherical thin liquid layer surrounding a rigid core is described using the defocusing nonlinear Schrödinger equation. Accordingly, azimuthal moving nonlinear waves are modeled by periodic dark solitons expressed by elliptic functions. In the quantum regime the algebraic Bethe ansatz is used in order to capture the energy levels of such motions, which we expect to be relevant for the dynamics of the nuclear clusters in deformed heavy nuclei surface modeled by quantum liquid drops. In order to validate the model we match our theoretical energy spectra with experimental results on energy, angular momentum, and parity for …

Control-Oriented Nonlinear Modeling Of Polyvinyl Chloride (Pvc) Gel Actuators, Mohammed Al-Rubaiai, Xinda Qi, Zachary Frank, Ryohei Tsuruta, Umesh Gandhi, Kwang J. Kim, Xiaobo Tan

Mechanical Engineering Faculty Research

Polyvinyl chloride (PVC) gel-based actuators are a new class of soft, electroactive polymer actuators with several attractive properties, including low cost, large compliance, large strain output, high-stress output, fast response, and stability against thermal influence. While PVC gel actuators are quickly gaining attention, they remain largely unexplored despite their great potential in a long list of applications compared with many other smart material actuators. In particular, little work has been reported on modeling nonlinear dynamics of PVC actuators. In this work a nonlinear, control-oriented Hammerstein model, with a polynomial nonlinearity preceding a transfer function, is proposed to capture the amplitude-dependent …

Voltage-Controlled Magnetic Anisotropy In Antiferromagnetic Mgo-Capped Mnpt Films, P. H. Chang, Wuzhang Fang, T. Ozaki, Kirill Belashchenko

Kirill Belashchenko Publications

The magnetic anisotropy in MgO-capped MnPt films and its voltage control are studied using first-principles calculations. Sharp variation of the magnetic anisotropy with film thickness, especially in the Pt-terminated film, suggests that it may be widely tuned by adjusting the film thickness. In thick films the linear voltage control coefficient is as large as 1.5 and -0.6 pJ/Vm for Pt-terminated and Mn-terminated interfaces, respectively. The combination of a widely tunable magnetic anisotropy energy and a large voltage-control coefficient suggest that MgO-capped MnPt films can serve as a versatile platform for magnetic memory and antiferromagnonic applications.

Impact Of Dynamic Sub-Populations Within Grafted Chains On The Protein Binding And Colloidal Stability Of Pegylated Nanoparticles, Delyan Hristov, Hender Lopez, Yannick Ortin, Kate O'Sullivan, Kenneth A. Dawson, Dermot F. Brougham

Articles

Polyethylene glycol grafting has played a central role in preparing the surfaces of nano-probes for biological interaction, to extend blood circulation times and to modulate protein recognition and cellular uptake. However, the role of PEG graft dynamics and conformation in determining surface recognition processes is poorly understood primarily due to the absence of a microscopic picture of the surface presentation of the polymer. Here a detailed NMR analysis reveals three types of dynamic ethylene glycol units on PEG-grafted SiO2 nanoparticles (NPs) of the type commonly evaluated as long-circulating theranostic nano-probes; a narrow fraction with fast dynamics associated with the chain …

Vibration Of A Cantilever Laboratory, Mark D. Shattuck

Open Educational Resources

Hands on laboratory to measure the vibrational frequencies of a cantilever.

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Aps March Meeting 2021 (Online) Updates On Scientific Research During Pandemic Times, Vianney Gimenez-Pinto

Title III Professional Development Reports

While the ongoing global pandemic continues to affect our everyday lives, researchers in Science, Technology, Engineering and Math found a way to come together at the American Physical Society (APS) March Meeting 2021. The conference was online-only and had more than 11,000 registered attendants who actively participated in the program during March 14- 19, 2021.

Exclusion Statistics For Particles With A Discrete Spectrum, Stéphane Ouvry, Alexios P. Polychronakos

Publications and Research

We formulate and study the microscopic statistical mechanics of systems of particles with exclusion statistics in a discrete one-body spectrum. The statistical mechanics of these systems can be expressed in terms of effective single-level grand partition functions obeying a generalization of the standard thermodynamic exclusion statistics equation of state. We derive explicit expressions for the thermodynamic potential in terms of microscopic cluster coefficients and show that the mean occupation numbers of levels satisfy a nesting relation involving a number of adjacent levels determined by the exclusion parameter. We apply the formalism to the harmonic Calogero model and point out a …

Ultrafast Spin-Currents And Charge Conversion At 3d-5d Interfaces Probed By Time-Domain Terahertz Spectroscopy, T. H. Dang, J. Hawecker, E. Rongione, G. Baez Flores, D. Q. To, J. C. Rojas-Sanchez, H. Nong, J. Mangeney, J. Tignon, F. Godel, S. Collin, P. Seneor, M. Bibes, A. Fert, M. Anane, J. M. George, L. Vila, M. Cosset-Cheneau, D. Dolfi, R. Lebrun, P. Bortolotti, Kirill Belashchenko, S. Dhillon, H. Jaffrès

Kirill Belashchenko Publications

Spintronic structures are extensively investigated for their spin-orbit torque properties, required for magnetic commutation functionalities. Current progress in these materials is dependent on the interface engineering for the optimization of spin transmission. Here, we advance the analysis of ultrafast spin-charge conversion phenomena at ferromagnetic-Transition metal interfaces due to their inverse spin-Hall effect properties. In particular, the intrinsic inverse spin-Hall effect of Pt-based systems and extrinsic inverse spin-Hall effect of Au:W and Au:Ta in NiFe/Au:(W,Ta) bilayers are investigated. The spin-charge conversion is probed by complementary techniques-ultrafast THz time-domain spectroscopy in the dynamic regime for THz pulse emission and ferromagnetic resonance spin-pumping …

Proximity-Induced Magnetization In Graphene: Towards Efficient Spin Gating, Mihovil Bosnar, Ivor Lončarić, P. Lazić, Kirill Belashchenko, Igor Žutić

Kirill Belashchenko Publications

Gate-tunable spin-dependent properties could be induced in graphene at room temperature through the magnetic proximity effect by placing it in contact with a metallic ferromagnet. Because strong chemical bonding with the metallic substrate makes gating ineffective, an intervening passivation layer is needed. Previously considered passivation layers result in a large shift of the Dirac point away from the Fermi level, so that unrealistically large gate fields are required to tune the spin polarization in graphene (Gr). We show that a monolayer of Au or Pt used as the passivation layer between Co and graphene brings the Dirac point closer to …

Detection Of Uncompensated Magnetization At The Interface Of An Epitaxial Antiferromagnetic Insulator, Pavel N. Lapa, Min Han Lee, Igor V. Roshchin, Kirill Belashchenko, Ivan K. Schuller

Kirill Belashchenko Publications

We have probed directly the temperature and magnetic field dependence of pinned uncompensated magnetization at the interface of antiferromagnetic FeF₂ with Cu, using FeF₂-Cu-Co spin valves. Electrons polarized by the Co layer are scattered by the pinned uncompensated moments at the FeF₂-Cu interface giving rise to giant magnetoresistance. We determined the direction and magnitude of the pinned uncompensated magnetization at different magnetic fields and temperatures using the angular dependencies of resistance. The strong FeF₂ anisotropy pins the uncompensated magnetization along the easy axis independent of the cooling field orientation. Most interestingly, magnetic fields as …

Reinvestigation Of The Intrinsic Magnetic Properties Of (Fe1-Xcox)2b Alloys And Crystallization Behavior Of Ribbons, Tej Nath Lamichhane, Olena Palasyuk, Vladimir P. Antropov, Ivan A. Zhuravlev, Kirill Belashchenko, Ikenna C. Nlebedim, Kevin W. Dennis, Anton Jesche, Matthew J. Kramer, Sergey L. Bud'ko, R. William Mccallum, Paul C. Canfield, Valentin Taufour

Kirill Belashchenko Publications

New determination of the magnetic anisotropy from single crystals of (Fe_1-xCo_x)2B alloys are presented. The anomalous temperature dependence of the anisotropy constant is discussed using the standard Callen-Callen theory, which is shown to be insufficient to explain the experimental results. A more material specific study using first-principles calculations with disordered moments approach gives a much more consistent interpretation of the experimental data. Since the intrinsic properties of the alloys with x=0.3-0.35 are promising for permanent magnets applications, initial investigation of the extrinsic properties are described, in particular the crystallization of melt spun ribbons with Cu, Al, …

Semi-Lagrangian Implicit Bhatnagar-Gross-Krook Collision Model For The Finite-Volume Discrete Boltzmann Method, Leitao Chen, Sauro Succi, Xiaofeng Cai, Laura Schaefer

Publications

In order to increase the accuracy of temporal solutions, reduce the computational cost of time marching, and improve the stability associated with collisions for the finite-volume discrete Boltzmann method, an advanced implicit Bhatnagar-Gross-Krook (BGK) collision model using a semi-Lagrangian approach is proposed in this paper. Unlike existing models, in which the implicit BGK collision is resolved either by a temporal extrapolation or by a variable transformation, the proposed model removes the implicitness by tracing the particle distribution functions (PDFs) back in time along their characteristic paths during the collision process. An interpolation scheme is needed to evaluate the PDFs at …

Introduction To Molecular Dynamics Simulations, Katharina Vollmayr-Lee

Faculty Journal Articles

We provide an introduction to molecular dynamics simulations in the context of the Kob–Andersen model of a glass. We introduce a complete set of tools for doing and analyzing the results of simulations at fixed NVE and NVT. The modular format of the paper allows readers to select sections that meet their needs. We start with an introduction to molecular dynamics independent of the programming language, followed by introductions to an implementation using PYTHON and then the freely available open source software package LAMMPS. We also describe analysis tools for the quick testing of the program during its development and …

Numerical Simulation Of The Trapping Reaction With Mobile And Reacting Traps, Joshua D. Hellerick, Robert C. Rhoades, Benjamin Vollmayr-Lee

Faculty Journal Articles

We study a variation of the trapping reaction, A+B→A, in which both the traps (A) and the particles (B) undergo diffusion, and the traps upon meeting react according to A+A→0 or A. This two-species reaction-diffusion system is known to exhibit a nontrivial decay exponent for the B particles, and recently renormalization group methods have predicted an anomalous dimension in the BB correlation function. To test these predictions, we develop a computer simulation method, motivated by the technique of Mehra and Grassberger [Phys. Rev. E 65, 050101(R) (2002)], that determines the complete probability distribution of the B particles …

Questaal: A Package Of Electronic Structure Methods Based On The Linear Muffin-Tin Orbital Technique, Dimitar Pashov, Swagata Acharya, Walter R.L. Lambrecht, Jerome Jackson, Kirill Belashchenko, Athanasios Chantis, Francois Jamet, Mark Van Schilfgaarde

Kirill Belashchenko Publications

This paper summarises the theory and functionality behind Questaal, an open-source suite of codes for calculating the electronic structure and related properties of materials from first principles. The formalism of the linearised muffin-tin orbital (LMTO) method is revisited in detail and developed further by the introduction of short-ranged tight-binding basis functions for full-potential calculations. The LMTO method is presented in both Green's function and wave function formulations for bulk and layered systems. The suite's full-potential LMTO code uses a sophisticated basis and augmentation method that allows an efficient and precise solution to the band problem at different levels of theory, …

Effects Of Intrinsic Defects And Alloying With Fe On The Half-Metallicity Of Co2Mnsi, G. G. Baez Flores, Ivan A. Zhuravlev, Kirill Belashchenko

Kirill Belashchenko Publications

The electronic structure and half-metallic gap of Co2MnSi in the presence of crystallographic defects, partial Fe substitution for Mn, and thermal spin fluctuations are studied using the coherent potential approximation and the disordered local moment method. In the presence of 5% Co or Mn vacancies the Fermi level shifts down to the minority-spin valence-band maximum. In contrast to NiMnSb, both types of Mn antisite defects in Co2MnSi are strongly exchange coupled to the host magnetization, and thermal spin fluctuations do not strongly affect the half-metallic gap. Partial substitution of Mn by Fe results in considerable changes in the Bloch spectral …

Optical Potts Machine Through Networks Of Three-Photon Down-Conversion Oscillators, Mostafa Honari-Latifpour, Mohammad-Ali Miri

Publications and Research

In recent years there has been a growing interest in optical simulation of lattice spin models for applications in classical computing. Here, we propose optical implementation of a three-state Potts spin model by using networks of coupled parametric oscillators with phase tristability. We first show that the cubic nonlinear process of spontaneous three-photon down-conversion is accompanied by a tristability in the phase of the subharmonic signal between three states with 2��/3 phase contrast. The phase of such a parametric oscillator behaves like a three-state spin system. Next, we show that a network of dissipatively coupled three-photon down-conversion oscillators emulates the …

From Critical Behavior To Catastrophic Runaways: Comparing Sheared Granular Materials With Bulk Metallic Glasses, Alan A. Long, Dmitry Denisov, Peter Schall, Todd C. Hufnagel, Xiaojun Gu, Wendelin J. Wright, Karin A. Dahmen

Faculty Journal Articles

The flow of granular materials and metallic glasses is governed by strongly correlated, avalanche-like deformation. Recent comparisons focused on the scaling regimes of the small avalanches, where strong similarities were found in the two systems. Here, we investigate the regime of large avalanches by computing the temporal profile or “shape” of each one, i.e., the time derivative of the stress-time series during each avalanche. We then compare the experimental statistics and dynamics of these shapes in granular media and bulk metallic glasses. We complement the experiments with a mean-field model that predicts a critical size beyond which avalanches turn into …

Multiplicativity Of Connes' Calculus, Partha Sarathi Chakraborty, Satyajit Guin

Journal Articles

In his book on noncommutative geometry, Connes constructed a differential graded algebra out of a spectral triple. Lack of monoidality of this construction is investigated. We identify a suitable monoidal subcategory of the category of spectral triples and show that when restricted to this subcategory the construction of Connes is monoidal. Richness of this subcategory is exhibited by establishing a faithful endofunctor to this subcategory.

Force Oscillations Distort Avalanche Shapes, Louis W. Mcfaul, Wendelin J. Wright, Jordan Sickle, Karin A. Dahmen

Faculty Journal Articles

Contradictory scaling behavior in experiments testing the principle of universality may be due to external oscillations. Thus, the effect of damped oscillatory external forces on slip avalanches in slowly deformed solids is simulated using a mean-field model. Akin to a resonance effect, oscillatory driving forces change the dynamics of avalanches with durations close to the oscillation period. This problem can be avoided by tuning mechanical resonance frequencies away from the range of the inverse avalanche durations. The results provide critical guidance for experimental tests for universality and a quantitative understanding of avalanche dynamics under a wide range of driving conditions.

Tracing Cyclic Homology Pairings Under Twisting Of Graded Algebras, Sayan Chakraborty, Makoto Yamashita

Journal Articles

We give a description of cyclic cohomology and its pairing with K-groups for 2-cocycle deformation of algebras graded over discrete groups. The proof relies on a realization of monodromy for the Gauss–Manin connection on periodic cyclic cohomology in terms of the cup product action of group cohomology.

Proximitized Materials, Igor Žutić, Alex Matos-Abiague, Benedikt Scharf, Hanan Dery, Kirill Belashchenko

Kirill Belashchenko Publications

Advances in scaling down heterostructures and having an improved interface quality together with atomically thin two-dimensional materials suggest a novel approach to systematically design materials. A given material can be transformed through proximity effects whereby it acquires properties of its neighbors, for example, becoming superconducting, magnetic, topologically nontrivial, or with an enhanced spin–orbit coupling. Such proximity effects not only complement the conventional methods of designing materials by doping or functionalization but also can overcome their various limitations. In proximitized materials, it is possible to realize properties that are not present in any constituent region of the considered heterostructure. While the …

Universality Class Of Explosive Percolation In Barabási-Albert Networks, Habib E. Islam, M. K. Hassan

Physics Faculty Publications

In this work, we study explosive percolation (EP) in Barabási-Albert (BA) network, in which nodes are born with degree k = m, for both product rule (PR) and sum rule (SR) of the Achlioptas process. For m = 1 we find that the critical point t_c = 1 which is the maximum possible value of the relative link density t; Hence we cannot have access to the other phase like percolation in one dimension. However, for m > 1 we find that t_c decreases with increasing m and the critical exponents ν, α, β and γ …