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Physical Chemistry

Wayne State University

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Fundamental Studies And Applications Of Strong Field Ionization, Lu Yan Jan 2013

Fundamental Studies And Applications Of Strong Field Ionization, Lu Yan

Wayne State University Dissertations

In an intense laser field, atoms and molecules experience tunneling ionization directly to the continuum. We used this method to study several aspects and applications of strong field ionization (SFI) in atoms and molecules. One study used SFI to probe the photofragments produced by photodissociation using DC sliced imaging. The photodissociation mechanism of two polyatomic molecules (sulfur dioxide and nitromethane) were investigated. In a second study, we show the strong field ionization rate depends on the sign of the magnetic number distribution. We detect the signal of sequential double ionization of argon dications by a pump-probe method to investigate the …