Computer Engineering Commons^™

Leveraging Nanocavity Harmonics For Control Of Optical Processes In 2d Semiconductors, Gleb M. Akselrod, Tian Ming, Christos Argyropoulos, Thang B. Hoang, Yuxuan Lin, Xi Ling, David R. Smith, Jing Kong, Maiken H. Mikkelsen

Department of Electrical and Computer Engineering: Faculty Publications

Optical cavities with multiple tunable resonances have the potential to provide unique electromagnetic environments at two or more distinct wavelengthscritical for control of optical processes such as nonlinear generation, entangled photon generation, or photoluminescence (PL) enhancement. Here, we show a plasmonic nanocavity based on a nanopatch antenna design that has two tunable resonant modes in the visible spectrum separated by 350 nm and with line widths of ∼60 nm. The importance of utilizing two resonances simultaneously is demonstrated by integrating monolayer MoS2, a two-dimensional semiconductor, into the colloidally synthesized nanocavities. We observe a 2000-fold enhancement in the PL intensity of …