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Full-Text Articles in Physical Sciences and Mathematics
Triply Differential Single Ionization Of Argon: Charge Effects For Positron And Electron Impact, Sebastian Otranto, Ronald E. Olson, O. G. De Lucio, Robert D. Dubois
Triply Differential Single Ionization Of Argon: Charge Effects For Positron And Electron Impact, Sebastian Otranto, Ronald E. Olson, O. G. De Lucio, Robert D. Dubois
Physics Faculty Research & Creative Works
Triply differential single ionization of Ar by 200 eV positron and electron impact is measured and calculated. For an unequivocal test of kinematic differences, fully differential ejected electron angular distributions are measured using the same experimental apparatus and conditions for both positron and electron impact. The binary/recoil intensity ratios are shown to significantly differ for the two projectiles. These data are used to test theoretical calculations.
Theoretical Study Of Photoelectron Angular Distributions In Single-Photon Ionization Of Aligned N₂ And Co₂, Cheng Jin, Anh-Thu Le, Song-Feng Zhao, R. R. Lucchese, C. D. Lin
Theoretical Study Of Photoelectron Angular Distributions In Single-Photon Ionization Of Aligned N₂ And Co₂, Cheng Jin, Anh-Thu Le, Song-Feng Zhao, R. R. Lucchese, C. D. Lin
Physics Faculty Research & Creative Works
We calculate photoelectron angular distributions (PADs) resulting from single-photon (43 eV) ionization of molecules that have been transiently aligned with a short laser pulse. The total ionization cross sections of N₂ and CO₂ vs the time delay between the aligning laser pulse and the soft x-ray photon are calculated and compared to experimental results reported by I. Thomann et al. [J. Phys. Chem. A 112, 9382 (2008)]. We present the PADs from these aligned molecules in the laboratory frame which can be compared directly with future experiments from aligned N₂ and CO₂. The alignment dependence of single-photon ionization, multiphoton ionization, …
Determination Of Structure Parameters In Strong-Field Tunneling Ionization Theory Of Molecules, Song-Feng Zhao, Cheng Jin, Anh-Thu Le, T. F. Jiang, C. D. Lin
Determination Of Structure Parameters In Strong-Field Tunneling Ionization Theory Of Molecules, Song-Feng Zhao, Cheng Jin, Anh-Thu Le, T. F. Jiang, C. D. Lin
Physics Faculty Research & Creative Works
In the strong field molecular tunneling ionization theory of Tong et al. [Phys. Rev. A 66, 033402 (2002)], the ionization rate depends on the asymptotic wave function of the molecular orbital from which the electron is removed. The orbital wave functions obtained from standard quantum chemistry packages in general are not good enough in the asymptotic region. Here we construct a one-electron model potential for several linear molecules using density functional theory. We show that the asymptotic wave function can be improved with an iteration method and after one iteration accurate asymptotic wave functions and structure parameters are determined. With …