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Full-Text Articles in Nanoscience and Nanotechnology

Chalcogenide Nanocrystal Assembly: Controlling Heterogeneity And Modulating Heterointerfaces, Jessica Davis Davis Jan 2017

Chalcogenide Nanocrystal Assembly: Controlling Heterogeneity And Modulating Heterointerfaces, Jessica Davis Davis

Wayne State University Dissertations

This dissertation work is focused on developing methods to facilitate charge transport in heterostructured materials that comprise a nanoscale component. Multicomponent semiconductor materials were prepared by (1) spin coating of discrete nanomaterials onto porous silicon (pSi) or (2) self-assembly. Spin-coating of colloidal quantum dot (QD) PbS solutions was employed to create prototype PbS QD based radiation detection devices using porous silicon (pSi) as an n-type support and charge transport material. These devices were initially tested as a photodetector to ascertain the possibility of their use in high energy radiation detection. Short chain thiolate ligands (4-fluorothiophenolate) and anion passivation at the …


Dynamic Rabi Oscillations In A Quantum Dot Embedded In A Nanobridge In The Presence Of Surface Acoustic Waves, Lev Mourokh, Achim Wixforth, Florian Beil, Max Bichler, Werner Wegscheider, Robert H. Blick Jan 2017

Dynamic Rabi Oscillations In A Quantum Dot Embedded In A Nanobridge In The Presence Of Surface Acoustic Waves, Lev Mourokh, Achim Wixforth, Florian Beil, Max Bichler, Werner Wegscheider, Robert H. Blick

Publications and Research

A quantum dot is created within a suspended nanobridge containing a two-dimensional electron gas. The electron current through this dot exhibits well-pronounced Coulomb blockade oscillations. When surface acoustic waves (SAW) are driven through the nanobridge, Coulomb blockade peaks are shifted. To explain this feature, we derive the expressions for the quantum dot level populations and electron currents through these levels and show that SAW-induced Rabi oscillations lead to the observed phenomenology.