Physics Commons^™

Steady-State Switching And Dispersion/Absorption Spectroscopy Of Multistate Atoms Inside An Optical Ring Cavity, Jiteng Sheng

Graduate Theses and Dissertations

This thesis mainly focuses on the experimental investigations of electromagnetically induced transparency (EIT) related phenomena in various systems involving multilevel atoms inside an optical ring cavity. Semiclassical methods, e.g. density-matrix equations, are used through out this thesis to simulate the experimental results. First, the cavity transmission spectrum can be significantly modified when multilevel atoms are placed inside an optical ring cavity. Such coupled atom-cavity systems are well explained by the intracavity dispersion/absorption properties. Specifically, three-level lambda-type, four-level N-type and double-lambda-type atoms inside an optical ring cavity are investigated by examining their cavity transmission spectra. Second, optical multistability (OM) has been …

Resonant Enhancement Of The Harmonic-Generation Spectrum Of Beryllium, Jean Marcel Ngoko Djiokap, Anthony F. Starace

Anthony F. Starace Publications

The high-order harmonic-generation (HHG) spectrum of Be is investigated in the multiphoton regime by solving the full-dimensional, two-active-electron, time-dependent Schr¨odinger equation in an intense (≈10¹³ W/cm²), 30-cycle laser field. As the laser frequency ω_L varies from 1.7 to 1.8 eV (which is in the tunable range of a Ti:sapphire laser), the seventh harmonic becomes resonant sequentially with the transition between the ground state and two doubly excited autoionizing states, 2p4s(¹P) (at ω_L = 1.734 eV) and 2p5s …

Molecular Fluorescence In The Vicinity Of A Charged Metallic Nanoparticle, H. Y. Chung, P. T. Leung, D. P. Tsai

Physics Faculty Publications and Presentations

The modified fluorescence properties of a molecule in the vicinity of a metallic nanoparticle are further studied accounting for the possible existence of extraneous charges on the particle surface. This is achieved via a generalization of the previous theory of Bohren and Hunt for light scattering from a charged sphere, with the results applied to the calculation of the various decay rates and fluorescence yield of the admolecule. Numerical results show that while charge effects will in general blue-shift all the plasmonic resonances of the metal particle, both the quantum yield and the fluorescence yield can be increased at emission …

Carrier-Envelope-Phase-Induced Asymmetries In Double Ionization Of Helium By An Intense Few-Cycle Xuv Pulse, Jean Marcel Ngoko Djiokap, N. L. Manakov, A. V. Meremianin, Anthony F. Starace

Anthony F. Starace Publications

The carrier-envelope-phase (CEP) dependence of electron angular distributions in double ionization of He by an arbitrarily polarized, few-cycle, intense XUV pulse is formulated using perturbation theory (PT) in the pulse amplitude. Owing to the broad pulse bandwidth, interference of first- and second-order PT amplitudes produces asymmetric angular distributions sensitive to the CEP. The PT parametrization is shown to be valid by comparing with results of solutions of the full-dimensional, two-electron time-dependent Schrödinger equation for the case of linear polarization.

Harmonic Generation Spectroscopy With A Two-Colour Laser Field Having Orthogonal Linear Polarizations, T. S. Sarantseva, M. V. Frolov, N. L. Manakov, M. Yu. Ivanov, Anthony F. Starace

Anthony F. Starace Publications

The interpretation of many high-order harmonic generation (HHG) experiments is based on the assumption that the HHG yield of an atom can be factorized into (i) a laser-dependent ‘electron wave packet’ with rather simple properties, including a nearly universal shape, and (ii) an atomic photorecombination cross section. We show that this factorization is restricted to linearly polarized laser fields and fails in two-colour laser fields with orthogonal polarizations. At the same time, we show how two-colour HHG spectroscopy using orthogonally polarized intense fundamental and relatively weak second harmonic fields makes a complete experiment possible that enables the retrieval of the …

Multi-Level Surface Enhanced Raman Scattering Using AgoX Thin Film, Ming Lun Tseng, Chia Min Chang, Bo Han Cheng, Pin Chieh Wu, K. S. Chung, M. K. Hsiao, H. W. Huang, D. W. Huang, Hai-Pang Chiang, P.T. Leung, D. P. Tsai

Physics Faculty Publications and Presentations

Ag nanostructures with surface-enhanced Raman scattering (SERS) activities have been fabricated by applying laser-direct writing (LDW) technique on silver oxide (AgOx) thin films. By controlling the laser powers, multi-level Raman imaging of organic molecules adsorbed on the nanostructures has been observed. This phenomenon is further investigated by atomic-force microscopy and electromagnetic calculation. The SERS-active nanostructure is also fabricated on transparent and flexible substrate to demonstrate our promising strategy for the development of novel and low-cost sensing chip.

Visualization Of Optical Wave Propagation In Femtosecond Photoemission Electron Microscopy, Rolf Kӧnenkamp, Robert Campbell Word, Joseph Fitzgerald

Physics Faculty Publications and Presentations

Photoemission electron microscopy (PEEM) combines in a unique way photon probing and electron imaging. The imaging electrons are generated in a photoelectric process by illuminating the sample with ultra-violet or x-ray light. After generation these electrons are accelerated and introduced into an electron-optical system to produce a microscopic image of the specimen surface. The advantages of PEEM are manifold:

The avoidance of electron beam exposure makes PEEM a much gentler method than standard electron microscopy. This advantage is important when fragile organic or biological structures are studied. PEEM is also highly surface sensitive, since the photoelectrons typically escape the sample …

Atomistic Simulation Of Plasma Interaction With Plasma Facing Components In Fusion Reactors, Xue Yang

Open Access Dissertations

The interaction between plasma and fusion relevant materials is one of the critical issues in successfully using those materials in Tokamak reactors. This research uses molecular dynamics, kinetic Monte Carlo and binary collision approximation methods to model fusion relevant material bombarded by energetic particles to investigate retention, deposition, sputtering, erosion, blistering effects, diffusion, and so on.

The deuterium bombardment of monocrystalline tungsten was modeled by LAMMPS code using Tersoff type interatomic potential. The deuterium trapping rate, implantation depth, and stopping time in 600-2000 K tungsten bombarded by 5-100 eV deuterium atoms were simulated. Irradiated monocrystalline tungsten became amorphous prior to …

All-Optical Control Of Electron Trapping In Plasma Channels, Serguei Y. Kalmykov, Bradley A. Shadwick, Xavier Davoine

Serge Youri Kalmykov

The accelerating bucket of a laser-plasma accelerator (a cavity of electron density maintained by the laser pulse radiation pressure) evolves slowly, in lock-step with the optical driver, and readily traps background electrons. The trapping process can thus be controlled by purely optical means. Sharp gradients in the nonlinear refractive index produce a large frequency red-shift, localized at the leading edge of the pulse. Negative group velocity dispersion associated with the plasma response compresses the laser pulse into a relativistic optical shock (ROS), slowing the pulse (and the bucket), reducing the electron dephasing length, and limiting energy gain. Even more importantly, …

Fully Coupled Fluid And Electrodynamic Modeling Of Plasmas: A Two-Fluid Isomorphism And A Strong Conservative Flux-Coupled Finite Volume Framework, Richard Joel Thompson

Doctoral Dissertations

Ideal and resistive magnetohydrodynamics (MHD) have long served as the incumbent framework for modeling plasmas of engineering interest. However, new applications, such as hypersonic flight and propulsion, plasma propulsion, plasma instability in engineering devices, charge separation effects and electromagnetic wave interaction effects may demand a higher-fidelity physical model. For these cases, the two-fluid plasma model or its limiting case of a single bulk fluid, which results in a single-fluid coupled system of the Navier-Stokes and Maxwell equations, is necessary and permits a deeper physical study than the MHD framework. At present, major challenges are imposed on solving these physical models …

Feedback Stabilization At Spear3, Daniel Kelley, Jeff Corbett

STAR Program Research Presentations

The SPEAR3 synchrotron lightsource at SLAC relies on a sophisticated radio frequency (RF) timing system to maintain current – electrons – in the storage ring. One problem SPEAR3 operators have dealt with is the thermal expansion of one of the cables supporting this RF timing system. As the cable expands and contracts with the diurnal rise and fall of the sun, the phase of the RF in the cable shifts. This shifting phase affects the timing accuracy of electron injections into the storage ring.

A common feedback control algorithm PID (Proportional Integral Derivative) has countless applications in engineering. PID feedback …

Study Of A Non-Equilibrium Plasma Pinch With Application For Microwave Generation, Ahmad Al Agry

UNLV Theses, Dissertations, Professional Papers, and Capstones

The Non-Equilibrium Plasma Pinch (NEPP), also known as the Dense Plasma Focus (DPF) is well known as a source of energetic ions, relativistic electrons and neutrons as well as electromagnetic radiation extending from the infrared to X-ray. In this dissertation, the operation of a 15 kJ, Mather type, NEPP machine is studied in detail. A large number of experiments are carried out to tune the machine parameters for best performance using helium and hydrogen as filling gases. The NEPP machine is modified to be able to extract the copious number of electrons generated at the pinch. A hollow anode with …

Characterization Of Microwave Discharge Plasmas For Surface Processing, Milka Nikolic

Physics Theses & Dissertations

We have developed several diagnostic techniques to characterize two types of microwave (MW) discharge plasmas: a supersonic flowing argon MW discharge maintained in a cylindrical quartz cavity at frequency ƒ = 2.45 GHz and a pulse repetitive MW discharge in air at ƒ = 9.5 GHz. Low temperature MW discharges have been proven to posses attractive properties for plasma cleaning and etching of niobium surfaces of superconductive radio frequency (SRF) cavities. Plasma based surface modification technologies offer a promising alternative for etching and cleaning of SRF cavities. These technologies are low cost, environmentally friendly and easily controllable, and present a …

Asymmetries In Production Of He+(N = 2) With An Intense Few-Cycle Attosecond Pulse, Jean Marcel Ngoko Djiokap, S. X. Hu, Wei-Chao Jiang, Liang-You Peng, Anthony F. Starace

Anthony F. Starace Publications

By solving the two-electron time-dependent Schrödinger equation, we study carrier-envelope-phase (CEP) effects on ionization plus excitation of He to He⁺(n = 2) states by a few-cycle attosecond pulse with a carrier frequency of 51 eV. For most CEPs the asymmetries in the photoelectron angular distributions with excitation of He⁺(2s) or He⁺(2p) have opposite signs and are two orders of magnitude larger than for ionization without excitation. These results indicate that attosecond pulse CEP effects may be significantly amplified in correlated two-electron ionization processes.

A 3-D Model Of The Auroral Ionosphere, Yishi Lee

Doctoral Dissertations and Master's Theses

A new 3-D model of the high latitude ionosphere is developed to study the coupling of the ionosphere with the magnetosphere and neutral atmosphere. The model consists of equations describing conservations of mass, momentum and energy for the six ionospheric constituents (O+, NO+, N+2 , O+2 , N+ and e-) and an electrostatic potential equation. This 3-D model is used to examine interrelated processes of ion heating, plasma structuring due to perpendicular transport, ion upflow, molecular ion generation, and neutral wave forcing. It is first validated by comparisons with a 2-D model, which uses similar mathematical and numerical approaches, and …

Approximate Solutions For Diffusion Equations On Cantor Space-Time, Xiao-Jun Yang

Xiao-Jun Yang

In this paper we investigate diffusion equations on Cantor space-time and we obtain approximate solutions by using the local fractional Adomian decomposition method derived from the local fractional operators. Analytical solutions are given in terms of the Mittag-Leffler functions defined on Cantor sets.

A Numerical Algorithm For Simulating Two Species Plasma, Richard F. Datwyler

All Graduate Theses and Dissertations, Spring 1920 to Summer 2023

In our ever-growing technology-dependent society, a great need for cleaner, more lucrative energy sources is being sought out. Nuclear fission power plants have been used to help provide energy for many years now. More recently, fusion test reactors have been built and planned as another means to fill the energy quota. A large part of understanding the fundamental principles in a fusion reactor focuses on the principles of plasma physics. This topic of plasma physics has been studied for many decades and much progress has been made in its understanding.

More recently, computers have become larger and faster allowing for …

Plasmonic Nanostructures For The Absorption Enhancement Of Silicon Solar Cells, Nathan Matthias Burford

Graduate Theses and Dissertations

In this work, computational investigation of plasmonic nanostructures was conducted using the commercial finite element electromagnetics solver Ansys® HFSS. Arrays of silver toroid nanoparticles located on the surface of an amorphous silicon thin-film absorbing layer were studied for particle sizes ranging from 20 nm to 200 nm in outer diameter. Parametric optimization by calculating an approximation of the photocurrent enhancement due to the nanoparticles was performed to determine optimal surface coverage of the nanoparticles. A comparison was made between these optimized nanotoroid arrays and optimized nanosphere arrays based on spectral absorption enhancement and potential photocurrent enhancement in an amorphous silicon …

Parallel Heat Transport In Magnetized Plasma, Mukta Sharma

All Graduate Theses and Dissertations, Spring 1920 to Summer 2023

A huge global increase in energy use is inevitable, so there is an urgent need to seek cleaner ways of producing energy on large scales. Fusion is the energy source of the universe and a promising way to fulfill energy needs of mankind for many centuries to come. It offers important advantages as a safe, sustainable, and environmentally friendly source of energy. The International Thermonuclear Experimental Reactor (ITER) aims to demonstrate magnetic fusion is an energy source of the future. The goal of ITER is to produce 500 MW of fusion power given 50 MW of input power—or ten times …

Compositional And Structural Analysis Of Nitrogen Incorporated And Ion Implanted Diamond Thin Films, Elias James Garratt

Dissertations

Significant progress in area of nano-structured thin film systems has taken place in recent decades. In particular, diamond thin film systems are being widely studied for their wear resistant, optical and electronic properties. Of the various methods researchers use to modify the structure of such films, three techniques in particular are of interest due to their versatility: modification of the growth atmosphere, growth on metalized substrates, providing an interfacial layer, and modification through post-growth ion implantation. The aim of this study is to investigate the effects each has to the structure and composition of elements. Different techniques are applied in …

Stable, Tunable, Quasimonoenergetic Electron Beams Produced In A Laser Wakefield Near The Threshold For Self-Injection, Sudeep Banerjee, Serguei Y. Kalmykov, Nathan D. Powers, Gregory Golovin, Vidiya Ramanathan, Nathan J. Cunningham, Kevin J. Brown, Shouyuan Chen, Isaac Ghebregziabher, Bradley A. Shadwick, Donald P. Umstadter, Benjamin A. Cowan, David L. Bruhwiler, Arnaud Beck, Erik Lefebvre

Donald P. Umstadter

Stable operation of a laser-plasma accelerator near the threshold for electron self-injection in the blowout regime has been demonstrated with 25–60 TW, 30 fs laser pulses focused into a 3–4 millimeter length gas jet. Nearly Gaussian shape and high nanosecond contrast of the focused pulse appear to be critically important for controllable, tunable generation of 250–430 MeV electron bunches with a low energy spread, ~ 10 pC charge, a few-mrad divergence and pointing stability, and a vanishingly small low-energy background. The physical nature of the near-threshold behavior is examined using three-dimensional particle-in-cell simulations. Simulations indicate that properly locating the nonlinear …

Stable, Tunable, Quasimonoenergetic Electron Beams Produced In A Laser Wakefield Near The Threshold For Self-Injection, Sudeep Banerjee, Serguei Y. Kalmykov, Nathan D. Powers, Gregory Golovin, Vidiya Ramanathan, Nathan J. Cunningham, Kevin J. Brown, Shouyuan Chen, Isaac Ghebregziabher, Bradley A. Shadwick, Donald P. Umstadter, Benjamin A. Cowan, David L. Bruhwiler, Arnaud Beck, Erik Lefebvre

Serge Youri Kalmykov

Stable operation of a laser-plasma accelerator near the threshold for electron self-injection in the blowout regime has been demonstrated with 25–60 TW, 30 fs laser pulses focused into a 3–4 millimeter length gas jet. Nearly Gaussian shape and high nanosecond contrast of the focused pulse appear to be critically important for controllable, tunable generation of 250–430 MeV electron bunches with a low energy spread, ~ 10 pC charge, a few-mrad divergence and pointing stability, and a vanishingly small low-energy background. The physical nature of the near-threshold behavior is examined using three-dimensional particle-in-cell simulations. Simulations indicate that properly locating the nonlinear …

Measurements Of Nh3 Linestrengths And Collisional Broadening Coefficients In N2, O2, Co2, And H2o Near 1103.46 Cm−1, Kyle Owen, Et-Touhami Es-Sebbar, Aamir Farooq

Dr. Et-touhami Es-sebbar

Laser-based ammonia gas sensors have useful applications in many fields including combustion, atmospheric monitoring, and medical diagnostics. Calibration-free trace gas sensors require the spectroscopic parameters including linestrengths and collisional broadening coefficients to be known. Ammonia's strong ν2 vibrational band between View the MathML source has the high absorption strength needed for sensing small concentrations. Within this band, the 1103.46 cm−1 feature is one of the strongest and has minimal interference from CO2 and H2O. However, the six rotational transitions that make up this feature have not been studied previously with absorption spectroscopy due to their small line spacing ranging from …

Dark-Current-Free Laser-Plasma Acceleration In Blowout Regime Using Nonlinear Plasma Lens, Serguei Y. Kalmykov

Serge Youri Kalmykov

It is demonstrated that a thin dense plasma slab (lens), placed before a multi-centimeter-length, low-density plasma (accelerator), overfocuses an incident petawatt laser pulse at a controlled location inside the accelerator, creating an expanding electron density bubble that traps plasma electrons over a brief time interval. As soon as the pulse stabilizes and self-guiding begins, the bubble stabilizes and transforms into the first (non-broken) bucket of a conventional three-dimensional nonlinear plasma wave, eliminating any chance for further injection. A well collimated, quasi-monoenergetic electron bunch with a zero low-energy background further accelerates to a multi-GeV energy.

Effects Of N2o And O2 Addition To Nitrogen Townsend Dielectric Barrier Discharges At Atmospheric Pressure On The Absolute Ground-State Atomic Nitrogen Density, Et. Es-Sebbar, N. Gherardi, F. Massines

Dr. Et-touhami Es-sebbar

Absolute ground-state density of nitrogen atoms N (2p3 4S3/2) in non-equilibrium Townsend dielectric barrier discharges (TDBDs) at atmospheric pressure sustained in N2/N2O and N2/O2 gas mixtures has been measured using Two-photon absorption laser-induced fluorescence (TALIF) spectroscopy. The quantitative measurements have been obtained by TALIF calibration using krypton as a reference gas. We previously reported that the maximum of N (2p3 4S3/2) atom density is around 3 × 1014 cm−3 in pure nitrogen TDBD, and that this maximum depends strongly on the mean energy dissipated in the gas. In the two gas mixtures studied here, results show that the absolute N …

Mechanical Analysis Of The 400 Mhz Rf-Dipole Crabbing Cavity Prototype For Lhc High Luminosity Upgrade, S. U. De Silva, H. Park, J. R. Delayen, Z. Li

Physics Faculty Publications

The proposed LHC high luminosity upgrade requires two crabbing systems in increasing the peak luminosity, operating both vertically and horizontally at two interaction points of IP1 and IP5. The required system has tight dimensional constraints and needs to achieve higher operational gradients. A proof-of-principle 400 MHz crabbing cavity design has been successfully tested and has proven to be an ideal candidate for the crabbing system. The cylindrical proof-of-principle rf-dipole design has been adapted in to a square shaped design to further meet the dimensional requirements. The new rf-dipole design has been optimized in meeting the requirements in rf-properties, higher order …

Analytic Description Of Elastic Electron-Atom Scattering In An Elliptically Polarized Laser Field, A. V. Flegel, M. V. Frolov, N. L. Manakov, Anthony F. Starace, A. N. Zheltukhin

Anthony F. Starace Publications

An analytic description of laser-assisted electron-atom scattering (LAES) in an elliptically polarized field is presented using time-dependent effective range (TDER) theory to treat both electron-laser and electron-atom interactions nonperturbatively. Closed-form formulas describing plateau features in LAES spectra are derived quantum mechanically in the low-frequency limit. These formulas provide an analytic explanation for key features of the LAES differential cross section. For the low-energy region of the LAES spectrum, our result generalizes the Kroll-Watson formula to the case of elliptic polarization. For the high-energy (rescattering) plateau in the LAES spectrum, our result generalizes prior results for a linearly polarized field valid …

Multipole Field Effects For The Superconducting Parallel-Bar/Rf-Dipole Deflecting/Crabbing Cavities, S. U. De Silva, J. R. Delayen

Physics Faculty Publications

The superconducting parallel-bar deflecting/crabbing cavity is currently being considered as one of the design options in rf separation for the Jefferson Lab 12 GeV upgrade and for the crabbing cavity for the proposed LHC luminosity upgrade. Knowledge of multipole field effects is important for accurate beam dynamics study of rf structures. The multipole components can be accurately determined numerically using the electromagnetic surface field data in the rf structure. This paper discusses the detailed analysis of those components for the fundamental deflecting/crabbing mode and higher order modes in the parallel-bar deflecting/crabbing cavity.

Geometry Effects On Multipole Components And Beam Optics In High-Velocity Multi-Spoke Cavities, C. S. Hopper, K. Deitrick, J. R. Delayen

Physics Faculty Publications

Velocity-of-light, multi-spoke cavities are being proposed to accelerate electrons in a compact light-source [1]. There are strict requirements on the beam quality which require that the linac have only small non-uniformities in the accelerating field. Beam dynamics simulations have uncovered varying levels of focusing and defocusing in the proposed cavities, which is dependent on the geometry of the spoke in the vicinity of the beam path. Here we present results for the influence different spoke geometries have on the multipole components of the accelerating field and how these components, in turn, impact the simulated beam properties.

Study Of Cavity Imperfection Impact On Rf-Parameters And Multipole Components In A Superconducting Rf-Dipole Cavity, R. G. Olave, J. R. Delayen, S. U. De Silva, Z. Li

Physics Faculty Publications

The ODU/SLAC superconducting rf-dipole cavity is under consideration for the crab-crossing system in the upcoming LHC luminosity upgrade. While the proposed cavity complies well within the rf-parameters and multipolar component restrictions for the LHC system, cavity imperfections arising from cavity fabrication, welding and frequency tuning may have a significant effect in these parameters. We report on an initial study of the impact of deviation from the ideal shape on the cavity’s performance in terms of rf-parameters and multipolar components.