Nuclear Engineering Commons^™

Modeling The Uranium-Silicon Phase Equilibria Based On Computational And Experimental Analysis, Tashiema Lixona Ulrich

Theses and Dissertations

As part of Accident tolerant fuel initiative, the uranium-silicide compound, U3Si2, is under consideration as a potential replacement for conventional uranium dioxide fuel. It is of interest as its higher uranium density of 11.3 g(U)/cm3 compared to 9.7 g(U)/cm3 for UO2 may allow use of more robust, but less neutronically economical fuel cladding. The improved uranium content would not only accommodate the neutronic penalty inherent to certain accident tolerant cladding concepts but also facilitate improved reactor performance with the potential for longer fuel cycles.

The U-Si system has been the subject of various studies that mainly focused on thermophysical properties, …