Open Access. Powered by Scholars. Published by Universities.®
Social and Behavioral Sciences Commons™
Open Access. Powered by Scholars. Published by Universities.®
Articles 1 - 8 of 8
Full-Text Articles in Social and Behavioral Sciences
Effects Of Atmospheric Light Scattering On Spectroscopic Observations Of Greenhouse Gases From Space: Validation Of Ppdf-Based Co 2 Retrievals From Gosat, Sergey Oshchepkov, Andrey Bril, Tatsuya Yokota, Isamu Morino, Yukio Yoshida, Tsuneo Matsunaga, Dmitry Belikov, Debra Wunch, Paul Wennberg, Geoffrey Toon, Christopher O'Dell, André Butz, Sandrine Guerlet, Austin Cogan, Hartmut Boesch, Nawo Eguchi, Nicholas Deutscher, David Griffith, Ronald Macatangay, Justus Notholt, Ralf Sussmann, Markus Rettinger, Vanessa Sherlock, John Robinson, Esko Kyro, Pauli Heikkinen, Dietrich G. Feist, Tomoo Nagahama, Nikolay Kadygrov, Shamil Maksyutov, Osamu Uchino, Hiroshi Watanabe
Effects Of Atmospheric Light Scattering On Spectroscopic Observations Of Greenhouse Gases From Space: Validation Of Ppdf-Based Co 2 Retrievals From Gosat, Sergey Oshchepkov, Andrey Bril, Tatsuya Yokota, Isamu Morino, Yukio Yoshida, Tsuneo Matsunaga, Dmitry Belikov, Debra Wunch, Paul Wennberg, Geoffrey Toon, Christopher O'Dell, André Butz, Sandrine Guerlet, Austin Cogan, Hartmut Boesch, Nawo Eguchi, Nicholas Deutscher, David Griffith, Ronald Macatangay, Justus Notholt, Ralf Sussmann, Markus Rettinger, Vanessa Sherlock, John Robinson, Esko Kyro, Pauli Heikkinen, Dietrich G. Feist, Tomoo Nagahama, Nikolay Kadygrov, Shamil Maksyutov, Osamu Uchino, Hiroshi Watanabe
Faculty of Science - Papers (Archive)
This report describes a validation study of Greenhouse gases Observing Satellite (GOSAT) data processing using ground-based measurements of the Total Carbon Column Observing Network (TCCON) as reference data for column-averaged dry air mole fractions of atmospheric carbon dioxide (X CO2). We applied the photon path length probability density function method to validate X CO2 retrievals from GOSAT data obtained during 22months starting from June 2009. This method permitted direct evaluation of optical path modifications due to atmospheric light scattering that would have a negligible impact on ground-based TCCON measurements but could significantly affect gas retrievals when observing reflected sunlight from …
Atmospheric Greenhouse Gases Retrieved From Sciamachy: Comparison To Ground-Based Fts Measurements And Model Results, O Schneising, P Bergamaschi, H Bovensmann, M Buchwitz, J P. Burrows, N M. Deutscher, D W. T Griffith, J Heymann, R Macatangay, J Messerschmidt, J Notholt, M Rettinger, M Reuter, R Sussmann, Voltaire A. Velazco, T Warneke, P O. Wennberg, D Wunch
Atmospheric Greenhouse Gases Retrieved From Sciamachy: Comparison To Ground-Based Fts Measurements And Model Results, O Schneising, P Bergamaschi, H Bovensmann, M Buchwitz, J P. Burrows, N M. Deutscher, D W. T Griffith, J Heymann, R Macatangay, J Messerschmidt, J Notholt, M Rettinger, M Reuter, R Sussmann, Voltaire A. Velazco, T Warneke, P O. Wennberg, D Wunch
Faculty of Science - Papers (Archive)
SCIAMACHY onboard ENVISAT (launched in 2002) enables the retrieval of global long-term columnaveraged dry air mole fractions of the two most important anthropogenic greenhouse gases carbon dioxide and methane (denoted XCO2 and XCH4). In order to assess the quality of the greenhouse gas data obtained with the recently introduced v2 of the scientific retrieval algorithm WFM-DOAS, we present validations with ground-based Fourier Transform Spectrometer (FTS) measurements and comparisons with model results at eight Total Carbon Column Observing Network (TCCON) sites providing realistic error estimates of the satellite data. Such validation is a prerequisite to assess the suitability …
A Fourier Transform Infrared Trace Gas And Isotope Analyser For Atmospheric Applications, D W. T Griffith, N M. Deutscher, C Caldow, G Kettlewell, M Riggenbach, S Hammer
A Fourier Transform Infrared Trace Gas And Isotope Analyser For Atmospheric Applications, D W. T Griffith, N M. Deutscher, C Caldow, G Kettlewell, M Riggenbach, S Hammer
Faculty of Science - Papers (Archive)
Concern in recent decades about human impacts on Earth's climate has led to the need for improved and expanded measurement capabilities of greenhouse gases in the atmosphere. In this paper we describe in detail an in situ trace gas analyser based on Fourier Transform Infrared (FTIR) spectroscopy that is capable of simultaneous and continuous measurements of carbon dioxide (CO2), methane (CH4), carbon monoxide (CO), nitrous oxide (N2O) and 13C in CO2 in air with high precision. High accuracy is established by reference to measurements of standard reference gases. Stable water isotopes can …
Gas-Particle Partitioning Of Atmospheric Hg(Ii) And Its Effect On Global Mercury Deposition, H M. Amos, D J. Jacob, C D. Holmes, Jenny A. Fisher, Q Wang, R M. Yantosca, E S. Corbitt, E Galarneau, A P. Rutter, M S. Gustin, A Steffen, J J. Schauer, J A. Graydon, V L. St Louis, R W. Talbot, E S. Edgerton, Y Zhang, E N. Sunderland
Gas-Particle Partitioning Of Atmospheric Hg(Ii) And Its Effect On Global Mercury Deposition, H M. Amos, D J. Jacob, C D. Holmes, Jenny A. Fisher, Q Wang, R M. Yantosca, E S. Corbitt, E Galarneau, A P. Rutter, M S. Gustin, A Steffen, J J. Schauer, J A. Graydon, V L. St Louis, R W. Talbot, E S. Edgerton, Y Zhang, E N. Sunderland
Faculty of Science - Papers (Archive)
Atmospheric deposition represents a major input of mercury to surface environments. The phase of mercury (gas or particle) has important implications for its removal from the atmosphere. We use long-term observations of reactive gaseous mercury (RGM), particle-bound mercury (PBM), fine particulate matter (PM2.5), and temperature at five sites in North America to derive an empirical gas-particle partitioning relationship log10(K-1) = (10 ± 1) − (2500 ± 300)/T where K = (PBM/PM2.5)/RGM with PBM and RGM in common mixing ratio units, PM2.5 in μg m−3, and T in …
Riverine Source Of Arctic Ocean Mercury Inferred From Atmospheric Observations, Jenny A. Fisher, Daniel J. Jacob, Anne L. Soerensen, Helen M. Amos, Alexandra Steffen, Elsie M. Sunderland
Riverine Source Of Arctic Ocean Mercury Inferred From Atmospheric Observations, Jenny A. Fisher, Daniel J. Jacob, Anne L. Soerensen, Helen M. Amos, Alexandra Steffen, Elsie M. Sunderland
Faculty of Science - Papers (Archive)
Methylmercury is a potent neurotoxin that accumulates in aquatic food webs. Human activities, including industry and mining, have increased inorganic mercury inputs to terrestrial and aquatic ecosystems. Methylation of this mercury generates methylmercury, and is thus a public health concern. Marine methylmercury is a particular concern in the Arctic, where indigenous peoples rely heavily on marine-based diets. In the summer, atmospheric inorganic mercury concentrations peak in the Arctic, whereas they reach a minimum in the northern mid-latitudes. Here, we use a global three-dimensional ocean–atmosphere model to examine the cause of this Arctic summertime maximum. According to our simulations, circumpolar rivers …
Atmospheric Carbon Dioxide Retrieved From The Greenhouse Gases Observing Satellite (Gosat): Comparison With Ground-Based Tccon Observations And Geos-Chem Model Calculations, A Cogan, H Boesch, R Parker, L Feng, Paul Palmer, J-F Blavier, Nicholas M. Deutscher, Ronald Macatangay, Justus Notholt, C M. Roehl, Thorsten Warneke, Debra Wunch
Atmospheric Carbon Dioxide Retrieved From The Greenhouse Gases Observing Satellite (Gosat): Comparison With Ground-Based Tccon Observations And Geos-Chem Model Calculations, A Cogan, H Boesch, R Parker, L Feng, Paul Palmer, J-F Blavier, Nicholas M. Deutscher, Ronald Macatangay, Justus Notholt, C M. Roehl, Thorsten Warneke, Debra Wunch
Faculty of Science - Papers (Archive)
We retrieved column-averaged dry air mole fractions of atmospheric carbon dioxide (XCO 2) from backscattered short-wave infrared (SWIR) sunlight measured by the Japanese Greenhouse gases Observing SATellite (GOSAT). Over two years of XCO 2 retrieved from GOSAT is compared with XCO 2 inferred from collocated SWIR measurements by seven ground-based Total Carbon Column Observing Network (TCCON) stations. The average difference between GOSAT and TCCON XCO 2 for individual TCCON sites ranges from -0.87 ppm to 0.77 ppm with a mean value of 0.1 ppm and standard deviation of 0.56 ppm. We find an average bias between all GOSAT and TCCON …
Atmospheric Tomography: A Bayesian Inversion Technique For Determining The Rate And Location Of Fugitive Emissions, Ruhi Humphries, Charles Jenkins, Ray Leuning, Steve Zegelin, David Griffith, Christopher Caldow, Henry Berko, Andrew Feitz
Atmospheric Tomography: A Bayesian Inversion Technique For Determining The Rate And Location Of Fugitive Emissions, Ruhi Humphries, Charles Jenkins, Ray Leuning, Steve Zegelin, David Griffith, Christopher Caldow, Henry Berko, Andrew Feitz
Faculty of Science - Papers (Archive)
A Bayesian inversion technique to determine the location and strength of trace gas emissions from a point source in open air is presented. It was tested using atmospheric measurements of N2O and CO2 released at known rates from a source located within an array of eight evenly spaced sampling points on a 20 m radius circle. The analysis requires knowledge of concentration enhancement downwind of the source and the normalized, three-dimensional distribution (shape) of concentration in the dispersion plume. The influence of varying background concentrations of ~1% for N2O and ~10% for CO2 was removed by subtracting upwind concentrations from …
Technical Note: Latitude-Time Variations Of Atmospheric Column-Average Dry Air Mole Fractions Of Co2, Ch4 And N2o, R Saito, P K. Patra, N Deutscher, D Wunch, K Ishijima, V Sherlock, T Blumenstock, S Dohe, D Griffith, F Hase, P Heikkinen, E Kyro, R Macatangay, J Mendonca, J Messerschmidt, I Morino, J Notholt, M Rettinger, K Strong, R Sussmann, T Warneke
Technical Note: Latitude-Time Variations Of Atmospheric Column-Average Dry Air Mole Fractions Of Co2, Ch4 And N2o, R Saito, P K. Patra, N Deutscher, D Wunch, K Ishijima, V Sherlock, T Blumenstock, S Dohe, D Griffith, F Hase, P Heikkinen, E Kyro, R Macatangay, J Mendonca, J Messerschmidt, I Morino, J Notholt, M Rettinger, K Strong, R Sussmann, T Warneke
Faculty of Science - Papers (Archive)
We present a comparison of an atmospheric general circulation model (AGCM)-based chemistry-transport model (ACTM) simulation with total column measurements of CO2, CH4 and N2O from the Total Carbon Column Observing Network (TCCON). The model is able to capture observed trends, seasonal cycles and inter hemispheric gradients at most sampled locations for all three species. The model-observation agreements are best for CO2, because the simulation uses fossil fuel inventories and an inverse model estimate of non-fossil fuel fluxes. The ACTM captures much of the observed seasonal variability in CO2 and N2O total columns (similar to 81% variance, R > 0.9 between ACTM …