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Full-Text Articles in Physics
Directly Photoexcited Dirac And Weyl Fermions In Zrsis And Nbas, Christopher P. Weber, Leslie M. Schoop, Stuart S. P. Parkin, Robert C. Newby, Alex Nateprov, Bettina Lotsch, Bala Murali Krishna Mariserla, J. Matthew Kim, Keshav M. Dani, Hans A. Bechtel, Ernerst Arushanov, Mazhar Ali
Directly Photoexcited Dirac And Weyl Fermions In Zrsis And Nbas, Christopher P. Weber, Leslie M. Schoop, Stuart S. P. Parkin, Robert C. Newby, Alex Nateprov, Bettina Lotsch, Bala Murali Krishna Mariserla, J. Matthew Kim, Keshav M. Dani, Hans A. Bechtel, Ernerst Arushanov, Mazhar Ali
Physics
We report ultrafast optical measurements of the Dirac line-node semimetal ZrSiS and the Weyl semimetal NbAs, using mid-infrared pump photons from 86 meV to 500 meV to directly excite Dirac and Weyl fermions within the linearly dispersing bands. In NbAs, the photoexcited Weyl fermions initially form a non-thermal distribution, signified by a brief spike in the differential reflectivity whose sign is controlled by the relative energy of the pump and probe photons. In ZrSiS, electron-electron scattering rapidly thermalizes the electrons, and the spike is not observed. Subsequently, hot carriers in both materials cool within a few picoseconds. This cooling, as …
Using Coherent Phonons For Ultrafast Control Of The Dirac Node Of Srmnsb2, Christopher P. Weber, Madison G. Masten, Thomas C. Ogloza, Bryan S. Berggren, Michael K. L. Man, Keshav M. Dani, Jinyu Liu, Zhiqiang Mao, Dennis D. Klug, Adebayo A. Adeleke, Yansun Yao
Using Coherent Phonons For Ultrafast Control Of The Dirac Node Of Srmnsb2, Christopher P. Weber, Madison G. Masten, Thomas C. Ogloza, Bryan S. Berggren, Michael K. L. Man, Keshav M. Dani, Jinyu Liu, Zhiqiang Mao, Dennis D. Klug, Adebayo A. Adeleke, Yansun Yao
Physics
SrMnSb2 is a candidate Dirac semimetal whose electrons near the Y point have the linear dispersion and low mass of a Dirac cone. Here we demonstrate that ultrafast, 800-nm optical pulses can launch coherent phonon oscillations in Sr0.94Mn0.92Sb2, particularly an Ag mode at 4.4 THz. Through first-principles calculations of the electronic and phononic structure of SrMnSb2, we show that high-amplitude oscillations of this mode would displace the atoms in a way that transiently opens and closes a gap at the node of the Dirac cone. The ability to control the …
Similar Ultrafast Dynamics Of Several Dissimilar Dirac And Weyl Semimetals, Christopher P. Weber, Bryan S. Berggren, Madison G. Masten, Thomas C. Ogloza, Skylar Deckoff-Jones, Julien Madéo, Michael K. L. Man, Keshav M. Dani, Lingxiao Zhao, Genfu Chen, Jinyu Liu, Zhiqiang Mao, Leslie M. Schoop, Bettina V. Lotsch, Stuart S. P. Parkin, Mazhar Ali
Similar Ultrafast Dynamics Of Several Dissimilar Dirac And Weyl Semimetals, Christopher P. Weber, Bryan S. Berggren, Madison G. Masten, Thomas C. Ogloza, Skylar Deckoff-Jones, Julien Madéo, Michael K. L. Man, Keshav M. Dani, Lingxiao Zhao, Genfu Chen, Jinyu Liu, Zhiqiang Mao, Leslie M. Schoop, Bettina V. Lotsch, Stuart S. P. Parkin, Mazhar Ali
Physics
Recent years have seen the rapid discovery of solids whose low-energy electrons have a massless, linear dispersion, such as Weyl, line-node, and Dirac semimetals. The remarkable optical properties predicted in these materials show their versatile potential for optoelectronic uses. However, little is known of their response in the picoseconds after absorbing a photon. Here, we measure the ultrafast dynamics of four materials that share non-trivial band structure topology but that differ chemically, structurally, and in their low-energy band structures: ZrSiS, which hosts a Dirac line node and Dirac points; TaAs and NbP, which are Weyl semimetals; and Sr1–y …
Ambipolar Spin Diffusion In P-Type Gaas: A Case Where Spin Diffuses More Than Charge, F. Cadiz, V. Notot, J. Filipovic, Christopher P. Weber, L. Martinelli, A.C. H. Rowe, S. Arscott
Ambipolar Spin Diffusion In P-Type Gaas: A Case Where Spin Diffuses More Than Charge, F. Cadiz, V. Notot, J. Filipovic, Christopher P. Weber, L. Martinelli, A.C. H. Rowe, S. Arscott
Physics
We investigate the diffusion of charge and spin at 15 K in p-type GaAs, combining transient-grating and energy-resolved microluminescence measurements to cover a broad range of photoelectron density. At very low optical power, in a unipolar nondegenerate regime, charge and spin diffuse at the same rate, implying that the spin-drag effects are negligible. Upon increasing the photoelectron concentration up to about 1016 cm–3, the charge diffusion constant decreases because of ambipolar electrostatic interactions with the slower-diffusing holes while the spin diffusion constant is reduced only weakly by the ambipolar interaction. A further increase in the excitation power causes increases in …
Room-Temperature Self-Powered Energy Photodetector Based On Optically Induced Seebeck Effect In Cd3As2, Niloufar Yavarishad, Tahereh Hosseini, Elaheh Kheirandish, Christopher P. Weber, Nikolai Kouklin
Room-Temperature Self-Powered Energy Photodetector Based On Optically Induced Seebeck Effect In Cd3As2, Niloufar Yavarishad, Tahereh Hosseini, Elaheh Kheirandish, Christopher P. Weber, Nikolai Kouklin
Physics
We demonstrate an intrinsically fast Seebeck-type metal–semimetal–metal infrared photodetector based on Cd3As2 crystals. The Seebeck voltage is induced under off-center illumination, leading to asymmetric temperature gradients and a net current flow. The room-temperature responsivity of the sensor is 0.27 mA/W. The photocurrent signal is readily registered at a modulation frequency of 6 kHz, and the intrinsic bandwidth of the sensor is predicted to approach the terahertz range. The photocurrent depends on the optical power and modulation frequency. Our study demonstrates that crystallineCd3As2 is a promising material for high-bandwidth and spectrally broad photosensing, imaging, and …
Transient Reflectance Of Photoexcited Cd3As2, Christopher P. Weber, Ernest Arushanov, Bryan S. Berggren, Tahereh Hosseini, Nikolai Kouklin, Alex Nateprov
Transient Reflectance Of Photoexcited Cd3As2, Christopher P. Weber, Ernest Arushanov, Bryan S. Berggren, Tahereh Hosseini, Nikolai Kouklin, Alex Nateprov
Physics
We report ultrafast transient-grating measurements of crystals of the three-dimensional Dirac semimetal cadmium arsenide, Cd3As2, at both room temperature and 80 K. After photoexcitation with 1.5-eV photons, charge-carriers relax by two processes, one of duration 500 fs and the other of duration 3.1 ps. By measuring the complex phase of the change in reflectance, we determine that the faster signal corresponds to a decrease in absorption, and the slower signal to a decrease in the light's phase velocity, at the probe energy. We attribute these signals to electrons' filling of phase space, first near the photon …
Rapid Diffusion Of Electrons In Gamnas, Christopher P. Weber, Eric A. Kittlaus, Kassandra B. Mattia, Christopher J. Waight, J. Hagmann, X. Liu, M. Dobrowolska, J. K. Furdyna
Rapid Diffusion Of Electrons In Gamnas, Christopher P. Weber, Eric A. Kittlaus, Kassandra B. Mattia, Christopher J. Waight, J. Hagmann, X. Liu, M. Dobrowolska, J. K. Furdyna
Physics
We report ultrafast transient‐grating measurements, above and below the Curie temperature, of the dilute ferromagnetic semiconductor (Ga,Mn)As containing 6% Mn. At 80 K (15 K), we observe that photoexcited electrons in the conduction band have a lifetime of 8 ps (5 ps) and diffuse at about 70 cm2/s (60 cm2/s). Such rapid diffusion requires either an electronic mobility exceeding 7700 cm2/V s or a conduction‐band effective mass less than half the GaAs value. Our data suggest that neither the scattering rate nor the effective mass of the (Ga,Mn)As conduction band differs significantly from that …
Diffusion Of Degenerate Minority Carrier In A P-Type Semiconductor, Christopher P. Weber, Eric A. Kittlaus
Diffusion Of Degenerate Minority Carrier In A P-Type Semiconductor, Christopher P. Weber, Eric A. Kittlaus
Physics
We report ultrafast transient-grating experiments on heavily p-type InP at 15 K. Our measurement reveals the dynamics and diffusion of photoexcited electrons and holes as a function of their density n in the range 2 × 1016 to 6 × 1017 cm−3. After the first few picoseconds, the grating decays primarily due to ambipolar diffusion. While, at low density, we observe a regime in which the ambipolar diffusion is electron-dominated and increases rapidly with n, it appears to saturate at 34 cm2/s at high n. We present a simple calculation that reproduces the main …
Measurement Of Spin Diffusion In Semi-Insulating Gaas, Christopher P. Weber, Craig A. Benko, Stanley C. Hiew
Measurement Of Spin Diffusion In Semi-Insulating Gaas, Christopher P. Weber, Craig A. Benko, Stanley C. Hiew
Physics
We use optical transient-grating spectroscopy to measure the spin diffusion of optically oriented electrons in bulk, semi-insulating GaAs(100). Trapping and recombination do not quickly deplete the photoexcited population. The spin diffusion coefficient of 88±12 cm2/s is roughly constant at temperatures from 15 K to 150 K, and the spin diffusion length is at least 450 nm. We show that it is possible to use spin diffusion to estimate the electron diffusion coefficient. Due to electron-electron interactions, the electron diffusion is 1.4 times larger than the spin diffusion.
Electronic Structure Of Warm Dense Copper Studied By Ultrafast X-Ray Absorption Spectroscopy, B. I. Cho, K. Engelhorn, A. A. Correa, T. Ogitsu, Christopher P. Weber, H. J. Lee, J. Feng, P. A. Ni, Y. Ping, A. J. Nelson, D. Prendergast, R. W. Lee, R. W. Falcone, P. A. Heimann
Electronic Structure Of Warm Dense Copper Studied By Ultrafast X-Ray Absorption Spectroscopy, B. I. Cho, K. Engelhorn, A. A. Correa, T. Ogitsu, Christopher P. Weber, H. J. Lee, J. Feng, P. A. Ni, Y. Ping, A. J. Nelson, D. Prendergast, R. W. Lee, R. W. Falcone, P. A. Heimann
Physics
We use time-resolved x-ray absorption spectroscopy to investigate the unoccupied electronic density of states of warm dense copper that is produced isochorically through the absorption of an ultrafast optical pulse. The temperature of the superheated electron-hole plasma, which ranges from 4000 to 10 000 K, was determined by comparing the measured x-ray absorption spectrum with a simulation. The electronic structure of warm dense copper is adequately described with the high temperature electronic density of state calculated by the density functional theory. The dynamics of the electron temperature is consistent with a two-temperature model, while a temperature-dependent electron-phonon coupling parameter is …
A Grazing Incidence X-Ray Streak Camera For Ultrafast, Single-Shot Measurements, J. Feng, K. Engelhorn, B. I. Cho, H. J. Lee, M. Greaves, Christopher P. Weber, R. W. Falcone, H. A. Padmore, P. A. Heimann
A Grazing Incidence X-Ray Streak Camera For Ultrafast, Single-Shot Measurements, J. Feng, K. Engelhorn, B. I. Cho, H. J. Lee, M. Greaves, Christopher P. Weber, R. W. Falcone, H. A. Padmore, P. A. Heimann
Physics
An ultrafast x-ray streak camera has been realized using a grazing incidence reflection photocathode. X-rays are incident on a gold photocathode at a grazing angle of 20° and photoemitted electrons are focused by a large aperture magnetic solenoid lens. The streak camera has high quantum efficiency, 600 fs temporal resolution, and 6 mm imaging length in the spectral direction. Its single shot capability eliminates temporal smearing due to sweep jitter, and allows recording of the ultrafast dynamics of samples that undergo nonreversible changes.
Emergence Of The Persistent Spin Helix In Semiconductor Quantum Wells, J. D. Koralek, Christopher P. Weber, J. Orenstein, B. Andrei Bernevig, Shou-Cheng Zhang, S. Mack, D. D. Awschalom
Emergence Of The Persistent Spin Helix In Semiconductor Quantum Wells, J. D. Koralek, Christopher P. Weber, J. Orenstein, B. Andrei Bernevig, Shou-Cheng Zhang, S. Mack, D. D. Awschalom
Physics
According to Noether’s theorem1, for every symmetry in nature there is a corresponding conservation law. For example, invariance with respect to spatial translation corresponds to conservation of momentum. In another well-known example, invariance with respect to rotation of the electron’s spin, or SU(2) symmetry, leads to conservation of spin polarization. For electrons in a solid, this symmetry is ordinarily broken by spin–orbit coupling, allowing spin angular momentum to flow to orbital angular momentum. However, it has recently been predicted that SU(2) can be achieved in a two-dimensional electron gas, despite the presence of spin–orbit coupling2. The …
Nondiffusive Spin Dynamics In A Two-Dimensional Electron Gas, Christopher P. Weber, J. Orenstein, B. Andrei Bernevig, Shou-Cheng Zhang, Jason Stephens, D. D. Awschalom
Nondiffusive Spin Dynamics In A Two-Dimensional Electron Gas, Christopher P. Weber, J. Orenstein, B. Andrei Bernevig, Shou-Cheng Zhang, Jason Stephens, D. D. Awschalom
Physics
We describe measurements of spin dynamics in the two-dimensional electron gas in GaAs=GaAlAs quantum wells. Optical techniques, including transient spin-grating spectroscopy, are used to probe the relaxation rates of spin polarization waves in the wave vector range from zero to 6 x 104 cm-1. We find that the spin polarization lifetime is maximal at a nonzero wave vector, in contrast with expectations based on ordinary spin diffusion, but in quantitative agreement with recent theories that treat diffusion in the presence of spin-orbit coupling
Low-Frequency Crossover Of The Fractional Power-Law Conductivity In Srruo3, J. S. Dodge, Christopher P. Weber, J. Corson, J. Orenstein, Z. Schlesinger, J. W. Reiner, M. R. Beasley
Low-Frequency Crossover Of The Fractional Power-Law Conductivity In Srruo3, J. S. Dodge, Christopher P. Weber, J. Corson, J. Orenstein, Z. Schlesinger, J. W. Reiner, M. R. Beasley
Physics
We combine the results of terahertz time-domain spectroscopy with far-infrared transmission and reflectivity to obtain the conductivity of SrRuO 3 over an unprecedented continuous range in frequency, allowing us to characterize the approach to zero frequency as a function of temperature. We show that the conductivity follows a simple phenomenological form, with an analytic structure fundamentally different from that predicted by the standard theory of metals.
Charge Dynamics In The Half-Metallic Ferromagnet Cro2, E. J. Singley, Christopher P. Weber, D. N. Basov, A. Barry, J. M. D. Coey
Charge Dynamics In The Half-Metallic Ferromagnet Cro2, E. J. Singley, Christopher P. Weber, D. N. Basov, A. Barry, J. M. D. Coey
Physics
Infrared spectroscopy is used to investigate the electronic structure and charge carrier relaxation in crystalline films of CrO2 which is the simplest of all half-metallic ferromagnets. Chromium dioxide is a bad metal at room temperature but it has a remarkably low residual resistivity (<5 >μΩ cm) despite the small spectral weight associated with free carrier absorption. The infrared measurements show that low residual resistivity is due to the collapse of the scattering rate at ω<2000 >cm-1. The blocking of the relaxation channels at low v and T can be attributed to the unique electronic structure of a …
Saturation In “Nonmagnetic” Stainless Steel, Christopher P. Weber, J. Fajans
Saturation In “Nonmagnetic” Stainless Steel, Christopher P. Weber, J. Fajans
Physics
Scientific equipment often uses “nonmagnetic” stainless steel, relying on the steel’s nonmagnetic behavior to leave external magnetic fields unaltered. However, stainless steel’s permeability can rise significantly when it is welded or machined, possibly perturbing an external field. Such perturbations will diminish well above the stainless steel’s saturation point. The authors measured the permeability of both welded and machined 304 stainless steel as a function of an external magnetic field, and found that both saturate at fields of approximately 0.25 T.