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Missouri University of Science and Technology

Atmospheric Aerosols

Articles 1 - 4 of 4

Full-Text Articles in Chemistry

In Situ Measurement Of The Aerosol Size Distribution In Stratospheric Solid Rocket Motor Exhaust Plumes, Martin N. Ross, Philip D. Whitefield, Donald E. Hagen, Alfred R. Hopkins Apr 1999

In Situ Measurement Of The Aerosol Size Distribution In Stratospheric Solid Rocket Motor Exhaust Plumes, Martin N. Ross, Philip D. Whitefield, Donald E. Hagen, Alfred R. Hopkins

Chemistry Faculty Research & Creative Works

The concentration and size distribution of aerosol in the stratospheric exhaust plumes of two Space Shuttle rockets and one Titan IV rocket were measured using a two component aerosol sampling system carried aboard a WB‐57F aircraft. Aerosol size distribution in the 0.01 µm to 4 µm diameter size range was measured using a two component sampling system. The measured distributions display a trimodal form with modes near 0.005 µm, 0.09 µm, and 2.03 µm and are used to infer the relative mass fractionation among the three modes. While the smallest mode has been estimated to contain as much as 10% …


Particle Concentration Characterization For Jet Engine Emissions Under Cruise Conditions, Jonathan D. Paladino, Philip D. Whitefield, Donald E. Hagen, Alfred R. Hopkins, Max B. Trueblood May 1998

Particle Concentration Characterization For Jet Engine Emissions Under Cruise Conditions, Jonathan D. Paladino, Philip D. Whitefield, Donald E. Hagen, Alfred R. Hopkins, Max B. Trueblood

Chemistry Faculty Research & Creative Works

Airborne particle measurements during NASA project SUCCESS have shown that particle concentration profiles serve as good indicators of aircraft exhaust plume encounters. During exhaust plume penetrations there is a strong anticorrelation between the ratio of nonvolatile/total particulates and Nitrogen Oxide (NO) concentrations. an increase in fuel sulfur content was found to increase the total particle emission index, while the nonvolatile emission index remained unchanged. the EI's increased by a factor of 2.6 as the fuel sulfur increased from 70 - 700 ppm. the large particle size distribution (200-400 nm) was seen as a good long term indicator of an aircraft …


Particulate Sizing And Emission Indices For A Jet Engine Exhaust Sampled At Cruise, Donald E. Hagen, Philip D. Whitefield, Jonathan D. Paladino, Max B. Trueblood May 1998

Particulate Sizing And Emission Indices For A Jet Engine Exhaust Sampled At Cruise, Donald E. Hagen, Philip D. Whitefield, Jonathan D. Paladino, Max B. Trueblood

Physics Faculty Research & Creative Works

Particle size and emission indices measurements for jet engines, primarily the Rolls Royce RB211 engines on a NASA 757 aircraft are reported. These data were used to estimate the fraction of fuel sulfur that was converted to particulates. These measurements were made in-situ with the sampling aircraft several kilometers behind the source. Some complimentary ground measurements on the same source aircraft and engines are also reported. Significant differences are seen between the ground observations and the in-situ observations, indicating that plume processes are changing the aerosol's characteristics.


Observation Of Upper Tropospheric Sulfur Dioxide- And Acetone-Pollution: Potential Implications For Hydroxyl Radical And Aerosol Formation, F. Arnold, J. Schneider, K. Gollinger, H. Schlager, P. Schulte, Donald E. Hagen, Philip D. Whitefield, Peter F. J. Van Velthoven Jan 1997

Observation Of Upper Tropospheric Sulfur Dioxide- And Acetone-Pollution: Potential Implications For Hydroxyl Radical And Aerosol Formation, F. Arnold, J. Schneider, K. Gollinger, H. Schlager, P. Schulte, Donald E. Hagen, Philip D. Whitefield, Peter F. J. Van Velthoven

Physics Faculty Research & Creative Works

Aircraft-based measurements of sulfur dioxide, acetone, carbon dioxide, and condensation nuclei (CN) were made over the north-eastern Atlantic at upper tropospheric altitudes, around 9000 m. On October 14, 1993, strong SO 2- and acetone-pollution (both up to 3 ppbv) were observed, which were accompanied by a CO 2-enhancement of up to 6 ppmv, and large CN-concentrations of up to about 1500 cm -3 (for radii ≥ 6 nm). CN, excess CO 2, and to a lesser degree also acetone, were positively correlated with SO 2. Air mass trajectory analyses indicate, that most of the air masses …