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Articles 61 - 67 of 67
Full-Text Articles in Physical Sciences and Mathematics
Computational Studies Of The Properties Of Copper Oxide Clusters And The Reactions Of Phenol And Chlorinated Phenols With Copper Oxide Clusters, Gyun-Tack Bae
LSU Doctoral Dissertations
We used ab initio simulations and calculations to study the structures and stabilities of copper oxide clusters, CunOn (n=1-8) and CuOn (n=1-6). The lowest energy structures of neutral and charged copper oxide clusters were determined using primarily the B3LYP/LANL2DZ model chemistry. In CunOn clusters with n=1-8, a transition from planar to nonplanar geometries occurs at n=4. In CuOn clusters with n=1-6, all geometries of neutral, positively, and negatively charged clusters are planar or near planar structures. Selected electronic properties, including binding energies, ionization energies, and electronic affinities, were calculated and examined as a function of n. Stabilities were examined by …
Scanning Probe Microscopy Investigations Of (1) Arrays Of Cysteine-Coated Cds Nanoparticles And (2) Structures Formed During The Early Stages Of The Corrosion Of Copper Surfaces, Brian Robert Lewandowski
Scanning Probe Microscopy Investigations Of (1) Arrays Of Cysteine-Coated Cds Nanoparticles And (2) Structures Formed During The Early Stages Of The Corrosion Of Copper Surfaces, Brian Robert Lewandowski
LSU Doctoral Dissertations
Scanning probe microscopy (SPM) characterizations are becoming more prevalent for surface investigations due to their capabilities for obtaining structural information and physical measurements. New capabilities of SPM for studying and controlling nanoscale processes are emerging as valuable assets in research. A fundamental understanding of the interactions of surface reactions provides essential information for developing workable applications for nanotechnology. Two applications of SPM are discussed in this dissertation. The first investigation uses atomic force microscopy (AFM) for the characterization of nanostructures produced with a newly developed lithographic technique called “two-particle” lithography. This new technique is based on particle lithography for the …
Merged Electrospray Ionization Mass Spectrometry, Jianan Dong
Merged Electrospray Ionization Mass Spectrometry, Jianan Dong
LSU Doctoral Dissertations
Ambient ionization allows the analysis of materials in their native environment without sample preparation by creating ions outside the mass spectrometer. The goal of this research was to develop new ambient ionization techniques for application to solids, liquids and particles under ambient conditions. Samples to be analyzed were directly merged with an electrospray of droplets, and then ionized and detected by a mass spectrometer. An ion trap mass spectrometer was modified with a nanoelectrospray source and configured for three experiments: merged electrospray ionization of dry particles, merged electrospray ionization of combustion products, and infrared laser desorption/ablation using electrospray for post-ionization. …
Task Specific Ionic Liquids For Enantiomeric Recognition And Nanomaterials For Biomedical Imaging, David Kipkogei Bwambok
Task Specific Ionic Liquids For Enantiomeric Recognition And Nanomaterials For Biomedical Imaging, David Kipkogei Bwambok
LSU Doctoral Dissertations
Ionic liquids (ILs) are organic salts that melt at or below 100°C. Interest in ILs continues to grow due to their unique properties such as lack of measurable vapor pressure, high thermal stability, tunability and recyclability. The first part of this dissertation explores the use of chiral ionic liquids (CILs) for enantiomeric recognition of chiral analytes using fluorescence spectroscopy. Chiral analyses continue to be a subject of considerable interest primarily as a result of legislation introduced by the Food and Drug Administration. This has led to an increased need for suitable chiral selectors and methods to verify the enantiomeric forms …
Creep Behavior Of Natural Fiber Reinforced Polymer Composites, Yanjun Xu
Creep Behavior Of Natural Fiber Reinforced Polymer Composites, Yanjun Xu
LSU Doctoral Dissertations
Creep behavior of natural fiber/polymer composites (NFPCs) was studied in response to the increasing application of this material as structural building products. Factors that influence creep behavior of the composites were investigated by analyzing creep curves of several different NFPC systems, which were designed for overall performance of the composites. Among different models, the 4-element Burgers type was mostly used for quantitative characterization of the creep curves to compare the properties of different composites. The parameters from the 4-element Burgers model were easily interpretable due to their physical meanings. Generalized Burgers models provided better fit by introducing extra Kelvin units, …
Stochastic Navier-Stokes Equations With Fractional Brownian Motions, Liqun Fang
Stochastic Navier-Stokes Equations With Fractional Brownian Motions, Liqun Fang
LSU Doctoral Dissertations
The aim of this dissertation is to study stochastic Navier-Stokes equations with a fractional Brownian motion noise. The second chapter will introduce the background results on fractional Brownian motions and some of their properties. The third chapter will focus on the Stokes operator and the semigroup generated by this operator. The Navier-Stokes equations and the evolution equation setup will be described in the next chapter. The main goal is to prove the existence and uniqueness of solutions for the stochastic Navier-Stokes equations with a fractional Brownian motion noise under suitable conditions. The proof is given with full details for two …
A Regularization Technique In Dynamic Optimization, Alvaro Guevara
A Regularization Technique In Dynamic Optimization, Alvaro Guevara
LSU Doctoral Dissertations
In this dissertation we discuss certain aspects of a parametric regularization technique which is based on recent work by R. Goebel. For proper, lower semicontinuous, and convex functions, this regularization is self-dual with respect to convex conjugation, and a simple extension of this smoothing exhibits the same feature when applied to proper, closed, and saddle functions. In Chapter 1 we give a introduction to convex and saddle function theory, which includes new results on the convergence of saddle function values that were not previously available in the form presented. In Chapter 2, we define the regularization and extend some of …