Physical Sciences and Mathematics Commons^™

Charge Transfer In Slow Collisions Of C⁴⁺ With H Below 1 Kev/Amu, Chen-Nan Liu, Anh-Thu Le, C. D. Lin

Physics Faculty Research & Creative Works

We reexamined charge-transfer cross sections for C⁴⁺ + H collisions for energies from 1 meV/amu to 1 keV/amu using the recently developed hyperspherical close-coupling method. Our results agree with several previous theoretical calculations using molecular-orbital expansion. However, these converged theoretical predictions do not agree with total cross sections from the merged-beam experiments.

Environment-Induced Degradation And Crack-Growth Studies Of Candidate Target Materials: Quarterly Progress Report (June 1 – August 31, 2003), Ajit K. Roy, Brendan O'Toole

Transmutation Sciences Materials (TRP)

As indicated in the original proposal, the primary objective of this task is to evaluate the effect of hydrogen on environment-assisted cracking of candidate target materials for applications in spallationneutron- target (SNT) systems such as accelerator production of tritium (APT) and accelerator transmutation of waste (ATW). The materials selected for evaluation and characterization are martensitic stainless steels including Alloy HT-9, Alloy EP 823 and Type 422 stainless steel. The susceptibility to stress corrosion cracking (SCC) and hydrogen embrittlement (HE) of these materials are being evaluated in aqueous environments of interest using tensile specimens under constant load and slow-strain-rate (SSR) conditions. …

Perturbation Approach To The Self-Energy Of Non-S Hydrogenic States, Eric Olivier Le Bigot, Ulrich D. Jentschura, Peter J. Mohr, Paul Indelicato, Gerhard Soff

Physics Faculty Research & Creative Works

We present results on the self-energy correction to the energy levels of hydrogen and hydrogenlike ions. The self energy represents the largest QED correction to the relativistic (Dirac-Coulomb) energy of a bound electron. We focus on the perturbation expansion of the self energy of non-S states, and provide estimates of the so-called A₆₀ perturbative coefficient, which can be considered as a relativistic Bethe logarithm. Precise values of A₆₀ are given for many P, D, F and G states, while estimates are given for other electronic states. These results can be used in high-precision spectroscopy experiments in hydrogen and …

Day 1. Monday, August 11, 2003: National Renewable Energy Lab, National Energy Renewable Laboratory

Energy Field Tour 2003 (August 11-16)

8 pages (includes illustrations).

Contains references.

Environment-Induced Degradation And Crack-Growth Studies Of Candidate Target Materials: Annual Progress Report (May 2002 – May 2003), Ajit K. Roy, Brendan O'Toole

Transmutation Sciences Materials (TRP)

As indicated in the original proposal, the primary objective of this task is to evaluate the effect of hydrogen on environment-assisted cracking of candidate target materials for applications in spallationneutron- target (SNT) systems such as accelerator production of tritium (APT) and accelerator transmutation of waste (ATW). The materials selected for evaluation and characterization are martensitic stainless steels including Alloy HT-9, Alloy EP 823 and Type 422 stainless steel. The susceptibility to stress corrosion cracking (SCC) and hydrogen embrittlement (HE) of these materials are being evaluated in aqueous environments of interest using tensile specimens under constant load and slow-strain-rate (SSR) conditions. …

Stress Corrosion Cracking Of Type 422 Stainless Steel For Applications In Spallation-Neutron-Target Systems, Ramprashad Prabhakaran

Transmutation Sciences Materials (TRP)

Introduction

• This research program is aimed at evaluating different types of environment-induced degradation of candidate target materials for applications in transmutation of spent nuclear fuels (SNF).

• Transmutation refers to the elimination of long-lived actinides and fission products from SNF.

Objectives

• Evaluate susceptibility of candidate target materials to stress corrosion cracking (SCC) and localized corrosion (pitting and crevice) in neutral and acidic aqueous environments at ambient and elevated temperatures

• Determine the extent and morphology of cracking in tested materials as functions of experimental and environmental variables including pH, temperature, loading conditions and specimen geometry

• Develop mechanistic …

Environment-Induced Degradation And Crack-Growth Studies Of Candidate Target Materials, Ajit K. Roy, Brendan O'Toole

Transmutation Sciences Materials (TRP)

During the past two years (2001-2002) of this project, the primary effort was focused on evaluating the effect of hydrogen on the cracking behavior of candidate target materials namely, Alloys EP-823, HT-9 and 422 in aqueous environments of different pH values at ambient and elevated temperatures. More recently, emphasis is being placed to evaluate the cracking behavior of these materials in molten lead-bismuth eutectic (LBE) environment at much higher testing temperatures so as to compare the cracking susceptibility in environments containing molten metals and aqueous solutions, respectively. The most recent tests to evaluate the cracking susceptibility were primarily based on …

Environment-Induced Degradation And Crack-Growth Studies Of Candidate Target Materials, Ajit K. Roy, Brendan O'Toole, Zhiyong Wang, David W. Hatchett

Transmutation Sciences Materials (TRP)

The primary objective of this task is to evaluate the potential for the environmentally-assisted cracking of candidate target materials for applications in spallation-neutron-target systems, such as accelerator-driven system for the transmutation of waste. The materials selected for evaluation and characterization are martensitic stainless steels (SS) including Alloys HT- 9, EP 823 and Type 422 stainless steel.

More recently, this experimental program has been expanded to evaluate the effect of molten lead-bismuth eutectic (LBE) on the corrosion behavior of target materials in the presence of oxygen. Since the materials performance laboratory (MPL) at UNLV currently cannot accommodate this type of testing, …

Perturbative And Nonperturbative Calculations Of Electron-Hydrogen Ionization, Stephenie J. Jones, Don H. Madison, Mark D. Baertschy

Physics Faculty Research & Creative Works

We compare calculations of the fully differential cross section for ionization of atomic hydrogen by electron impact using two different theories-the perturbative CDW-EIS (continuum distorted wave with eikonal initial state) approximation and the nonperturbative ECS (exterior complex scaling) method. For this comparison, we chose an impact energy of 54.4 eV, since this is near the lowest energy that our perturbative approach would be applicable and near the highest energy that can be tackled by the ECS method with our present computational resources. For the case of equal-energy outgoing electrons investigated here, the two theories predict nearly identical results except that …

Comparison Between Hydrogen And Dihydrogen Bonds Among H3bnh3, H2bnh2, And Nh3, T. Kar, Steve Scheiner

Chemistry and Biochemistry Faculty Publications

Several possible binary complexes among ammonia-borane, aminoborane, and ammonia, via hydrogen and/or dihydrogen bonds, have been investigated to understand the effect of different hybridization. Møller–Plesset second-order perturbation theory with aug-cc-pVDZ basis set was used. The interaction energy is corrected for basis set superposition error, and the Morokuma–Kitaura method was employed to decompose the total interaction energy. Like H₃BNH₃, the sp² hybridized H₂BNH₂ also participates in H- and dihydrogen bond formation. However, such bonds are weaker than their sp³ analogs. The contractions of BN bonds are associated with blueshift in …

Measurement Of Inclusive Spin Structure Functions Of The Deuteron, J. Yun, S. E. Kuhn, G. E. Dodge, T. A. Forest, M. Bektasoglu, L. Ciciani, C. E. Hyde-Wright, A. Klein, A. V. Klimenko, L. M. Qin, S. Stepanyan, L. B. Weinstein, Et Al., Clas Collaboration

Physics Faculty Publications

We report the results of a new measurement of spin structure functions of the deuteron in the region of moderate momentum transfer [Q² = 0.27-1.3 (GeV/c)²] and final hadronic state mass in the nucleon resonance region (W=1.08-2.0 GeV). We scattered a 2.5 GeV polarized continuous electron beam at Jefferson Lab off a dynamically polarized cryogenic solid state target (¹⁵ND₃) and detected the scattered electrons with the CEBAF large acceptance spectrometer. From our data, we extract the longitudinal double spin asymmetry A∥ and the spin structure function g₁^d. Our data are …