Engineering Commons^™

Characterization Of The Acquisition Parameters Of A Submersible Gamma-Ray Computed Tomography System, Zhongmin Jin

Doctoral Dissertations

"The purpose of this work is to study a component of a submersible gamma-ray computed tomography (CT) system used in the non-destructive testing of irradiated nuclear fuels. The first section of this study proposes two acceleration approaches for rapidly modeling a transmission-type gamma-ray tomography system. The first relies on Monte Carlo simulations with a monodirectionally biased source sampled from a sub-volume of the whole source volume. This method estimates the real count rate using analytical correction factors. The second way of acceleration is based on deterministic calculations that use the Beer-Lambert law and detector response characteristics. It shows that both …

Validation Of Athlet With Purdue University Multi-Dimensional Integral Test Assembly (Puma) Test, Emin Fatih Ozdem

Masters Theses

"Following the Three Mile Island Unit 2 (TMI-2) disaster, the development of a diagnostic system for emergency situations in a nuclear power plant was identified as an essential research area to strengthen the safety of nuclear power plants. A real-time estimation system of vital safety parameters on the main side of a PWR (Pressurized Water Reactor) facility was investigated since precise post-event scenario estimations are thought to be a crucial component of the diagnostic system. The alarm system of the plant can detect an SB-LOCA (Small Break Loss-Of-Coolant-Accident), but there were a couple of potential long-term transient occurrences. The accident …

Physical Properties Of Copper Niobium Nanolamellar Composites Fabricated By Accumulative Roll Bonding, Jared Justice

Nuclear Engineering ETDs

Nanolamellar composites with high interface density have increased strength due to interfaces serving as barriers to dislocation movement and high radiation damage resistance. However, these interfaces also serve as barriers to electron motion, reducing the electrical resistivity and thermal conductivity. This work seeks to understand the inherent tradeoff between strength and physical properties of nanolamellar composites produced by accumulative roll bonding with layer thickness ranging from 25 nm to 193 nm. The electrical resistivity was investigated over temperatures ranging from 2 K to 300 K. The effect of longitudinal rolling and cross rolling was also investigated. Electrical resistivity results were …

Dynamics Modeling Of Molten Salt Reactors, Visura Umesh Pathirana

Doctoral Dissertations

The abundance of energy is a necessity for the prosperity of humans. The rise in energy demand has created energy shortages and issues related to energy security. Nuclear energy can produce vast amounts of reliable energy without many of the negative externalities associated with other competing energy sources, such as coal and natural gas. As a result, public interest in nuclear power has increased in the past decade. Many new types of nuclear reactor are proposed. These nuclear reactor designs feature many passive technologies that can operate without external influence. Reactors that feature advanced passive safety features are catagorized as …

Development Of A Portable, Tileable, Dual-Particle Radiography System, Christian Xavier Young

Doctoral Dissertations

A scalable, portable, multi-particle neutron radiography device has been developed using commercial-off-the-shelf-parts. The IDEAS ROSSPAD readout module was selected for use in developing the radiography panel due to its single-wire Power-over-Ethernet (PoE) connectivity and its tileable form factor. Each ROSSPAD detector is paired with an 8 by 8 array of 6-mm-pitch Sensl J-Series silicon photomultipliers (SiPMs). With both single and multi-ROSSPAD testing, a detection package consisting of a 3-mm-thick sheet of EJ-200 plastic scintillator and a 3-mm-thick sheet of acrylic light spreader was coupled to the SiPM board face. After both quality assurance of the detector packages and the calibration …

Characterizing The Structure And Radiation Resistance Of Weberite-Type Complex Oxides, Igor M. Gussev

Doctoral Dissertations

Weberite-type A₃BO₇ oxides, where A is a trivalent rare earth and B is a pentavalent element like Ta, have been a focus of research due to the discovery of the weberite-type local atomic arrangement in ceramics with a defect-fluorite structure. Earlier studies primarily examined their long-range structures, leaving gaps in understanding their short-range atomic behavior. This thesis investigates various weberite-type tantalates across all structural scales. There has been debate over the long-range structure of Y₃TaO₇, a medium-sized rare earth tantalate oxide, particularly regarding its spacegroup symmetry. This work identifies Y₃TaO_{7 …}

The Nuclear System-Of-Systems Capabilities Analytic Process, Robert Boone Gilbreath

Doctoral Dissertations

This work includes the first known capabilities-based vulnerability analysis process able to evaluate a system of systems exposed to nuclear weapon environments: the Nuclear System-of-Systems Capabilities Analytic Process (NuSCAPTM). This approach, executed by an automated Python® application, calculates the magnitudes of eight nuclear weapon environment quantities by calling on the US Strategic Command Probability of Damage Calculator (PDCALC) code, the Los Alamos National Laboratory Simple Nuclear Effects Calculator (SNEC) program, and the Monte Carlo N-Particle® (MCNP®) code. Calculated nuclear weapon environment values are compared with user-provided dysfunction thresholds for all components, subsystems, and systems in the model to determine the …

Radiation Exposure Calibration Of The Al2o3:C With Radium-226 And Cesium-137 Using The Osl Method, Selma Tepeli Aydin

All Theses

Optically stimulated luminescence (OSL) dosimetry was utilized to calibrate Al₂O₃:C powder dosimeters, available commercially as the nanoDot® from Landauer Inc., and compare the dosimeter response to radium-226 (²²⁶Ra) and cesium-137 (¹³⁷Cs). The signal from the OSL was quantified using a microSTARii^® OSL reader also produced by Landauer Inc. Dose-response curves were developed for ²²⁶Ra and ¹³⁷Cs experiments (5 dosimeters each) at thirteen absorbed doses. Individual dosimeter response was tracked by serial number. Linear regression analysis was performed to determine if there were significant differences between the intercepts of the …

Preparation Of The Ej301d, A Deuterated Liquid Organic Scintillation Detector, For Spectroscopy Of Fast And High Energy Neutrons, Albert Du

Masters Theses

The focus of this research is on the preparation of a deuterated organic scintillation detector for fast and high energy neutron spectroscopy. The underlying physics of organic scintillation detectors, the process in which a neutron undergoes interaction with the detector material, as well as the readout and data processing procedure is introduced.

For methodology, a comprehensive setup of an EJ301-D deuterated organic scin- tillation detector is detailed. This includes algorithmic development for three distinct purposes. Firstly, it involves the creation of iterative unfolding algorithms, specif- ically the GRAVEL and Maximum Likelihood Expectation-Maximization (MLEM)

algorithm. The second development is conformal binning …

Uncertainty Quantification Framework For Design Optimization, Austin Ryan Williams

Masters Theses

Difficulty to obtain neutron sources of interest have driven the need for optimization
techniques to tailor a neutron generator as a replacement. A proposed solution uses
off-the-shelf neutron sources coupled with an energy-tuning assembly to mimic the
source of interest (i.e. AmLi, AmBe, thermonuclear fission spectra, etc.). These
energy-tuning assemblies have been designed with complex optimization algorithms
coupled with Monte Carlo simulations. These new system surrogate designs often
do not have an experimental counterpart for validation and comparison, and lack
non-statistical uncertainties. This work aims to improve confidence in the predictions
by providing a tool for fast uncertainty quantification to …

Application Of An Empirical Density Law Via Python For Aqueous Plutonium Chloride Systems For Mcnp6, Riley Bulso

Nuclear Engineering ETDs

A predictive density law has been implemented and developed into a Python tool to reduce bias and the high degree of conservatism in criticality safety calculations for aqueous plutonium chloride systems. Based upon available data and parameters, an empirical method was used to create this law. This method was used in the development of a Python tool to predict the density and composition of such a solution, which may then populate material data in an MCNP6 input file.

This tool and the density law equation have been verified against experimental data points for accuracy. Density is predicted with a maximum …

Direct Measurement Of The 114cd(��, ��)115cd Cross Section In The 1 Ev To 300 Kev Energy Range, Kofi Tutu Addo Assumin-Gyimah

Theses and Dissertations

The large thermal cross section of cadmium makes it ideal for many practical applications where screening of thermal neutrons is desired. For example, in non-destructive assay techniques, or for astrophysical studies of the s-process. All such applications require precise knowledge of the neutron-capture cross section on cadmium. Although there are some data on neutron-capture cross sections particularly at thermal energies and at energies relevant for astrophysics, there is very little data at most other energies. Further, the evaluated cross sections from the ENDF and JENDL databases disagree at high energies. Therefore, there is a critical need for precise knowledge of …

Development Of A Detailed And Reduced-Order Neutronics Models For Fusion Reactor Blanket And Systems Design Optimization, Felipe Santos Novais

Doctoral Dissertations

Fusion neutronics plays a critical role in the design and operation of fusion reactors. However, there are a number of challenges associated with fusion neutronics that must be overcome in order to help achieve practical and sustainable fusion energy. The primary objective of this project is to develop and demonstrate a broad neutronics analysis capability in support of system studies for U.S. concepts such as the Fusion Nuclear Science Facility (FNSF). According to a detailed TBR analysis that included an examination of reaction rates and the impact of facility (FNSf) components on neutron spectra and TBR, Li-6 will generate the …

Electrochemical Approaches To Life-Support Resources In Space Missions And Nuclear Technologies: Hydrogen Peroxide And Uranium Films, Armando Manuel Pena-Duarte

Open Access Theses & Dissertations

Space race has developed several technological advances that have achieved and continue to achieve the success of space missions in the aerospace timeline. Currently, the number of space technical and scientific innovations is still growing––demanding new materials and developments for extreme performing applications of fuel cells, batteries, supercapacitors, and systems of nuclear energy. Space missions require life-support solutions, auto-sustainable closed-loop living environments, cleaning and sanitizing solutions against pathogens, and safe nuclear-based resources of energy––with fissile materials with well-controlled dimensions within the core fuel elements. Likewise, to guarantee safety conditions, reduce costs, and facilitate operational logistics, space missions must reduce their …

Preparation Of High Entropy Titanite Pyrochlore And Radiation Stability Study, Adam Gootgeld

All Theses

Pyrochlore has been studied as a host phase for safe storage of radionuclides and exists naturally with long-term stability with good long-range order [1]. High entropy oxides show promising tunable properties that could demonstrate favorable bulk deposit of radioactive materials such as spent nuclear fuel (Uranium and other actinides). It is proposed that using high entropy oxides (HEOs) as the cation in this framework will shift the gibbs free energy so that radioactive nuclear waste will be stabilized for safe, long-term, eco-friendly storage. We have established a consistent method to fabricate high entropy titanite pyrochlores. In this study, ion beam …

A Comparison Of Fixed Versus Moving Eulerian Meshes For 1-D Radiative Shock Problems, Dylan Weatherred

Nuclear Engineering ETDs

Testing codes used to solve the radiation-hydrodynamics equations requires the use of radiative shock problems. These problems contain stiff shocks and test the coupling of the material motion and the energy exchange between the radiation and material. However, these problems are difficult to solve due to large differences in time scale between radiation and material equations, resolving shocks, and modeling radiation and material interactions. This thesis will look to solve radiative shock problems in 1-D using the Eulerian formulation on fixed and moving meshes. The moving mesh method proposed takes advantage of the more simple Eulerian formulation of the radiation …

Miniature, Submersible Electromagnetic Pumps Of Molten Lead And Sodium For Gen-Iv Nuclear Reactors Development, Ragai M. Altamimi

Nuclear Engineering ETDs

Heavy metals and alkali Liquid Metals are suitable coolants for Generation IV terrestrial nuclear reactors for operating at elevated temperatures for achieving plant thermal efficiency more than 40% and the thermochemical generation of hydrogen fuel. In addition, the low vapor pressure of these liquids eliminates the need for a pressure vessel and instead operates slightly below ambient pressure. A primary issue with the uses of these coolants is their compatibility with nuclear fuel, cladding and core structure materials at elevated temperatures more than 500oC. Therefore, in pile and out-of-pile test loops have been constructed or being considered for quantifying the …

Antineutrino Monitoring Studies Using Nuscale As A Case Study, Emma C. Houston

Masters Theses

The proposed growth of nuclear technology presents challenges to the current safeguard regimes [51]. Non-invasive, non-intrusive, and remote monitoring is desired to safeguard the new fleet of advanced reactors. Decades of antineutrino detector research has shown the ability for this technology to monitor nuclear reactors from significant standoff distances [64]. Antineutrino detectors can provide a Continuity of Knowledge, unique to the current safeguards framework [20]. In this study, we propose the use of an antineutrino detector, ”outside of the fence”, for safeguard applications at a mutli-core SMR site. Ideally, smaller and shallower antineutrino detectors could be used to reduce operational …

Sensitivity And Uncertainty Analysis Of Inertial Confinement Fusion Experiments, Colin A. Weaver

Nuclear Engineering ETDs

Sandia National Laboratories conducts Magnetized Liner Inertial Fusion (MagLIF) experiments at the Z Pulsed Power Facility. Their objective is to study the burning plasma formed under magnetic direct drive Inertial Confinement Fusion (ICF) conditions and use the inferred information to reduce uncertainty in computational models and improve experimental designs. The Z machine has five neutron time-of-flight (nToF) detectors that measure the fusion neutron time spectrum from three lines-of-sight. Together, these signals are used to infer the ion temperature, target liner mass density, and the burn history of the MagLIF experiment from measured data. These parameters are a few used by …

Measurements Of Scintillation Light Quenching For Protons In Rare-Earth Inorganic Scintillators, Tatiana Nathaly Espinoza

Nuclear Engineering ETDs

Scintillator detectors have become a leading choice of radiation detectors for a variety of applications, including space science. Due to their intrinsic characteristics, rare-earth inorganic scintillators provide the capability to detect both gamma and charged particles in a small detector. The response of these detectors is typically characterized using isotropic gamma sources. However, the light output produced in the scintillator from an incident gamma of a particular energy differs from the light output produced from an incident charged particle of the same energy; a phenomenon known as quenching. Using two types of rare-earth inorganic scintillators, Y2SiO5(YSO:Ce), and Gd₃Al₂Ga₃O₁₂(GAGG:Ce), we measured …

Conceptual Design And Preliminary Safety Analysis Of A Proposed Nuclear Microreactor For Mobile Application, A. S. M. Fakhrul Islam

Theses and Dissertations

Conceptual design and preliminary safety analysis of a proposed helium-cooled Micro Nuclear reactor In ONe megawatt (MINION) thermal output is done through three-dimensional computational analysis. Compared with the conventional high temperature gas-cooled reactors (HTGR) that use tri-structural or bi-structural isotropic (TRISO or BISO) fuel particles, MINION uses traditional clad fuel pellets. This greatly simplifies the core design and allows for a substantially more compact design thanks to the fuel’s signif-icantly higher U-235 atom density. Uranium carbide (UC) enriched up to 19.75% in U-235 is used as fuel. In the power-flattened design, U-235 enrichment varies radially between 19.75% and 10.5% in …

Vi Energy-Efficient Memristor-Based Neuromorphic Computing Circuits And Systems For Radiation Detection Applications, Jorge Iván Canales Verdial

Electrical and Computer Engineering ETDs

Radionuclide spectroscopic sensor data is analyzed with minimal power consumption through the use of neuromorphic computing architectures. Memristor crossbars are harnessed as the computational substrate in this non-conventional computing platform and integrated with CMOS-based neurons to mimic the computational dynamics observed in the mammalian brain’s visual cortex. Functional prototypes using spiking sparse locally competitive approximations are presented. The architectures are evaluated for classification accuracy and energy efficiency. The proposed systems achieve a 90% true positive accuracy with a high-resolution detector and 86% with a low-resolution detector.

Material Reliability For A Molten Chloride Salt System, Aaron A.H. Overacker

Nuclear Engineering ETDs

Energy efficiency and cost reduction can both be improved upon using overall higher temperatures for the working fluid. This interest is shared in both nuclear energy as well as concentrated solar power. To achieve higher temperatures would require industry to change working fluids. The United States Department of Energy set out a goal of operating concentrated solar to above 700℃. This would help reduce the cost by having more efficiency in the thermal energy storage, while not a concern for nuclear, these high temperatures can reduce the safety risk and pressure use with the implementation of molten salts. The National …

Nuclear Thermal Rocket Engine Instrumentation Addressing Environmental Limitations On Temperature Measurements, Dan C Floyd

Doctoral Dissertations

The development of nuclear thermal rockets has received renewed interest in recent years due to the benefits that can attained from this method of propulsion. Currently, instrumentation work is focused on the evaluation of current and near-term technology for implementation within a nuclear thermal rocket engine. One aspect of this evaluation is focused on the various instrumentation requirements of the system regarding necessary measurement parameters and environmental conditions for survivability. Historical nuclear rocket programs that have been conducted in the United States provide the basis for this information and indicates a critical need for high temperature measurement technology that can …

Sensitivity Analysis Of Thermophysical Properties Of Molten Salts Using A Molten Salt Demonstration Reactor Model In Transform, Sarah Elizabeth Creasman

Doctoral Dissertations

Molten Salt Reactors (MSRs) are currently of interest due to the push for smaller reactors that are easier to deploy and the need for sustainable energy around the world. Nuclear energy can play an important role in addressing the issue of energy inequality and climate change. One of the main obstacles to deploying MSRs is licensing. An important aspect to understand in terms of licensing is the uncertainty of the thermophysical properties of the molten salt at the beginning of the cycle and during normal operations and transients. MSRs have already been proven as a viable concept; two research reactors—The …

Fabrication, Measurements, And Modeling Of Semiconductor Radiation Detectors For Imaging And Detector Response Functions, Corey David Ahl

Doctoral Dissertations

In the first part of this dissertation, we cover the development of a diamond semiconductor alpha-tagging sensor for associated particle imaging to solve challenges with currently employed scintillators. The alpha-tagging sensor is a double-sided strip detector made from polycrystalline CVD diamond. The performance goals of the alpha-tagging sensor are 700-picosecond timing resolution and 0.5 mm spatial resolution. A literature review summarizes the methodology, goals, and challenges in associated particle imaging. The history and current state of alpha-tagging sensors, followed by the properties of diamond semiconductors are discussed to close the literature review. The materials and methods used to calibrate the …

Improved Spatial Resolution For Double-Sided Strip Detectors Using Lithium Indium Diselenide Semiconductors, Jake Alexander Gallagher

Doctoral Dissertations

This research focuses on the evaluation of lithium indium diselenide (LISe) semiconductors in double-sided strip detector (DSSDs) designs as an example for the potential to achieve unparalleled neutron detection efficiency, spatial resolution, and timing resolution detection. LISe semiconductors offer high neutron detection efficiency due to the ~25% atomic ratio of Lithium-6, maximizing its efficiency of ~75% with 1 mm thickness at 2.8 angstroms. Furthermore, the 4.78 MeV 𝑄-value enables high intrinsic gamma discrimination in a pixelated design (electron range). These characteristics make LISe an alternative option for neutron radiography, energy-resolved imaging, and other neutron interrogation techniques. This dissertation summarizes my …

Development Of A Low-Dose Radiation Therapy Device For Acute Respiratory Distress Syndrome, Thomas Heath Davis

Doctoral Dissertations

This research focuses on developing a low-dose radiotherapy (LD-RT) device for treating acute respiratory distress syndrome (ARDS). This respiratory illness affects millions of people a year. Using orthovoltage (200 – 500 keV) X-ray energy provides many advantages over traditional radiotherapy delivery with linear accelerators, such as low cost and greater accessibility. In addition, X-ray tubes have been shown throughout history to provide good treatment outcomes for pneumonia, and research has shown LD-RT to be just as effective with ARDS. This proposal summarizes my efforts in determining the dosimetric properties of an LD-RT system to deliver treatment quickly and effectively. My …

Total Absorption Spectroscopy Of Mo-106 And Tc-106, Michael Cooper

Doctoral Dissertations

Total absorption spectroscopy is a method of gamma-ray spectroscopy that has gained prominence in the past several decades, as nuclear data revisions are performed on older nuclear data, which is often incomplete. A strong understanding of underlying nuclear data, particularly fission and beta decay data, is essential for nuclear reactors and nuclear fuel decay heat. This PhD work involves the analysis of fission fragments 106Mo [Mo-106] and 106Tc [Tc-106]. These neutron rich isotopes contribute upwards of 6% of the cumulative fission yield of 241Pu [Pu-241] fission, and 4% of 239Pu [Pu-239] fission. Prior data for these two fission fragments only …

Use Of Automatic Metaheuristic Optimizations For Boron Neutron Capture Therapy, Christopher Busch

Masters Theses

Boron Neutron Capture therapy (BNCT) is a cancer treatment method investigated to reach malignant tumors that have added complications due to shape, size, or location. The unique property of BNCT is that it can deposit an immense dose gradient between the tumor cells and normal cells. This is done by selectively concentrating boron compounds in tumor cells and then irradiating the cells with an epithermal neutron beam. Due to complex nature of neutron interactions, a high fidelity neutronic model is needed to design and predict the outcomes of a BNCT experiment. This work aims to introduce a high level autonomous …