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Magnetic Transitions In Disordered Gdal2, D. Williams, Paul Shand, Thomas Pekarek, Ralph Skomski, Valeri Petkov, Diandra Leslie-Pelecky
Magnetic Transitions In Disordered Gdal2, D. Williams, Paul Shand, Thomas Pekarek, Ralph Skomski, Valeri Petkov, Diandra Leslie-Pelecky
Thomas M. Pekarek
The role of disorder in magnetic ordering transitions is investigated using mechanically milled GdAl2. Crystalline GdAl2 is a ferromagnet while amorphous GdAl2 is a spin glass. Nanostructured GdAl2 shows a paramagnetic-to-ferromagnetic transition and glassy behavior, with the temperature and magnitude of each transition dependent on the degree and type of disorder. Disorder is parametrized by a Gaussian distribution of Curie temperatures TC with mean TC and breadth Δ TC. A nonzero coercivity is observed at temperatures more than 20 K above the highest TC of any known Gd-Al phase; however, the coercivity decreases with decreasing temperature over the same temperature …
Disorder-Induced Depression Of The Curie Temperature In Mechanically Milled Gdal2, Marco Morales Torres, D. Williams, Paul Shand, C. Stark, Thomas Pekarek, L. Yue, Valeri Petkov, Diandra Leslie-Pelecky
Disorder-Induced Depression Of The Curie Temperature In Mechanically Milled Gdal2, Marco Morales Torres, D. Williams, Paul Shand, C. Stark, Thomas Pekarek, L. Yue, Valeri Petkov, Diandra Leslie-Pelecky
Thomas M. Pekarek
The effect of disorder on the ferromagnetic transition is investigated in mechanically milled GdAl2. GdAl2is a ferromagnet when crystalline and a spin glass when amorphous. Mechanical milling progressively disorders the alloy, allowing observation of the change from ferromagnetic to a disordered magnetic state. X-ray diffraction and pair-distribution-function analysis are used to determine the grain size, lattice parameter, and mean-squared atomic displacements. The magnetization as a function of temperature is described by a Gaussian distribution of Curie temperatures. The mean Curie temperature decreases with decreasing lattice parameter, where lattice parameter serves as a measure of defect concentration. Two different rates of …