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Multidimensional Spectroscopy Of Semiconductor Quantum Dots, Jason Michael Bylsma
Multidimensional Spectroscopy Of Semiconductor Quantum Dots, Jason Michael Bylsma
USF Tampa Graduate Theses and Dissertations
The coherent properties of semiconductor nanostructures are inherently difficult to measure and one-dimensional spectroscopies are often unable to separate inhomogeneous and homogeneous linewidths. We have refined and improved a method of performing multidimensional Fourier transform spectroscopy based on four-wave
mixing (FWM) experiments in the box geometry. We have modified our system with broadband beamsplitters in all interferometer arms, high-resolution translation stages and the ability to work in reflection geometry. By improving the phase-stability of our setup and scanning pulse delays with sub-optical cycle precision, we are able to
reproduce 2DFT spectra of GaAs multiple quantum wells. With the FWM signal …