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Full-Text Articles in Nuclear Engineering

Double-Pulse Nd:Yag-Co2 Libs Excitation For Bulk And Trace Analytes, Jason R. Becker, Patrick Skrodzki, Prasoon Diwakar, Sivanandan Harilal, Ahmed Hassanein Aug 2014

Double-Pulse Nd:Yag-Co2 Libs Excitation For Bulk And Trace Analytes, Jason R. Becker, Patrick Skrodzki, Prasoon Diwakar, Sivanandan Harilal, Ahmed Hassanein

The Summer Undergraduate Research Fellowship (SURF) Symposium

Laser-induced breakdown spectroscopy [LIBS] is a commonly used technique for multi-element analyses for various applications such as space exploration, nuclear forensics, environmental analysis, process monitoring. The advantages of the LIBS technique include robustness, ease of use, field portability, and real-time, non-invasive multi-element analyses. However, in comparison to other lab based analytical techniques, it suffers from low precision and low sensitivity. In order to overcome these drawbacks, various approaches have been used, including double-pulse LIBS [DPLIBS]. Typically, various wavelength combinations of two Nd: yttrium aluminum garnet [YAG] lasers have been used for DPLIBS. However, the use of long wavelength (CO2 …


Doube-Pulse Laser-Induced Breakdown Spectroscopy Of Multi-Element Sample Containing Low- And High-Z Analytes, Patrick J. Skrodzki, Jason R. Becker, Prasoon K. Diwakar Ph. D., Sivanandan S. Harilal Ph. D., Ahmed Hassanein Ph. D. Aug 2014

Doube-Pulse Laser-Induced Breakdown Spectroscopy Of Multi-Element Sample Containing Low- And High-Z Analytes, Patrick J. Skrodzki, Jason R. Becker, Prasoon K. Diwakar Ph. D., Sivanandan S. Harilal Ph. D., Ahmed Hassanein Ph. D.

The Summer Undergraduate Research Fellowship (SURF) Symposium

Laser-induced breakdown spectroscopy (LIBS) is a portable, remote, non-invasive analytical technique which effectively distinguishes neutral and ionic species for a range of low- to high-Z elements in a multi-element target. Subsequently, LIBS holds potential in special nuclear material (SNM) sensing and nuclear forensics requiring minimal sample preparation and detecting isotopic shifts which allows for differentiation in SNM (namely U) enrichment levels. Feasible applications include not only nonproliferation and homeland security but also nuclear fuel prospecting and industrial safeguard endorsement. Elements of higher mass with complex atomic structures, such as U, however, result in crowded emission spectra with LIBS, and characteristic …