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Full-Text Articles in Nuclear Engineering
Thermodynamic Characterization And Isothermal Separability Of Heavy Fission Product Chelates For Post-Detonation Nuclear Forensic Analysis, Steven Adam Stratz
Thermodynamic Characterization And Isothermal Separability Of Heavy Fission Product Chelates For Post-Detonation Nuclear Forensic Analysis, Steven Adam Stratz
Doctoral Dissertations
Nuclear terrorism, one of the most critical threats to national security, exhibits complexities that do not exist with similar threats from sanctioned state actors. Responding to a domestic nuclear terrorism strike is difficult when the original source of the weapon may be unknown, given that terrorist organizations (at the time of writing) do not themselves have nuclear technology sufficient to design and build nuclear weapons. Consequently, the development of forensic techniques to help source and characterize nuclear weapons after detonation has recently become an area of interest. This relatively new field of science, known as post-detonation nuclear forensics, aims to …
Improved Sample Utilization In Thermal Ionization Mass Spectrometry Isotope Ratio Measurements: Refined Development Of Porous Ion Emitters For Nuclear Forensic Applications, Matthew Louis Baruzzini
Improved Sample Utilization In Thermal Ionization Mass Spectrometry Isotope Ratio Measurements: Refined Development Of Porous Ion Emitters For Nuclear Forensic Applications, Matthew Louis Baruzzini
Doctoral Dissertations
The precise and accurate determination of isotopic composition in nuclear forensic samples is vital for assessing origin, intended use and process history. Thermal ionization mass spectrometry (TIMS) is widely accepted as the gold standard for high performance isotopic measurements and has long served as the workhorse in the isotopic ratio determination of nuclear materials. Nuclear forensic and safeguard specialists have relied heavily on such methods for both routine and atypical efforts. Despite widespread use, TIMS methods for the assay of actinide systems continue to be hindered by poor ionization efficiency, often less than tenths of a percent; the majority of …