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Full-Text Articles in Physical Sciences and Mathematics
Solution-Printed Organic Semiconductor Blends Exhibiting Transport Properties On Par With Single Crystals, Muhammad R. Niazi, Ruipeng Li, Er Qiang Li, Ahmad R. Kirmani, Maged Abdelsamie, Qingxiao Wang, Wenyang Pan, Marcia M. Payne, John E. Anthony, Detlef-M. Smilgies, Sigurdur T. Thoroddsen, Emmanuel P. Giannelis, Aram Amassian
Solution-Printed Organic Semiconductor Blends Exhibiting Transport Properties On Par With Single Crystals, Muhammad R. Niazi, Ruipeng Li, Er Qiang Li, Ahmad R. Kirmani, Maged Abdelsamie, Qingxiao Wang, Wenyang Pan, Marcia M. Payne, John E. Anthony, Detlef-M. Smilgies, Sigurdur T. Thoroddsen, Emmanuel P. Giannelis, Aram Amassian
Chemistry Faculty Publications
Solution-printed organic semiconductors have emerged in recent years as promising contenders for roll-to-roll manufacturing of electronic and optoelectronic circuits. The stringent performance requirements for organic thin-film transistors (OTFTs) in terms of carrier mobility, switching speed, turn-on voltage and uniformity over large areas require performance currently achieved by organic single-crystal devices, but these suffer from scale-up challenges. Here we present a new method based on blade coating of a blend of conjugated small molecules and amorphous insulating polymers to produce OTFTs with consistently excellent performance characteristics (carrier mobility as high as 6.7 cm2V−1s−1, low threshold …
Low-Voltage Polymer/Small-Molecule Blend Organic Thin-Film Transistors And Circuits Fabricated Via Spray Deposition, Simon Hunter, Jeremy W. Ward, Marcia M. Payne, John E. Anthony, Oana D. Jurchescu, Thomas D. Anthopoulos
Low-Voltage Polymer/Small-Molecule Blend Organic Thin-Film Transistors And Circuits Fabricated Via Spray Deposition, Simon Hunter, Jeremy W. Ward, Marcia M. Payne, John E. Anthony, Oana D. Jurchescu, Thomas D. Anthopoulos
Chemistry Faculty Publications
Organic thin-film electronics have long been considered an enticing candidate in achieving high-throughput manufacturing of low-power ubiquitous electronics. However, to achieve this goal, more work is required to reduce operating voltages and develop suitable mass-manufacture techniques. Here, we demonstrate low-voltage spray-cast organic thin-film transistors based on a semiconductor blend of 2,8-difluoro- 5,11-bis (triethylsilylethynyl) anthradithiophene and poly(triarylamine). Both semiconductor and dielectric films are deposited via successive spray deposition in ambient conditions (air with 40%–60% relative humidity) without any special precautions. Despite the simplicity of the deposition method, p-channel transistors with hole mobilities of >1 cm2/Vs are realized at −4 …