Physics Commons^™

A Study Of Optical Nonlinearities At The Single-Photon Level For Quantum Logic, Balakrishnan Viswanathan

Graduate Theses and Dissertations

In this dissertation, we shall focus on theoretically studying quantum nonlinear optical schemes to construct a conditional phase gate at the single-photon level. With an aim to develop analytical models, we shall carry out a rigorous quantized multimode field analysis of some of these schemes involving only the interacting field operators. More specifically, we shall first study the three-wave mixing process involving two single-photons in a second-order nonlinear medium (x(2)) under two different cases viz. when the photons are traveling with equal velocities and when they are traveling with different velocities, and explore the possibility of using them for building …

Infrared Energy Conversion In Plasmonic Fields At Two-Dimensional Semiconductors, Gregory Thomas Forcherio

Graduate Theses and Dissertations

Conversion of infrared energy within plasmonic fields at two-dimensional, semiconductive transition metal dichalcogenides (TMD) through plasmonic hot electron transport and nonlinear frequency mixing has important implications in next-generation optoelectronics. Drude-Lorentz theory and approximate discrete dipole (DDA) solutions to Maxwell’s equations guided metal nanoantenna design towards strong infrared localized surface plasmon resonance (LSPR). Excitation and damping dynamics of LSPR in heterostructures of noble metal nanoantennas and molybdenum- or tungsten-disulfide (MoS2; WS2) monolayers were examined by parallel synthesis of (i) DDA electrodynamic simulations and (ii) near-field electron energy loss (EELS) and far-field optical transmission UV-vis spectroscopic measurements. Susceptibility to second-order nonlinear frequency …

Measuring Nonlinear Properties Of Graphene Thin Films Using Z-Scan Technique, Thekrayat Hassan Al Abdulaal

Graduate Theses and Dissertations

The nonlinear studies of two-dimensional (2D) nanomaterials, specifically graphene, are very significant since graphene is finding its usefulness in handling the enormous heat in nanoscale high-density power electronics. Graphene has emerged to be a promising nanomaterial as an excellent heat spreader due to its high thermal conductivity. However, the experimental nonlinear study of graphene materials and their application in developing future optoelectronic devices demands for more developed research.

The research objective is first to build a precise, and sensitive technique to investigate and understand the thermal nonlinear properties, including nonlinear refractive index (n2), nonlinear absorption coefficient (β), and thermo-optic coefficient …

Phase Control In Atomic Coherence, Utsab Khadka

Graduate Theses and Dissertations

In this thesis, atomic coherence is used to enhance nonlinear optical processes in multi-level atoms. The multi-photon transitions are driven resonantly, and at the same time without absorptive losses, by using electromagnetically induced transparency (EIT), thereby allowing the study of χ⁽³⁾ and χ⁽⁵⁾ nonlinearities using weak driving fields. The coherently modified probe beam(s) and the atom-radiated signal fields arising from four- and six- wave- mixing (FWM and SWM) processes are measured in the spectral, temporal and spatial domains.

In a three-level ladder-type atomic system, multiple peaks having spectral asymmetries are observed in the EIT window as well as …

Imaging Second-Harmonic Radiation And Scattering Patterns In Zno Micro/Nanostructures, Katrina Marie Geren

Graduate Theses and Dissertations

The optical characteristics of ZnO nanostructures have recently garnered interest due to the inclusion of these structures in many nanoscale optical and optoelectronic devices. This thesis will address several characteristics involving second harmonic generation and scattering in ZnO nano- and microstructures. A method will be presented for determining the nonlinear coefficients of the second order susceptibility in a single ZnO rod. This method uses transmission geometry where previous methods have employed back-reflected irradiation. The nonlinear coefficients found using this new technique were consistent with previous data from similar structures. Models will be presented for predicting the second harmonic scattering patterns …