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Full-Text Articles in Engineering
Seasonal Variability And Long-Term Evolution Of Tropospheric Composition In The Tropics And Southern Hemisphere, K. M. Wai, S. Wu, A. Kumar, H. Liao
Seasonal Variability And Long-Term Evolution Of Tropospheric Composition In The Tropics And Southern Hemisphere, K. M. Wai, S. Wu, A. Kumar, H. Liao
Michigan Tech Publications
Impacts on tropospheric composition in the tropics and the Southern Hemisphere from biomass burning and other emission sources are studied using a global chemical transport model, surface measurements and satellite retrievals. Seasonal variations in observed CO at remote island sites are examined. Easter Island (eastern Pacific Ocean) is impacted indirectly by the hemispheric zonal transport of CO due to the burning in southern Africa/South America, via the westerlies. An increasing trend in CO by 0.33 ppb yr-1 in the past decade at Ascension Island is attributed to the combined effects of South American/southern Africa burnings and the increases in CH4 …
Projected Effect Of 2000-2050 Changes In Climate And Emissions On Aerosol Levels In China And Associated Transboundary Transport, H. Jiang, H. Liao, H. O.T. Pye, S. Wu, L. J. Mickley, J. H. Seinfeld, X. Y. Zhang
Projected Effect Of 2000-2050 Changes In Climate And Emissions On Aerosol Levels In China And Associated Transboundary Transport, H. Jiang, H. Liao, H. O.T. Pye, S. Wu, L. J. Mickley, J. H. Seinfeld, X. Y. Zhang
Michigan Tech Publications
We investigate projected 2000-2050 changes in concentrations of aerosols in China and the associated transboundary aerosol transport by using the chemical transport model GEOS-Chem driven by the Goddard Institute for Space Studies (GISS) general circulation model (GCM) 3 at 4° × 5° resolution. Future changes in climate and emissions projected by the IPCC A1B scenario are imposed separately and together through sensitivity simulations. Accounting for sulfate, nitrate, ammonium, black carbon (BC), and organic carbon (OC) aerosols, concentrations of individual aerosol species change by -1.5 to +0.8 μg m-3, and PM2.5 levels are projected to change by about 10-20% in eastern …
Impact Of Aging Mechanism On Model Simulated Carbonaceous Aerosols, Y. Huang, S. Wu, M. K. Dubey, N. H.F. French
Impact Of Aging Mechanism On Model Simulated Carbonaceous Aerosols, Y. Huang, S. Wu, M. K. Dubey, N. H.F. French
Michigan Tech Publications
Carbonaceous aerosols including organic carbon and black carbon have significant implications for both climate and air quality. In the current global climate or chemical transport models, a fixed hydrophobic-to-hydrophilic conversion lifetime for carbonaceous aerosol (τ) is generally assumed, which is usually around one day. We have implemented a new detailed aging scheme for carbonaceous aerosols in a chemical transport model (GEOS-Chem) to account for both the chemical oxidation and the physical condensation-coagulation effects, where τ is affected by local atmospheric environment including atmospheric concentrations of water vapor, ozone, hydroxyl radical and sulfuric acid. The updated τ exhibits large spatial and …
Quantifying The Impact Of Boreal Forest Fires On Tropospheric Oxidants Over The Atlantic Using Aircraft And Satellites (Bortas) Experiment: Design, Execution And Science Overview, P. I. Palmer, M. Parrington, J. D. Lee, A. C. Lewis, A. R. Rickard, P. F. Bernath, T. J. Duck, D. L. Waugh, D. W. Tarasick, R. C. Owen, Et. Al.
Quantifying The Impact Of Boreal Forest Fires On Tropospheric Oxidants Over The Atlantic Using Aircraft And Satellites (Bortas) Experiment: Design, Execution And Science Overview, P. I. Palmer, M. Parrington, J. D. Lee, A. C. Lewis, A. R. Rickard, P. F. Bernath, T. J. Duck, D. L. Waugh, D. W. Tarasick, R. C. Owen, Et. Al.
Michigan Tech Publications
We describe the design and execution of the BORTAS (Quantifying the impact of BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites) experiment, which has the overarching objective of understanding the chemical aging of air masses that contain the emission products from seasonal boreal wildfires and how these air masses subsequently impact downwind atmospheric composition. The central focus of the experiment was a two-week deployment of the UK BAe-146-301 Atmospheric Research Aircraft (ARA) over eastern Canada, based out of Halifax, Nova Scotia. Atmospheric ground-based and sonde measurements over Canada and the Azores associated with the planned …
Modeling Of 2008 Kasatochi Volcanic Sulfate Direct Radiative Forcing: Assimilation Of Omi So < Inf> 2 Plume Height Data And Comparison With Modis And Caliop Observations, J. Wang, S. Park, J. Zeng, C. Ge, K. Yang, S. Carn, N. Krotkov, A. H. Omar
Modeling Of 2008 Kasatochi Volcanic Sulfate Direct Radiative Forcing: Assimilation Of Omi So < Inf> 2 Plume Height Data And Comparison With Modis And Caliop Observations, J. Wang, S. Park, J. Zeng, C. Ge, K. Yang, S. Carn, N. Krotkov, A. H. Omar
Michigan Tech Publications
Volcanic SO2 column amount and injection height retrieved from the Ozone Monitoring Instrument (OMI) with the Extended Iterative Spectral Fitting (EISF) technique are used to initialize a global chemistry transport model (GEOS-Chem) to simulate the atmospheric transport and lifecycle of volcanic SO2 and sulfate aerosol from the 2008 Kasatochi eruption, and to subsequently estimate the direct shortwave, top-of-the-atmosphere radiative forcing of the volcanic sulfate aerosol. Analysis shows that the integrated use of OMI SO2 plume height in GEOS-Chem yields: (a) good agreement of the temporal evolution of 3-D volcanic sulfate distributions between model simulations and satellite observations from the Moderate …
Validation Of The Fall3d Model For The 2008 Chaitén Eruption Using Field And Satellite Data, María Soledad Osores, Arnau Folch, Estela Collini, Gustavo Villarosa, Adam J. Durant, Gloria Pujol, José G. Viramonte
Validation Of The Fall3d Model For The 2008 Chaitén Eruption Using Field And Satellite Data, María Soledad Osores, Arnau Folch, Estela Collini, Gustavo Villarosa, Adam J. Durant, Gloria Pujol, José G. Viramonte
Michigan Tech Publications
The 2008 Chaitén Volcano eruption began on 2 May 2008 with an explosive phase that injected large amounts of tephra into the atmosphere. During the first week of the eruption, volcanic ash clouds were transported for hundreds of kilometres over Argentina by the prevailing westerly winds. Tephra deposition extended to the Atlantic Ocean and severely affected the Argentinean Patagonia. Impacts included air and water quality degradation, disruption of ground transportation systems and cancellation of flights at airports more than 1,500 km apart. We use the FALL3D tephra transport model coupled with the Weather Research and Forecasting-Advanced Research Weather (WRF-ARW) meteorological …
Impacts Of Changes In Land Use And Land Cover On Atmospheric Chemistry And Air Quality Over The 21st Century, S. Wu, L. J. Mickley, J. O. Kaplan, D. J. Jacob
Impacts Of Changes In Land Use And Land Cover On Atmospheric Chemistry And Air Quality Over The 21st Century, S. Wu, L. J. Mickley, J. O. Kaplan, D. J. Jacob
Michigan Tech Publications
The effects of future land use and land cover change on the chemical composition of the atmosphere and air quality are largely unknown. To investigate the potential effects associated with future changes in vegetation driven by atmospheric CO 2 concentrations, climate, and anthropogenic land use over the 21st century, we performed a series of model experiments combining a general circulation model with a dynamic global vegetation model and an atmospheric chemical-transport model. Our results indicate that climate-and CO 2-induced changes in vegetation composition and density between 2100 and 2000 could lead to decreases in summer afternoon surface ozone of up …
Ethane, Ethyne And Carbon Monoxide Concentrations In The Upper Troposphere And Lower Stratosphere From Ace And Geos-Chem: A Comparison Study, G. González Abad, N. D.C. Allen, P. F. Bernath, C. D. Boone, S. D. Mcleod, G. L. Manney, G. C. Toon, C. Carouge, Y. Wang, Shiliang Wu, X
Ethane, Ethyne And Carbon Monoxide Concentrations In The Upper Troposphere And Lower Stratosphere From Ace And Geos-Chem: A Comparison Study, G. González Abad, N. D.C. Allen, P. F. Bernath, C. D. Boone, S. D. Mcleod, G. L. Manney, G. C. Toon, C. Carouge, Y. Wang, Shiliang Wu, X
Michigan Tech Publications
Near global upper tropospheric concentrations of carbon monoxide (CO), ethane (C2H6) and ethyne (C2H2) from ACE (Atmospheric Chemistry Experiment) Fourier transform spectrometer on board the Canadian satellite SCISAT-1 are presented and compared with the output from the Chemical Transport Model (CTM) GEOS-Chem. The retrievals of ethane and ethyne from ACE have been improved for this paper by using new sets of microwindows compared with those for previous versions of ACE data. With the improved ethyne retrieval we have been able to produce a near global upper tropospheric distribution of C2H2 from space. Carbon monoxide, ethane and ethyne concentrations retrieved using …
Opportunistic Validation Of Sulfur Dioxide In The Sarychev Peak Volcanic Eruption Cloud, S. Carn, T. M. Lopez
Opportunistic Validation Of Sulfur Dioxide In The Sarychev Peak Volcanic Eruption Cloud, S. Carn, T. M. Lopez
Michigan Tech Publications
We report attempted validation of Ozone Monitoring Instrument (OMI) sulfur dioxide (SO 2) retrievals in the stratospheric volcanic cloud from Sarychev Peak (Kurile Islands) in June 2009, through opportunistic deployment of a ground-based ultraviolet (UV) spectrometer (FLYSPEC) as the volcanic cloud drifted over central Alaska. The volcanic cloud altitude (∼12-14 km) was constrained using coincident CALIPSO lidar observations. By invoking some assumptions about the spatial distribution of SO 2, we derive averages of FLYSPEC vertical SO 2 columns for comparison with OMI SO 2 measurements. Despite limited data, we find minimum OMI-FLYSPEC differences within measurement uncertainties, which support the validity …
Sulphur Dioxide As A Volcanic Ash Proxy During The April-May 2010 Eruption Of Eyjafjallajökull Volcano, Iceland, H. E. Thomas, A. J. Prata
Sulphur Dioxide As A Volcanic Ash Proxy During The April-May 2010 Eruption Of Eyjafjallajökull Volcano, Iceland, H. E. Thomas, A. J. Prata
Michigan Tech Publications
The volcanic ash cloud from the eruption of Eyjafjallajökull volcano in April and May 2010 resulted in unprecedented disruption to air traffic in Western Europe causing significant financial losses and highlighting the importance of efficient volcanic cloud monitoring. The feasibility of using SO2 as a tracer for the ash released during the eruption is investigated here through comparison of ash retrievals from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) with SO2 measurements from a number of infrared and ultraviolet satellite-based sensors. Results demonstrate that the eruption can be divided into an initial ash-rich phase, a lower intensity middle phase …
Impacts Of Future Climate Change And Effects Of Biogenic Emissions On Surface Ozone And Particulate Matter Concentrations In The United States, Y. F. Lam, J. S. Fu, S. Wu, L. J. Mickley
Impacts Of Future Climate Change And Effects Of Biogenic Emissions On Surface Ozone And Particulate Matter Concentrations In The United States, Y. F. Lam, J. S. Fu, S. Wu, L. J. Mickley
Michigan Tech Publications
Simulations of present and future average regional ozone and PM 2.5 concentrations over the United States were performed to investigate the potential impacts of global climate change and emissions on regional air quality using CMAQ. Various emissions and climate conditions with different biogenic emissions and domain resolutions were implemented to study the sensitivity of future air quality trends from the impacts of changing biogenic emissions. A comparison of GEOS-Chem and CMAQ was performed to investigate the effect of downscaling on the prediction of future air quality trends. For ozone, the impacts of global climate change are relatively smaller when compared …
Determination Of Time-And Height-Resolved Volcanic Ash Emissions And Their Use For Quantitative Ash Dispersion Modeling: The 2010 Eyjafjallajökull Eruption, A. Stohl, A. J. Prata, S. Eckhardt, L. Clarisse, A. Durant, S. Henne, N. I. Kristiansen, A. Minikin, U. Schumann, P. Seibert, K. Stebel, H. E. Thomas, T. Thorsteinsson, K. Tørseth, B. Weinzierl
Determination Of Time-And Height-Resolved Volcanic Ash Emissions And Their Use For Quantitative Ash Dispersion Modeling: The 2010 Eyjafjallajökull Eruption, A. Stohl, A. J. Prata, S. Eckhardt, L. Clarisse, A. Durant, S. Henne, N. I. Kristiansen, A. Minikin, U. Schumann, P. Seibert, K. Stebel, H. E. Thomas, T. Thorsteinsson, K. Tørseth, B. Weinzierl
Michigan Tech Publications
The Aprilg-May, 2010 volcanic eruptions of Eyjafjallajökull, Iceland caused significant economic and social disruption in Europe whilst state of the art measurements and ash dispersion forecasts were heavily criticized by the aviation industry. Here we demonstrate for the first time that large improvements can be made in quantitative predictions of the fate of volcanic ash emissions, by using an inversion scheme that couples a priori source information and the output of a Lagrangian dispersion model with satellite data to estimate the volcanic ash source strength as a function of altitude and time. From the inversion, we obtain a total fine …
Source Attribution And Interannual Variability Of Arctic Pollution In Spring Constrained By Aircraft (Arctas, Arcpac) And Satellite (Airs) Observations Of Carbon Monoxide, J. A. Fisher, D. J. Jacob, M. T. Purdy, M. Kopacz, P. Le Sager, Shiliang Wu, Et. Al.
Source Attribution And Interannual Variability Of Arctic Pollution In Spring Constrained By Aircraft (Arctas, Arcpac) And Satellite (Airs) Observations Of Carbon Monoxide, J. A. Fisher, D. J. Jacob, M. T. Purdy, M. Kopacz, P. Le Sager, Shiliang Wu, Et. Al.
Michigan Tech Publications
We use aircraft observations of carbon monoxide (CO) from the NASA ARCTAS and NOAA ARCPAC campaigns in April 2008 together with multiyear (2003–2008) CO satellite data from the AIRS instrument and a global chemical transport model (GEOS-Chem) to better understand the sources, transport, and interannual variability of pollution in the Arctic in spring. Model simulation of the aircraft data gives best estimates of CO emissions in April 2008 of 26 Tg month−1 for Asian anthropogenic, 9.4 for European anthropogenic, 4.1 for North American anthropogenic, 15 for Russian biomass burning (anomalously large that year), and 23 for Southeast Asian biomass burning. …
Technical Note: A New Method For The Lagrangian Tracking Of Pollution Plumes From Source To Receptor Using Gridded Model Output, R. C. Owen, R. E. Honrath
Technical Note: A New Method For The Lagrangian Tracking Of Pollution Plumes From Source To Receptor Using Gridded Model Output, R. C. Owen, R. E. Honrath
Michigan Tech Publications
Lagrangian particle dispersion models (LPDMs) are powerful and popular tools used for the analysis of atmospheric trace gas measurements. However, it can be difficult to determine the transport pathway of emissions from their source to a receptor using the standard gridded model output, particularly during complex meteorological scenarios. In this paper we present a method to clearly and easily identify the pathway taken by only those emissions that arrive at a receptor at a particular time, by combining the standard gridded output from forward (e.g., concentration) and backward (e.g., residence time) LPDM simulations. By comparing the pathway determined from this …