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Articles 61 - 71 of 71
Full-Text Articles in Physical Sciences and Mathematics
Radiative Electron Capture Into High- Z Few-Electron Ions: Alignment Of The Excited Ionic States, Andrey S. Surzhykov, Ulrich D. Jentschura, Th H. Stohlker, Stephan Fritzsche
Radiative Electron Capture Into High- Z Few-Electron Ions: Alignment Of The Excited Ionic States, Andrey S. Surzhykov, Ulrich D. Jentschura, Th H. Stohlker, Stephan Fritzsche
Physics Faculty Research & Creative Works
We lay out a unified formalism for the description of radiative electron capture into excited states of heavy, few-electron ions and their subsequent decay, including a full account of many-electron effects and higher-order multipoles of the radiation field. In particular, the density-matrix theory is applied to explore the magnetic sublevel population of the residual ions, as described in terms of alignment parameters. For the electron capture into the initially hydrogenlike U91+ and lithiumlike U89+ uranium projectiles, the alignment parameters are calculated, within the multiconfiguration Dirac-Fock approach, as a function of the collision energy and for different ionic states. …
Mutual Ionization In 200-Kev H⁻+ He Collisions, T. Ferger, Daniel Fischer, Michael Schulz, R. Moshammer, A. B. Voitkiv, B. Najjari, J. Ullrich
Mutual Ionization In 200-Kev H⁻+ He Collisions, T. Ferger, Daniel Fischer, Michael Schulz, R. Moshammer, A. B. Voitkiv, B. Najjari, J. Ullrich
Physics Faculty Research & Creative Works
We studied mutual ionization in 200-keV H-+He collisions in a kinematically complete experiment by measuring the fully momentum-analyzed recoil ions and both active electrons in coincidence. Comparison of the data to our calculations, based on various theoretical models, show that mutual ionization proceeds predominantly through the interaction between both electrons. The post-collision interaction between the outgoing ejected electrons as well as higher order processes involving the interaction between the core of both collision partners are also important.
Comparison Of Hyperspherical Versus Common-Reaction-Coordinate Close-Coupling Methods For Ion-Atom Collisions At Low Energies, Anh-Thu Le, C. D. Lin, L. F. Errea, L. Mendez, A. Riera, B. Pons
Comparison Of Hyperspherical Versus Common-Reaction-Coordinate Close-Coupling Methods For Ion-Atom Collisions At Low Energies, Anh-Thu Le, C. D. Lin, L. F. Errea, L. Mendez, A. Riera, B. Pons
Physics Faculty Research & Creative Works
We present detailed comparisons between the two quantal approaches--hyperspherical close-coupling and common-reaction-coordinate close-coupling methods--on an exemplary case of He²⁺ + H(1s) collisions at center-of-mass energy from 20eV up to 1.6keV. It is shown that the partial-wave charge-transfer cross sections from the two approaches agree very well at low energy below 200eV down to 30eV. This good agreement is a strong indication of the validity of both methods. The small difference at very low energies and the convergence with respect to the number of channels in both approaches at higher energies are also discussed.
Probing Scattering Wave Functions Close To The Nucleus, Don H. Madison, Daniel Fischer, Matthew S. Foster, Michael Schulz, Robert Moshammer, Stephenie J. Jones, Joachim Hermann Ullrich
Probing Scattering Wave Functions Close To The Nucleus, Don H. Madison, Daniel Fischer, Matthew S. Foster, Michael Schulz, Robert Moshammer, Stephenie J. Jones, Joachim Hermann Ullrich
Physics Faculty Research & Creative Works
Recently, three-dimensional imaging of the ejected electrons following 100 MeV/amu C6+ single ionization of helium led to the observation of a new structure not predicted by theory [M. Schulz et al., Nature (London) 422, 48 (2003)]. Instead of the usual “recoil lobe” centered on the momentum-transfer axis, a ring-shaped structure centered on the beam axis was observed. New measurements at 2 MeV/amu exhibit a similar structure, which is now predicted by theory. We argue that the same theory failed at 100 MeV/amu because the faster projectiles probe distances much closer to the nucleus, where our multiple-scattering model is expected …
Role Of The Ground State In Electron-Atom Double Ionization, Stephenie J. Jones, Don H. Madison
Role Of The Ground State In Electron-Atom Double Ionization, Stephenie J. Jones, Don H. Madison
Physics Faculty Research & Creative Works
Recently, absolute measurements have been reported for double ionization of helium by 5.6 keV electron-impact. At this high energy, one would think that the first Born approximation for the interaction of the projectile with the atom would be valid. However, on the basis of a lowest-order implementation of a Faddeev-type approach, Berakdar concluded that the approximation was not valid. Here we argue that (i) it is valid at this energy and (ii) the previous discrepancy between calculations in the first Born approximation and the overall magnitude of the measurements was due to a poor description of the ground state.
Disorder-Induced Rounding Of Certain Quantum Phase Transitions, Thomas Vojta
Disorder-Induced Rounding Of Certain Quantum Phase Transitions, Thomas Vojta
Physics Faculty Research & Creative Works
We study the influence of quenched disorder on quantum phase transitions in systems with overdamped dynamics. For Ising order-parameter symmetry disorder destroys the sharp phase transition by rounding because a static order parameter can develop on rare spatial regions. This leads to an exponential dependence of the order parameter on the coupling constant. At finite temperatures the static order on the rare regions is destroyed. This restores the phase transition and leads to a double exponential relation between critical temperature and coupling strength. We discuss the behavior based on Lifshitz-tail arguments and illustrate the results by simulations of a model …
Perturbative And Nonperturbative Calculations Of Electron-Hydrogen Ionization, Stephenie J. Jones, Don H. Madison, Mark D. Baertschy
Perturbative And Nonperturbative Calculations Of Electron-Hydrogen Ionization, Stephenie J. Jones, Don H. Madison, Mark D. Baertschy
Physics Faculty Research & Creative Works
We compare calculations of the fully differential cross section for ionization of atomic hydrogen by electron impact using two different theories-the perturbative CDW-EIS (continuum distorted wave with eikonal initial state) approximation and the nonperturbative ECS (exterior complex scaling) method. For this comparison, we chose an impact energy of 54.4 eV, since this is near the lowest energy that our perturbative approach would be applicable and near the highest energy that can be tackled by the ECS method with our present computational resources. For the case of equal-energy outgoing electrons investigated here, the two theories predict nearly identical results except that …
Slow Convergence Of The Born Approximation For Electron-Atom Ionization, Stephenie J. Jones, Don H. Madison
Slow Convergence Of The Born Approximation For Electron-Atom Ionization, Stephenie J. Jones, Don H. Madison
Physics Faculty Research & Creative Works
It is usually assumed that the first-Born approximation for electron-atom ionization becomes valid for the fully differential cross section at sufficiently high impact energies, at least for asymmetric collisions where the projectile suffers only a small energy loss and is scattered by a small angle. Here we investigate this assumption quantitatively for ionization of hydrogen atoms. We find that convergence of the Born approximation to the correct nonrelativistic result is generally achieved only at energies where relativistic effects start to become important. Consequently, the assumption that the Born approximation becomes valid for high energy is inaccurate, since by the time …
Doubly Differential Electron-Emission Spectra In Single And Multiple Ionization Of Noble-Gas Atoms By Fast Highly-Charged-Ion Impact, Tom Kirchner, Laszlo Gulyas, Robert Moshammer, Michael Schulz, Joachim Hermann Ullrich
Doubly Differential Electron-Emission Spectra In Single And Multiple Ionization Of Noble-Gas Atoms By Fast Highly-Charged-Ion Impact, Tom Kirchner, Laszlo Gulyas, Robert Moshammer, Michael Schulz, Joachim Hermann Ullrich
Physics Faculty Research & Creative Works
Low-energy electron emission spectra are studied in collisions of 3.6 MeV/amu Au53+ ions with neon and argon atoms for well-defined degrees of target ionization. We calculate doubly differential cross sections as functions of the recoil-ion charge state in the continuum-distorted-wave with eikonal initial-state approximation using a binomial analysis of the total and differential ionization probabilities, and compare them with the present and with previously published experimental data. Very good agreement is found for the single-ionization spectra and for double ionization of neon, while some discrepancies are observed in the spectra for double and triple ionization of argon.
Electric Field Controlled, Pulsed Autoionization In Two Electron Wave Packets, J. Greg Story, Heider N. Ereifej
Electric Field Controlled, Pulsed Autoionization In Two Electron Wave Packets, J. Greg Story, Heider N. Ereifej
Physics Faculty Research & Creative Works
In this paper, control of the evolution of a two electron wave packet through the application of a static electric field is demonstrated. Specifically, application of a small electric field is used to produce pulsed autoionization events, the timing of which can be controlled on a picosecond time scale. The technique is demonstrated by exciting calcium atoms using a short-pulsed laser to the 4p3/219d doubly excited state, which is energy degenerate with the 4p1/2nk stark states. Evolution of the resultant wave packet is monitored through the application of a second short laser pulse, which stimulates the …
Auger Resonance Decay Process In Ar 2p Shell Excitation And Ionization, Y. Lu, Wayne C. Stolte, J.A. R. Samson
Auger Resonance Decay Process In Ar 2p Shell Excitation And Ionization, Y. Lu, Wayne C. Stolte, J.A. R. Samson
Chemistry and Biochemistry Faculty Research
The production and subsequent autoionization of the Ar+ (1D2)6d1 satellite state that is formed either by shake-up or recapture during the Auger decay of a 2p vacancy in Ar has been studied by photoelectron spectroscopy in the energy region from 243 to 256 eV. The creation of near zero energy electrons below and immediately above the Ar 2p ionization threshold is discussed. Some ambiguous points in previous studies are clarified.