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- Time-resolved fluorescence anisotropy (2)
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Articles 1 - 30 of 36
Full-Text Articles in Physics
Non-Hermitian Matter-Wave Mixing In Bose-Einstein Condensates: Dissipation-Induced Amplification, S. Wuster, Ramy El-Ganainy
Non-Hermitian Matter-Wave Mixing In Bose-Einstein Condensates: Dissipation-Induced Amplification, S. Wuster, Ramy El-Ganainy
Ramy El-Ganainy
We investigate the nonlinear scattering dynamics in interacting atomic Bose-Einstein condensates under non-Hermitian dissipative conditions. We show that, by carefully engineering a momentum-dependent atomic loss profile, one can achieve matter-wave amplification through four-wave mixing in a quasi-one-dimensional nearly-free-space setup—a process that is forbidden in the counterpart Hermitian systems due to energy mismatch. Additionally, we show that similar effects lead to rich nonlinear dynamics in higher dimensions. Finally, we propose a physical realization for selectively tailoring the momentum-dependent atomic dissipation. Our strategy is based on a two-step process: (i) exciting atoms to narrow Rydberg or metastable excited states, and (ii) introducing …
Modeling Out-Of-Plane Actuation In Thin-Film Nematic Polymer Networks: From Chiral Ribbons To Auto-Origami Boxes Via Twist And Topology, Vianney Gimenez-Pinto, Fangfu Ye, Badel Mbanga, Jonathan Selinger, Robin Selinger
Modeling Out-Of-Plane Actuation In Thin-Film Nematic Polymer Networks: From Chiral Ribbons To Auto-Origami Boxes Via Twist And Topology, Vianney Gimenez-Pinto, Fangfu Ye, Badel Mbanga, Jonathan Selinger, Robin Selinger
Jonathan Selinger
Phase Transition And Surface Sublimation Of A Mobile Potts Model, A. Bailly Reyre, H. T. Diep, M. Kaufman
Phase Transition And Surface Sublimation Of A Mobile Potts Model, A. Bailly Reyre, H. T. Diep, M. Kaufman
Miron Kaufman
We study in this paper the phase transition in a mobile Potts model by the use of Monte Carlo simulation. The mobile Potts model is related to a diluted Potts model, which is also studied here by a mean-field approximation. We consider a lattice where each site is either vacant or occupied by a q-state Potts spin. The Potts spin can move from one site to a nearby vacant site. In order to study the surface sublimation, we consider a system of Potts spins contained in a recipient with a concentration c defined as the ratio of the number of …
Gait Transition Dynamics Are Modulated By Experimental Protocol, Mohammad Abdolvahab, Jason Gordon
Gait Transition Dynamics Are Modulated By Experimental Protocol, Mohammad Abdolvahab, Jason Gordon
Mohammad Abdolvahab
No abstract provided.
Application Of Transfer Matrix Method To Secondharmonic Generation In Nonlinear Photonic Bandgap Structures: Oblique Incidence, Han Li
Han Li
No abstract provided.
Sucralose Destabilization Of Protein Structure, Christina M. Othon
Sucralose Destabilization Of Protein Structure, Christina M. Othon
Christina M Othon
Sucralose is a commonly employed artificial sweetener that behaves very differently than its natural disaccharide counterpart, sucrose, in terms of its interaction with biomolecules. The presence of sucralose in solution is found to destabilize the native structure of two model protein systems: the globular protein bovine serum albumin and an enzyme staphylococcal nuclease. The melting temperature of these proteins decreases as a linear function of sucralose concentration. We correlate this destabilization to the increased polarity of the molecule. The strongly polar nature is manifested as a large dielectric friction exerted on the excited-state rotational diffusion of tryptophan using time-resolved fluorescence …
Second-Harmonic Generation At Oblique Angles In Photonic Bandgap Structures, Han Li
Second-Harmonic Generation At Oblique Angles In Photonic Bandgap Structures, Han Li
Han Li
No abstract provided.
Second Harmonic Generation At Oblique Angles In Photonic Bandgap Structures, Han Li
Second Harmonic Generation At Oblique Angles In Photonic Bandgap Structures, Han Li
Han Li
No abstract provided.
Heterogeneous Rotational Diffusion Of A Fluorescent Probe In Lipid Monolayers, Christina M. Othon
Heterogeneous Rotational Diffusion Of A Fluorescent Probe In Lipid Monolayers, Christina M. Othon
Christina M Othon
The rotational correlation time of the lipid probe 1-palmitoyl-2-{6-[(7-nitro-2-1,3-benzoxadiazol-4-yl)amino]hexanoyl}-sn-glycero-3-phosphocholine (NBD-PC) is measured using fluorescence anisotropy for two lipid species. We measure the rotational diffusion in a monolayer of 1,2-Didecanoyl-sn-glycero-3-phosphocholine (DPPC) which displays a phase transition at room temperature from the liquid expanded to the liquid-condensed phase. The constant rotational diffusion of the probe throughout the phase transition reflects the measurement of dynamics in only the liquid-expanded phase. We contrast the dynamic changes during this phase coexistence to the continuous density increase observed in 1,2-dimyristoyl-sn-glycero-3-phosphocholine (DMPC) at room temperature. We observe a non-exponential decay of the probe diffusion consistent with heterogeneity …
A New Class Of Scalable Parallel Pseudorandom Number Generators Based On Pohlig-Hellman Exponentiation Ciphers, Paul Beale
Paul Beale
Parallel supercomputer-based Monte Carlo applications depend on pseudorandom number generators that produce independent pseudorandom streams across many separate processes. We propose a new scalable class of parallel pseudorandom number generators based on Pohlig--Hellman exponentiation ciphers. The method generates uniformly distributed floating point pseudorandom streams by encrypting simple sequences of integer \textit{messages} into \textit{ciphertexts} by exponentiation modulo prime numbers. The advantages of the method are: the method is trivially parallelizable by parameterization with each pseudorandom number generator derived from an independent prime modulus, the method is fully scalable on massively parallel computing clusters due to the large number of primes available …
Electrical Current In Sinai Billiards Under General Small Forces, Pengfei Zhang
Electrical Current In Sinai Billiards Under General Small Forces, Pengfei Zhang
Pengfei Zhang
No abstract provided.
Application Of The Transfer Matrix Method To Reflection Gratings In Positive And Negative Index Materials, Han Li
Han Li
No abstract provided.
On The Thresholds In Linear And Nonlinear Boolean Equations, Yifan Sun Dr
On The Thresholds In Linear And Nonlinear Boolean Equations, Yifan Sun Dr
Yifan Sun
No abstract provided.
Algebraic Characteristics And Satisfiability Threshold Of Random Boolean Equations, Binghui Guo Dr, Wei Wei Dr, Yifan Sun Dr, Zhiming Zheng Dr
Algebraic Characteristics And Satisfiability Threshold Of Random Boolean Equations, Binghui Guo Dr, Wei Wei Dr, Yifan Sun Dr, Zhiming Zheng Dr
Yifan Sun
No abstract provided.
Steady States Of A Nonequilibrium Lattice Gas, Edward Lyman, Beate Schmittmann
Steady States Of A Nonequilibrium Lattice Gas, Edward Lyman, Beate Schmittmann
Beate Schmittmann
We present a Monte Carlo study of a lattice gas driven out of equilibrium by a local hopping bias. Sites can be empty or occupied by one of two types of particles, which are distinguished by their response to the hopping bias. All particles interact via excluded volume and a nearest-neighbor attractive force. The main result is a phase diagram with three phases: a homogeneous phase and two distinct ordered phases. Continuous boundaries separate the homogeneous phase from the ordered phases, and a first-order line separates the two ordered phases. The three lines merge in a nonequilibrium bicritical point.
Exact Dynamics Of A Reaction-Diffusion Model With Spatially Alternating Rates, M. Mobilia, Beate Schmittmann, R. K. P. Zia
Exact Dynamics Of A Reaction-Diffusion Model With Spatially Alternating Rates, M. Mobilia, Beate Schmittmann, R. K. P. Zia
Beate Schmittmann
We present the exact solution for the full dynamics of a nonequilibrium spin chain and its dual reaction-diffusion model, for arbitrary initial conditions. The spin chain is driven out of equilibrium by coupling alternating spins to two thermal baths at different temperatures. In the reaction-diffusion model, this translates into spatially alternating rates for particle creation and annihilation, and even negative “temperatures” have a perfectly natural interpretation. Observables of interest include the magnetization, the particle density, and all correlation functions for both models. Two generic types of time dependence are found: if both temperatures are positive, the magnetization, density, and correlation …
Anomalous Nucleation Far From Equilibrium, I. T. Georgiev, Beate Schmittmann, R. K. P. Zia
Anomalous Nucleation Far From Equilibrium, I. T. Georgiev, Beate Schmittmann, R. K. P. Zia
Beate Schmittmann
We present precision Monte Carlo data and analytic arguments for an asymmetric exclusion process, involving two species of particles driven in opposite directions on a 2×L lattice. To resolve a stark discrepancy between earlier simulation data and an analytic conjecture, we argue that the presence of a single macroscopic cluster is an intermediate stage of a complex nucleation process: in smaller systems, this cluster is destabilized while larger systems form multiple clusters. Both limits lead to exponential cluster size distributions, controlled by very different length scales.
Driven Diffusive Systems: How Steady States Depend On Dynamics, D. P. Landau, Wooseop Kwak, Beate Schmittmann
Driven Diffusive Systems: How Steady States Depend On Dynamics, D. P. Landau, Wooseop Kwak, Beate Schmittmann
Beate Schmittmann
In contrast to equilibrium systems, nonequilibrium steady states depend explicitly on the underlying dynamics. Using Monte Carlo simulations with Metropolis, Glauber, and heat bath rates, we illustrate this expectation for an Ising lattice gas, driven far from equilibrium by an “electric” field. While heat bath and Glauber rates generate essentially identical data for structure factors and two-point correlations, Metropolis rates give noticeably weaker correlations, as if the “effective” temperature were higher in the latter case. We also measure energy histograms and define a simple ratio which is exactly known and closely related to the Boltzmann factor for the equilibrium case. …
Reply To “Comment On ‘Classical Density Functional Theory Of Freezing In Simple Fluids: Numerically Induced False Solutions’ ”, M. Valera, F. J. Pinski, Duane D. Johnson
Reply To “Comment On ‘Classical Density Functional Theory Of Freezing In Simple Fluids: Numerically Induced False Solutions’ ”, M. Valera, F. J. Pinski, Duane D. Johnson
Duane D. Johnson
Recently we solved, via discrete numerical grids, the Ramakrishna-Yossouff density-functional theory equations for the freezing transition and obtained an intricate phase diagram of hard-sphere mixtures. Even though such methods provide more variational freedom than basis-set methods, we found that the thermodynamic quantities were sensitive to the spacing of numerical grids employed and observed numerically induced false minima. Dasgupta and Valls have commented that these false minima were due to our use of k-space methods and, hence, their early works based on a fully r-space approach are qualitatively correct, despite also being sensitive to the mesh granularity. Here, we clarify the …
Stationary Correlations For A Far-From-Equilibrium Spin Chain, Beate Schmittmann, F. Schmüser
Stationary Correlations For A Far-From-Equilibrium Spin Chain, Beate Schmittmann, F. Schmüser
Beate Schmittmann
A kinetic one-dimensional Ising model on a ring evolves according to a generalization of Glauber rates, such that spins at even (odd) lattice sites experience a temperature Te (To). Detailed balance is violated so that the spin chain settles into a nonequilibrium stationary state, characterized by multiple interactions of increasing range and spin order. We derive the equations of motion for arbitrary correlation functions and solve them to obtain an exact representation of the steady state. Two nontrivial amplitudes reflect the sublattice symmetries; otherwise, correlations decay exponentially, modulo the periodicity of the ring. In the long-chain limit, they factorize into …
Classical Density Functional Theory Of Freezing In Simple Fluids: Numerically Induced False Solutions, M. Valera, F. J. Pinski, Duane D. Johnson
Classical Density Functional Theory Of Freezing In Simple Fluids: Numerically Induced False Solutions, M. Valera, F. J. Pinski, Duane D. Johnson
Duane D. Johnson
Density functional theory (DFT) has provided many insights into the freezing of simple fluids. Several analytical and numerical solution have shown that the DFT provides an accurate description of freezing of hard spheres and their mixtures. Compared to other techniques, numerical, grid-based algorithms for solving the DFT equations have more variational freedom and are capable of describing subtle behavior, as that seen in mixtures with multipeaked density profiles. However the grid-based approach is sensitive to the coarseness of the mesh employed. Here we summarize how the granularity of the mesh affects the freezing point within the DFT. For coarse meshes, …
Microscopic Kinetics And Time-Dependent Structure Factors, T. Aspelmeier, Beate Schmittmann, R. K. P. Zia
Microscopic Kinetics And Time-Dependent Structure Factors, T. Aspelmeier, Beate Schmittmann, R. K. P. Zia
Beate Schmittmann
The time evolution of structure factors (SF) in the disordering process of an initially phase-separated lattice depends crucially on the microscopic disordering mechanism, such as Kawasaki dynamics (KD) or vacancy-mediated disordering (VMD). Monte Carlo simulations show unexpected “dips” in the SFs. A phenomenological model is introduced to explain the dips in the odd SFs, and an analytical solution of KD is derived, in excellent agreement with simulations. The presence (absence) of dips in the even SFs for VMD (KD) marks a significant but not yet understood difference of the two dynamics.
Viability Of Competing Field Theories For The Driven Lattice Gas, Beate Schmittmann, H. K. Janssen, U. C. Tauber, R. K. P. Zia, K.-T. Leung, J. L. Cardy
Viability Of Competing Field Theories For The Driven Lattice Gas, Beate Schmittmann, H. K. Janssen, U. C. Tauber, R. K. P. Zia, K.-T. Leung, J. L. Cardy
Beate Schmittmann
It has recently been suggested that the driven lattice gas should be described by an alternate field theory in the limit of infinite drive. We review the original and the alternate field theory, invoking several well-documented key features of the microscopics. Since the alternate field theory fails to reproduce these characteristics, we argue that it cannot serve as a viable description of the driven lattice gas. Recent results, for the critical exponents associated with this theory, are reanalyzed and shown to be incorrect.
Universal Aspects Of Vacancy-Mediated Disordering Dynamics: The Effect Of External Fields, Wannapong Triampo, Timo Aspelmeier, Beate Schmittmann
Universal Aspects Of Vacancy-Mediated Disordering Dynamics: The Effect Of External Fields, Wannapong Triampo, Timo Aspelmeier, Beate Schmittmann
Beate Schmittmann
We investigate the disordering of an initially phase-segregated binary alloy, due to a highly mobile defect which couples to an electric or gravitational field. Using both mean-field and Monte Carlo methods, we show that the late stages of this process exhibit dynamic scaling, characterized by a set of exponents and scaling functions. A new scaling variable emerges, associated with the field. While the scaling functions carry information about the field and the boundary conditions, the exponents are universal. They can be computed analytically, in excellent agreement with simulation results.
Field-Induced Vacancy Localization In A Driven Lattice Gas: Scaling Of Steady States, M. Thies, Beate Schmittmann
Field-Induced Vacancy Localization In A Driven Lattice Gas: Scaling Of Steady States, M. Thies, Beate Schmittmann
Beate Schmittmann
With the help of Monte Carlo simulations and a mean-field theory, we investigate the ordered steady-state structures resulting from the motion of a single vacancy on a periodic lattice which is filled with two species of oppositely “charged” particles. An external field biases particle-vacancy exchanges according to the particle’s charge, subject to an excluded volume constraint. The steady state exhibits charge segregation, and the vacancy is localized at one of the two characteristic interfaces. Charge and hole density profiles, an appropriate order parameter, and the interfacial regions themselves exhibit characteristic scaling properties with system size and field strength. The lattice …
Structure Factors And Their Distributions In Driven Two-Species Models, G. Korniss, Beate Schmittmann
Structure Factors And Their Distributions In Driven Two-Species Models, G. Korniss, Beate Schmittmann
Beate Schmittmann
We study spatial correlations and structure factors in a three-state stochastic lattice gas, consisting of holes and two oppositely “charged” species of particles, subject to an “electric” field at zero total charge. The dynamics consists of two nearest-neighbor exchange processes, occurring on different times scales, namely, particle-hole and particle-particle exchanges. Using both Langevin equations and Monte Carlo simulations, we study the steady-state structure factors and correlation functions in the disordered phase, where density profiles are homogeneous. In contrast to equilibrium systems, the average structure factors here show a discontinuity singularity at the origin. The associated spatial correlation functions exhibit intricate …
Frozen Disorder In A Driven System, Beate Schmittmann, K. E. Bassler
Frozen Disorder In A Driven System, Beate Schmittmann, K. E. Bassler
Beate Schmittmann
We investigate the effects of quenched disorder on the universal properties of a randomly driven Ising lattice gas. The Hamiltonian fixed point of the pure system becomes unstable in the presence of a quenched local bias, giving rise to a new fixed point which controls a novel universality class. We determine the associated scaling forms of correlation and response functions, quoting critical exponents to two-loop order in an expansion around the upper critical dimension dc=5.
Phase Transitions In Driven Bilayer Systems: A Monte Carlo Study, C. C. Hill, R. K. P. Zia, Beate Schmittmann
Phase Transitions In Driven Bilayer Systems: A Monte Carlo Study, C. C. Hill, R. K. P. Zia, Beate Schmittmann
Beate Schmittmann
We investigate the phase diagram of a system with two layers of an Ising lattice gas at half filling. In addition to the usual intralayer nearest neighbor attractive interaction, there is an interlayer potential J. Under equilibrium conditions, the phase diagram is symmetric under J→−J, though the ground states are different. The effects of imposing a uniform external drive, studied by simulation techniques, are dramatic. The mechanisms responsible for such behavior are discussed.
Critical Dynamics Of Nonconserved Ising-Like Systems, K. E. Bassler, Beate Schmittmann
Critical Dynamics Of Nonconserved Ising-Like Systems, K. E. Bassler, Beate Schmittmann
Beate Schmittmann
We show that the dynamical fixed point of Ising-like models, characterized by a single scalar, nonconserved ordering field, is stable near four dimensions with respect to all dynamic perturbations, including those of a nonequilibrium nature.
Spontaneous Structure Formation In Driven Systems With Two Species: Exact Solutions In A Mean-Field Theory, I. Vilfan, R. K. P. Zia, Beate Schmittmann
Spontaneous Structure Formation In Driven Systems With Two Species: Exact Solutions In A Mean-Field Theory, I. Vilfan, R. K. P. Zia, Beate Schmittmann
Beate Schmittmann
A stochastic lattice gas of particles, subject to an excluded volume constraint and to a uniform external driving field, is investigated. Using a mean-field theory for a system with equal number of oppositely charged particles, exact results are obtained. Focusing on the current-vs-density plot, we propose an explanation for the discontinuous transition found in earlier simulations. A critical value of the drive, below which this transition becomes continuous, is found. These results are supported by a bifurcation analysis, leading to an equation of motion for the amplitude of the soft mode.