Mechanical Engineering Commons^™

Composite Gel Polymer Electrolytes For Extended Cyclability Of Lithium-Oxygen Batteries, Marcus Carlton Herndon

FIU Electronic Theses and Dissertations

In lithium-oxygen (Li-O₂) batteries, addressing challenges like electrode degradation, cell stability and electrolyte decomposition are key to creating more practical applications. Despite many attempts to minimize anode oxidation and cathode byproduct formation, the electrolyte remains the leading source for rapid capacity fading and poor cyclability in Li-O₂batteries. Understanding the loss of functionality in electrolytes, carbon nanotube (CNT) fillers and redox mediators (RM), during cycling within Li-O₂battery systems, could be the solution to prolonging battery lifetime. Determining the efficiency of these battery components and additives will push the medium towards lifelong, rechargeable and safe battery …