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Full-Text Articles in Physics

Hyperpolarizability Dispersion Measured For Carbon Disulfide Vapor, Rodrigo N. Fernandez Aug 2021

Hyperpolarizability Dispersion Measured For Carbon Disulfide Vapor, Rodrigo N. Fernandez

UNLV Theses, Dissertations, Professional Papers, and Capstones

The second hyperpolarizability (γ) of carbon disulfide (CS2) was measured by gas phase electric-field-induced second harmonic generation (ESHG), for laser wavelengths in the range of 765-1064 nm. The observed hyperpolarizability is decomposed into electronic (γ^e) and vibrational (γ^v) contributions, and the dispersion curve for γ^eis extrapolated to the static limit, with the result γ^e_0 = 12558 ± 93 atomic units. The results of this experiment agree with other recent nonlinear optical measurements and theoretical calculations.


Vibration Overtone Hyperpolarizability Measured For H2 Using Electric Field Induced Second Harmonic Generation, Rachel Ellis Dec 2020

Vibration Overtone Hyperpolarizability Measured For H2 Using Electric Field Induced Second Harmonic Generation, Rachel Ellis

UNLV Theses, Dissertations, Professional Papers, and Capstones

The vibrational contribution to the second hyperpolarizability (γ) of gas phase H2 was measured using electric field induced second harmonic generation. Measurements were made for the pure vibrational 3-0 Q(J) overtone transitions (v=0,J → v’=3,J for J = 0,1,2,3). Measured intensities were found to be 4-14% larger than ab initio calculations. The first chapter of this thesis provides an introduction to nonlinear optics, second harmonic generation, and the tensor nature of hyperpolarizabilities. The second chapter provides theoretical expressions for γ and relevant static and Raman polarizabilities. The third chapter covers the experimental design and electric field induced second harmonic generation. …


Development Of Co2 Laser-Heating For The Study Of Wide Band Gap Oxide Materials, Christian Matthew Childs May 2020

Development Of Co2 Laser-Heating For The Study Of Wide Band Gap Oxide Materials, Christian Matthew Childs

UNLV Theses, Dissertations, Professional Papers, and Capstones

The ability to access a vast region of the pressure-temperature landscape using energy density tuning enables exotic states of matter to be probed. A well documented method for such exploration, under static conditions, is the use of the laser-heated diamond anvil cell (LH-DAC), accessing a combination of high pressure (>300 GPa) and high temperature (>5000 K). This thesis presents our development of direct CO2 laser heating techniques to study a series of wide band gap insulators, La2Sn2O7, ZrO2, and CeO2, under high pressure conditions. The lasing frequency of CO2 lasers is such that these wide band gap materials …


High-Pressure High-Temperature Exploration Of Phase Boundaries Using Raman Spectroscopy, Jasmine Kashmir Hinton May 2019

High-Pressure High-Temperature Exploration Of Phase Boundaries Using Raman Spectroscopy, Jasmine Kashmir Hinton

UNLV Theses, Dissertations, Professional Papers, and Capstones

Metastability of states can provide interesting properties that may not be readily accessible in a material’s ground state. Many materials show high levels of polymorphism, indicating a rich energy landscape and a potential for metastable states. Melt crystallization techniques provide a potential route to these states. We use a resistively heated diamond anvil cell (DAC) with fine control of a system’s pressure and temperature to explore these systems. Raman spectroscopy is used to track subtle structural changes across phase boundaries. Organic systems, such as glycine and aspirin, were our initial interest due to their high polymorphism and reported low melting …


Design And Fabrication Of An Infrared Optical Pyrometer Asic As A Diagnostic For Shock Physics Experiments, Jared Gordon Dec 2013

Design And Fabrication Of An Infrared Optical Pyrometer Asic As A Diagnostic For Shock Physics Experiments, Jared Gordon

UNLV Theses, Dissertations, Professional Papers, and Capstones

Optical pyrometry is the sensing of thermal radiation emitted from an object using a photoconductive device to convert photons into electrons, and is an important diagnostic tool in shock physics experiments. Data obtained from an optical pyrometer can be used to generate a blackbody curve of the material prior to and after being shocked by a high speed projectile. The sensing element consists of an InGaAs photodiode array, biasing circuitry, and multiple transimpedance amplifiers to boost the weak photocurrent from the noisy dark current into a signal that can eventually be digitized. Once the circuit elements have been defined, more …


High-Performance, Scalable Optical Network-On-Chip Architectures, Xianfang Tan Aug 2013

High-Performance, Scalable Optical Network-On-Chip Architectures, Xianfang Tan

UNLV Theses, Dissertations, Professional Papers, and Capstones

The rapid advance of technology enables a large number of processing cores to be integrated into a single chip which is called a Chip Multiprocessor (CMP) or a Multiprocessor System-on-Chip (MPSoC) design. The on-chip interconnection network, which is the communication infrastructure for these processing cores, plays a central role in a many-core system. With the continuously increasing complexity of many-core systems, traditional metallic wired electronic networks-on-chip (NoC) became a bottleneck because of the unbearable latency in data transmission and extremely high energy consumption on chip. Optical networks-on-chip (ONoC) has been proposed as a promising alternative paradigm for electronic NoC with …


Spectroscopic Studies Of Melamine At High Pressure, Martin Donald Galley Dec 2011

Spectroscopic Studies Of Melamine At High Pressure, Martin Donald Galley

UNLV Theses, Dissertations, Professional Papers, and Capstones

We have performed mid- and far- Infra Red (IR) absorption, Raman spectroscopy, and angular dispersive x-ray diffraction (XRD) studies on melamine under high pressure and room temperature. We have verified the presence of two prior reported phase transitions, the first between 1-2 GPa, and the second between 7-9 GPa. We have also found evidence of a third unreported phase transition between 14-16 GPa, during which, there was a sudden disappearance of all low energy peaks (-1 ) in both the Raman and IR spectra. The far-IR peak movement experiences a discontinuity as the rate of peak movement suddenly changes. …


Thin Film Optical Filter Fabrication And Characterization, Adam G. Hammouda, David P. Shelton Aug 2010

Thin Film Optical Filter Fabrication And Characterization, Adam G. Hammouda, David P. Shelton

Undergraduate Research Opportunities Program (UROP)

Thin film coatings have a large number of applications. For example, one can eliminate unwanted reflection on a photographic lens or unwanted wavelengths of light in optics experimentation. The fabrication and characterization of films whose refractive indices can be arbitrarily modulated (‘Rugate Filters’) is an ongoing exploration in materials science1,2. Therefore, calibrating a process which can manufacture such films is a relevant pursuit in forwarding such explorations. Reactive magnetron sputter deposition is a commonly used technique for the productions of thin films3,4. This technique steadily flows reactive gas (RG) into a vacuum chamber in which an electric field has been …