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Simulated Associating Polymer Networks, Joris Billen
Simulated Associating Polymer Networks, Joris Billen
CGU Theses & Dissertations
Telechelic associating polymer networks consist of polymer chains terminated by endgroups that have a different chemical composition than the polymer backbone. When dissolved in a solution, the endgroups cluster together to form aggregates. At low temperature, a strongly connected reversible network is formed and the system behaves like a gel. Telechelic networks are of interest since they are representative for biopolymer networks (e.g. F-actin) and are widely used in medical applications (e.g. hydrogels for tissue engineering, wound dressings) and consumer products (e.g. contact lenses, paint thickeners).
In this thesis such systems are studied by means of a molecular dynamics/Monte Carlo …