Nuclear Engineering Commons^™

Optimization Of Transcurium Isotope Production In The High Flux Isotope Reactor, Susan Hogle

Doctoral Dissertations

The Radiochemical Engineering Development Center at Oak Ridge National Laboratory is the world's leader in production of californium-252. This and other heavy actinides are produced by irradiation of mixed curium/americium targets in the High Flux Isotope Reactor. Due to the strong dependence of isotopic cross sections upon incoming neutron energy, the efficiency with which an isotope is transmuted is highly dependent upon the neutron flux energy spectrum and intensities. There are certain energy ranges in which the rate of fissions in feedstock materials can be minimized relative to the rate of (n,γ) absorptions. This work shows that by perturbing the …