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Department of Electrical and Computer Engineering: Faculty Publications

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Plasmonics

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Nonlinear Strong Coupling By Second-Harmonic Generation Enhancement In Plasmonic Nanopatch Antennas, Bryson Krause, Dhananjay Mishra, Jiyang Chen, Christos Argyropoulos, Thang Hoang Aug 2022

Nonlinear Strong Coupling By Second-Harmonic Generation Enhancement In Plasmonic Nanopatch Antennas, Bryson Krause, Dhananjay Mishra, Jiyang Chen, Christos Argyropoulos, Thang Hoang

Department of Electrical and Computer Engineering: Faculty Publications

Enhanced electromagnetic fields within plasmonic nanocavity mode volumes enable multiple significant effects that lead to applications in both the linear and nonlinear optical regimes. In this work, we demonstrate enhanced second harmonic generation from individual plasmonic nanopatch antennas which are formed by separating silver nanocubes from a smooth gold film using a sub-10 nm zinc oxide spacer layer. When the nanopatch antennas are excited at their fundamental plasmon frequency, a 104-fold increase in the intensity of the second harmonic generation wave is observed. Moreover, by integrating quantum emitters that have an absorption energy at the fundamental frequency, a …


Plasmonic Waveguides To Enhance Quantum Electrodynamic Phenomena At The Nanoscale, Ying Li, Christos Argyropoulos Feb 2021

Plasmonic Waveguides To Enhance Quantum Electrodynamic Phenomena At The Nanoscale, Ying Li, Christos Argyropoulos

Department of Electrical and Computer Engineering: Faculty Publications

The emerging field of plasmonics can lead to enhanced light-matter interactions at extremely nanoscale regions. Plasmonic (metallic) devices promise to efficiently control both classical and quantum properties of light. Plasmonic waveguides are usually used to excite confined electromagnetic modes at the nanoscale that can strongly interact with matter. The analysis of these nanowaveguides exhibits similarities with their low frequency microwave counterparts. In this article, we review ways to study plasmonic nanostructures coupled to quantum optical emitters from a classical electromagnetic perspective. These quantum emitters are mainly used to generate single-photon quantum light that can be employed as a quantum bit …


Tunable Subnanometer Gap Plasmonic Metasurfaces, Dennis Doyle, Nicholas Charipar, Christos Argyropoulos, Scott A. Trammell, Rafaela Nita, Jawad Naciri, Alberto Piqué, Joseph B. Herzog, Jake Fontana Jan 2017

Tunable Subnanometer Gap Plasmonic Metasurfaces, Dennis Doyle, Nicholas Charipar, Christos Argyropoulos, Scott A. Trammell, Rafaela Nita, Jawad Naciri, Alberto Piqué, Joseph B. Herzog, Jake Fontana

Department of Electrical and Computer Engineering: Faculty Publications

The index of refraction governs the flow of light through materials. At visible and near-infrared wavelengths the real part of the refractive index is limited to less than 3 for naturally occurring transparent materials, fundamentally restricting applications. Here, we carried out experiments to study the upper limit of the effective refractive index of self-assembled metasurfaces at visible and near-infrared wavelengths. The centimeter-scale metasurfaces were made of a hexagonally close packed (HCP) monolayer of gold nanospheres coated with tunable alkanethiol ligand shells, controlling the interparticle gap from 2.8 to 0.45 nm. In contrast to isolated dimer studies, the macroscale areas allow …


Flatland Plasmonics And Nanophotonics Based On Graphene And Beyond, Pai-Yen Chen, Christos Argyropoulos, Mohamed Farhat, J. Sebastian Gomez-Diaz Jan 2017

Flatland Plasmonics And Nanophotonics Based On Graphene And Beyond, Pai-Yen Chen, Christos Argyropoulos, Mohamed Farhat, J. Sebastian Gomez-Diaz

Department of Electrical and Computer Engineering: Faculty Publications

In this paper, we review and discuss how the recently discovered two-dimensional (2D) Dirac materials, particularly graphene, may be utilized as new efficient platforms for excitations of propagating and localized surface plasmon polaritons (SPPs) in the terahertz (THz) and mid-infrared (MIR) regions. The surface plasmon modes supported by the metallic 2D materials exhibit tunable plasmon resonances that are essential, yet missing, ingredients needed for THz and MIR photonic and optoelectronic devices. We describe how the atomically thin graphene monolayer and metamaterial structures based on it may tailor and control the spectral, spatial, and temporal properties of electromagnetic radiation. In the …


Leveraging Nanocavity Harmonics For Control Of Optical Processes In 2d Semiconductors, Gleb M. Akselrod, Tian Ming, Christos Argyropoulos, Thang B. Hoang, Yuxuan Lin, Xi Ling, David R. Smith, Jing Kong, Maiken H. Mikkelsen Jan 2015

Leveraging Nanocavity Harmonics For Control Of Optical Processes In 2d Semiconductors, Gleb M. Akselrod, Tian Ming, Christos Argyropoulos, Thang B. Hoang, Yuxuan Lin, Xi Ling, David R. Smith, Jing Kong, Maiken H. Mikkelsen

Department of Electrical and Computer Engineering: Faculty Publications

Optical cavities with multiple tunable resonances have the potential to provide unique electromagnetic environments at two or more distinct wavelengthscritical for control of optical processes such as nonlinear generation, entangled photon generation, or photoluminescence (PL) enhancement. Here, we show a plasmonic nanocavity based on a nanopatch antenna design that has two tunable resonant modes in the visible spectrum separated by 350 nm and with line widths of ∼60 nm. The importance of utilizing two resonances simultaneously is demonstrated by integrating monolayer MoS2, a two-dimensional semiconductor, into the colloidally synthesized nanocavities. We observe a 2000-fold enhancement in the PL intensity of …


Negative Refraction, Gain And Nonlinear Effects In Hyperbolic Metamaterials, Christos Argyropoulos, Nasim Mohammadi Estakhri, Francesco Monticone, Andrea Alu Jan 2013

Negative Refraction, Gain And Nonlinear Effects In Hyperbolic Metamaterials, Christos Argyropoulos, Nasim Mohammadi Estakhri, Francesco Monticone, Andrea Alu

Department of Electrical and Computer Engineering: Faculty Publications

The negative refraction and evanescent-wave canalization effects supported by a layered metamaterial structure obtained by alternating dielectric and plasmonic layers is theoretically analyzed. By using a transmission-line analysis, we formulate a way to rapidly analyze the negative refraction operation for given available materials over a broad range of frequencies and design parameters, and we apply it to broaden the bandwidth of negative refraction. Our analytical model is also applied to explore the possibility of employing active layers for loss compensation. Nonlinear dielectrics can also be considered within this approach, and they are explored in order to add tunability to the …