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Articles 1 - 30 of 55
Full-Text Articles in Physical Sciences and Mathematics
Orbital Structure Of Fetio3 Ilmenite Investigated With Polarization-Dependent X-Ray Absorption Spectroscopy And Band Structure Calculations, S W. Chen, M J. Huang, P A. Lin, H T. Jeng, J M. Lee, S C. Haw, S A. Chen, H J. Lin, K T. Lu, Dapeng Chen, S X. Dou, X L. Wang, J M. Chen
Orbital Structure Of Fetio3 Ilmenite Investigated With Polarization-Dependent X-Ray Absorption Spectroscopy And Band Structure Calculations, S W. Chen, M J. Huang, P A. Lin, H T. Jeng, J M. Lee, S C. Haw, S A. Chen, H J. Lin, K T. Lu, Dapeng Chen, S X. Dou, X L. Wang, J M. Chen
Shi Xue Dou
We explored the orbital structure of FeTiO3 with polarization-dependent x-ray absorption spectra complemented with electronic structure calculations. The electronic structure, near the bottom of conduction band, is composed of O 2p and Ti 3d orbitals. Ti 3d/4p hybridization dominantly lies on the ab plane. The highly delocalized Ti 4p orbital might hybridize with O 2p orbital and even extend to the next-neighbor Fe atom whereby establishing a linear orbital combination of Ti-O-Fe. A clear picture of the orbital construction in FeTiO3 will help to elucidate the paths of pressure-induced charge transfer and other physical or magnetic characteristics.
Magnetic Properties Of Bi2femno6: A Multiferroic Material With Double-Perovskite Structure, Yi Du, Zhenxiang Cheng, S X. Dou, Xiaolin Wang, Hua Zhao, Hideo Kimura
Magnetic Properties Of Bi2femno6: A Multiferroic Material With Double-Perovskite Structure, Yi Du, Zhenxiang Cheng, S X. Dou, Xiaolin Wang, Hua Zhao, Hideo Kimura
Shi Xue Dou
Single phase Bi2FeMnO6 was synthesized on Si substrates by an electrospray method. Three peaks were observed in the temperature dependence of magnetization curve, which is attributed to the inhomogeneous distribution of Fe3+ and Mn3+. The observed magnetic peaks at 150 K, 260 K, and 440 K correspond to orderings of the ferrimagnetic Fe–O–Mn, and antiferromagnetic Mn–O–Mn and Fe–O–Fe, respectively. Heat capacity measurements were carried out to confirm these magnetic transitions. The Debye temperature of Bi2FeMnO6 is 339 K, calculated from Debye–Einstein fitting.
The Effects Of Annealing Temperature On The In-Field Jc And Surface Pinning In Silicone Oil Doped Mgb2 Bulks And Wires, M S. Hossain, A Motaman, O Cicek, H Agil, E Ertekin, A Gencer, Xiaolin Wang, S X. Dou
The Effects Of Annealing Temperature On The In-Field Jc And Surface Pinning In Silicone Oil Doped Mgb2 Bulks And Wires, M S. Hossain, A Motaman, O Cicek, H Agil, E Ertekin, A Gencer, Xiaolin Wang, S X. Dou
Shi Xue Dou
No abstract provided.
Apparent Negative Mobility Of Vortex Matter Due To Inhomogeneous Pinning, X B Xu, H Fangohr, Shichao Ding, M Gu, T.B Tang, Z Han, Dongqi Shi, S X. Dou
Apparent Negative Mobility Of Vortex Matter Due To Inhomogeneous Pinning, X B Xu, H Fangohr, Shichao Ding, M Gu, T.B Tang, Z Han, Dongqi Shi, S X. Dou
Shi Xue Dou
We investigate the transport of vortices in superconductors with inhomogeneous pinning under a driving force. The inhomogeneity of pinning is simplified as strong-weak pinning regions. It is demonstrated that the interactions between the vortices captured by strong pinning potentials and the vortices in the weak pinning region cause absolute negative motion (ANM) of vortices: The vortices which are climbing toward the high barriers induced by the strong pinning with the help of driving force move toward the opposite direction of the force and back to their equilibrium positions in the weak pinning region as the force decreases or is withdrawn. …
Inhomogeneities In Yba 2cu 3o 7 Thin Films With Reduced Thickness, O V. Shcherbakova, A V. Pan, S K. Gorman, S A. Fedoseev, I A. Golovchanskiy, S. X. Dou
Inhomogeneities In Yba 2cu 3o 7 Thin Films With Reduced Thickness, O V. Shcherbakova, A V. Pan, S K. Gorman, S A. Fedoseev, I A. Golovchanskiy, S. X. Dou
Shi Xue Dou
Morphology and physical properties of mono- (YBa2Cu3O7) and multilayered (YBa2Cu3O7/SmBa2Cu3O7/ YBa2Cu3O7) superconducting thin films with thickness ranging from 90 nm to 28 nm have been investigated. For both types of samples, the superconducting properties degraded with reduction of film thickness. Structural and electromagnetic properties were visualized through scanning electron microscopy and magneto-optical imaging, respectively, and revealed high level of inhomogeneity for thinner (<58 >nm) samples. However, samples with thickness above 58 nm showed enhanced homogeneity, which …
Flux Distribution In Fe-Based Superconducting Materials By Magneto-Optical Imaging, Zhi Wei Lin, Jian Guo Zhu, You Guang Guo, Xiaolin Wang, S X. Dou, Tom H. Johansen, Xun Shi, K Y. Choi
Flux Distribution In Fe-Based Superconducting Materials By Magneto-Optical Imaging, Zhi Wei Lin, Jian Guo Zhu, You Guang Guo, Xiaolin Wang, S X. Dou, Tom H. Johansen, Xun Shi, K Y. Choi
Shi Xue Dou
"This paper presents the magnetic flux distributions in Fe-based superconducting materials including single crystal of Ba(Fe1.9Ni0.1)As2 and Ba(Fe1.8Co0.2)As2, as well as polycrystalline SmFeO0.75F0.2As by means of magneto-optical imaging (MOI) technique. The single crystals were grown out of FeAs flux while polycrystalline sample was grown by hot-press. A MOI film with in-plan magnetization was used to visualize flux distributions at the sample surface. A series of magneto-optical images was taken when the samples were zero-field cooled and field cooled. The flux behavior, including penetration into and expelling from the samples, as well as pinning properties were studied. When external fields increase, …
Anisotropic And Excellent Magnetocaloric Properties Of La 0.7ca0.3mno3 Single Crystal With Anomalous Magnetization, J.C Debnath, Rong Zeng, Jung Ho Kim, Dapeng Chen, S X. Dou
Anisotropic And Excellent Magnetocaloric Properties Of La 0.7ca0.3mno3 Single Crystal With Anomalous Magnetization, J.C Debnath, Rong Zeng, Jung Ho Kim, Dapeng Chen, S X. Dou
Shi Xue Dou
Magnetic properties and the magnetocaloric effect (MCE) have been investigated in La0.7Ca0.3MnO3 single crystal with applied field along both the ab-plane and the c-direction. Due to the magnetocrystalline anisotropy, the crystal exhibits anisotropy in the MCE. Upon application of a 5 T field, the magnetic entropy changes (SM), reaching values of 7.668 J/(kg K) and 6.412 J/(kg K) for both the ab-plane and the c-direction, respectively. A magnetic entropy change of 3.3 J/(kg K) was achieved for a magnetic field change of 1.5 T at the Curie temperature, TC = 245 K. Due to the absence of grains in the …
Lanthanum Doped Multiferroic Dyfeo3: Structural And Magnetic Properties, Yi Du, Zhenxiang Cheng, Xiaolin Wang, S X. Dou
Lanthanum Doped Multiferroic Dyfeo3: Structural And Magnetic Properties, Yi Du, Zhenxiang Cheng, Xiaolin Wang, S X. Dou
Shi Xue Dou
Lanthanum doped multiferroic DyFeO3 was synthesized by solid state reaction. X-ray diffraction and refinement show that the lattice parameters of Dy1−xLaxFeO3 increase linearly with the La content. Raman spectroscopy reveals that the short-range force constant in Dy1−xLaxFeO3 is decreased by La3+ ion substitution. The spin reorientation phase transition temperature (TSRPT) is observed to decrease along with the doping level. The antiferromagnetic ordering temperature TN of Fe3+ ions is depressed with increasing doping level. Both decreasing TSRPT and decreasing TN indicate that Fe–Dy and Fe–Fe interactions are weakened by La substitution. It is found that the electron configuration of Fe3+ is …
The Control Of Time-Dependent Buckling Patterns In Thin Confined Elastomer Film, Brad Winton, Mihail Ionescu, S X. Dou
The Control Of Time-Dependent Buckling Patterns In Thin Confined Elastomer Film, Brad Winton, Mihail Ionescu, S X. Dou
Shi Xue Dou
Low energy metal ion implantation has been used to combine an easy “bottom-up” way of creating and tuning different topographic structures on submicron to micrometer scales with the embedding of a metallic element-rich functionalized layer at the surface for a variety of scientific and technological applications. The self-organizing and complex patterns of functionalized topographic structures are highly dependent on the implanted metal ion species, variations in the geometric confinement of the buckled areas on the larger unmodified elastomer film, and the boundary conditions of the buckled regions. Systematic investigations of these dependencies have been carried out via optical and atomic …
In-Field Jc Improvement By Oxygen-Free Pyrene Gas Diffusion Into Highly Dense Mgb2 Superconductor, Minoru Maeda, Jung Ho Kim, Y Zhao, Yoon-Uk Heo, K Takase, Y Kubota, C Moriyoshi, F Yoshida, Y Kuroiwa, S X. Dou
In-Field Jc Improvement By Oxygen-Free Pyrene Gas Diffusion Into Highly Dense Mgb2 Superconductor, Minoru Maeda, Jung Ho Kim, Y Zhao, Yoon-Uk Heo, K Takase, Y Kubota, C Moriyoshi, F Yoshida, Y Kuroiwa, S X. Dou
Shi Xue Dou
Oxygen-free pyrene gas as a carbon (C) dopant was delinked and incorporated into highly dense MgB2 structure via a gas phase diffusion method. The technique offers the advantages that molecular C is homogeneously distributed into MgB2 and substituted at the boron sites without any severe deterioration of grain connectivity. The C substitution causes a significant shrinkage of the a-lattice parameter and an increase in the lattice strain, resulting in high disorder. The introduction of structural disorder as a result of C doping leads to a considerable enhancement of the in-field critical current density (Jc) and upper critical field.
Correlation Between Structural Parameters And The Magnetocaloric Effect In Epitaxial La0.8ca0.2mno3/Laalo3 Thin Film, J C. Debnath, J H. Kim, Y Heo, A M. Strydom, S X. Dou
Correlation Between Structural Parameters And The Magnetocaloric Effect In Epitaxial La0.8ca0.2mno3/Laalo3 Thin Film, J C. Debnath, J H. Kim, Y Heo, A M. Strydom, S X. Dou
Shi Xue Dou
An epitaxial La0.8Ca0.2MnO3/LaAlO 3 (LCMO/LAO) thin film was fabricated using the pulsed laser deposition technique to evaluate the correlation between the crystal structure and the magnetocaloric effect. In our study, the LCMO film was 200 nm in thickness and appeared to have a strong out-of plane texture. We found that each column in the LCMO thin film layer is a domain which has a different ordering direction. These microscopic feature results in anisotropic properties of magnetization, entropy, and relative cooling power. The film exhibited a paramagnetic-to-ferromagnetic second order phase transition at 249 K. The lack of any hysteresis loss also …
The Mechanical And The Electrical Properties Of Conducting Polypyrrole Fibers, Javad Foroughi, Shaban R. Ghorbani, Germanas Peleckis, Geoffrey M. Spinks, Gordon G. Wallace, Xiaolin Wang, S X. Dou
The Mechanical And The Electrical Properties Of Conducting Polypyrrole Fibers, Javad Foroughi, Shaban R. Ghorbani, Germanas Peleckis, Geoffrey M. Spinks, Gordon G. Wallace, Xiaolin Wang, S X. Dou
Shi Xue Dou
The mechanical and the electrical properties of polypyrrole (PPy) fibers and electrochemically deposited PPy films were studied. It was found that the PPy fibers showed a significantly higher strength than the PPy films due to better orientation of the molecular structure. The electrochemically prepared PPy films had a higher electrical conductivity than that of the fibers at high temperature. At low temperature, the PPy fibers showed the higher conductivity. The conductivity results were analyzed in the frame of the three-dimensional variable range hopping model. The results showed that at room temperature the average hopping distance for the fibers was about …
Comparison Of Small-Field Behaviour In Mgb2, Low And High Temperature Superconductors, Alexey V. Pan, S X. Dou
Comparison Of Small-Field Behaviour In Mgb2, Low And High Temperature Superconductors, Alexey V. Pan, S X. Dou
Shi Xue Dou
Different types of superconductors have been investigated at small magnetic fields (Ba) over wide temperature (T) ranges at different Ba orientations. It has been shown that the temperature dependence of the characteristic field (B*), separating the Ba-independent critical current density (Jc) plateau (single vortex pinning regime) and the region with Jc(Ba) (collective pinning), can be attributed either to the temperature dependence of the magnetic penetration depth for Nb-film and MgB2bulk superconductors, or to thermally activated processes for Bi-based superconductors and YBa2Cu3O7−δ superconducting films. In both cases the vortex pinning influence appears to have a secondary role, affecting the effective vortex …
Reduction Of Superconducting Transition Temperature And Flux Pinning In Al And C Codoped Mgb2 With Insight From First-Principles Calculations, Aihua Li, Xiaolin Wang, S X. Dou, Qiwen Yao, Zhenxiang Cheng, Saeid Soltanian, J M. Yoo, P Munroe
Reduction Of Superconducting Transition Temperature And Flux Pinning In Al And C Codoped Mgb2 With Insight From First-Principles Calculations, Aihua Li, Xiaolin Wang, S X. Dou, Qiwen Yao, Zhenxiang Cheng, Saeid Soltanian, J M. Yoo, P Munroe
Shi Xue Dou
We report for the first time the Al and C codoping effect on the structures and superconductivity in MgB2. It was found that both the lattice parameters and the Tc decreased monotonically with increasing doping level of both Al and C. The Tc dropped to 27.5 and 7 K for x=0.2 and for x =0.4, respectively. The reduction of Tc for the codoping was found to be quicker than for individual Al doping and slower than for individual C doping at the same doping levels. First-principles calculations indicated that the observed decrease in Tc …
Investigation Of The Critical Behavior In Mn0.94nb 0.06coge Alloy By Using The Field Dependence Of Magnetic Entropy Change, J C. Debnath, P Shamba, A M. Strydom, Jianli Wang, S X. Dou
Investigation Of The Critical Behavior In Mn0.94nb 0.06coge Alloy By Using The Field Dependence Of Magnetic Entropy Change, J C. Debnath, P Shamba, A M. Strydom, Jianli Wang, S X. Dou
Shi Xue Dou
The critical behaviour of Mn0.94Nb0.06CoGe alloy around the paramagnetic-ferromagnetic phase transition was studied based on the field dependence on magnetic entropy change. By using the obtained exponents, the modified Arrott plot is consistent with that by using conventional method. These critical exponents are confirmed by the Widom scaling relation. Based on these critical exponents, the magnetization, field and temperature data around Tc collapse into two curves obeying the single scaling equation MðH; e)¼ebf6(H/ebþc). The calculated critical exponents not only obey the scaling theory but also anastomose the deduced results from the Kouvel-Fisher method [J. S. Kouvel and M. E. Fisher, …
Effect Of Frozen Spin On The Magnetocaloric Property Of La0.7ca0.3coo3 Polycrystalline And Single Crystal Samples, J C. Debnath, R Zeng, J H. Kim, P Shamba, Dapeng Chen, S X. Dou
Effect Of Frozen Spin On The Magnetocaloric Property Of La0.7ca0.3coo3 Polycrystalline And Single Crystal Samples, J C. Debnath, R Zeng, J H. Kim, P Shamba, Dapeng Chen, S X. Dou
Shi Xue Dou
Polycrystalline (PC) and single crystalline (SC) samples of La0.7Ca0.3CoO3 (LCCO) with the perovskite structure were synthesized by conventional solid-state reaction and the floating-zone growth method. We conducted isothermal magnetization measurements of the PC and SC samples at temperatures from 2.8 K to 140 K, and evaluated the magnetic entropy change (−ΔSM) under zero field cooling (ZFC) and field cooling (FC) to 2.8 K. An interesting result has been obtained, where the −ΔSM–T curves in the low temperature range show totally different features between the ZFC and FC cooling procedures. The −ΔSM shows a large inverse irreversibility value for the ZFC …
Magnetic And Superconducting Properties Of Spin-Fluctuation-Limited Superconducting Nanoscale Vnx, R Zeng, J Liu, G Du, W. X. Li, J Wang, J Horvat, S X. Dou
Magnetic And Superconducting Properties Of Spin-Fluctuation-Limited Superconducting Nanoscale Vnx, R Zeng, J Liu, G Du, W. X. Li, J Wang, J Horvat, S X. Dou
Shi Xue Dou
"VNx nanoparticles and nanowires have been prepared by nitrifying V2O5 nanoparticles (NP) and nanowires (NW). The V2O5 NP and NW were synthesized by a facile hydrothermal method. Magnetic susceptibility (chi) and magnetization measurements showed long range superconducting ordering (LRSO) at the temperature of 5.8 K for NW, but there was no observation of LRSO (at least down to 2 K) for the NP sample, which is a much lower temperature than for the corresponding bulk, while both NP and NW showed the absence of long range magnetic ordering, at least down to 2 K. However, the chi data showed that …
La And Nb Codoped Bifeo3 Multiferroic Thin Films On Lanio3/Si And Iro2/Si Substrates, Zhenxiang Cheng, Xiaolin Wang, Hideo Kimura, Kiyoshi Ozawa, S X. Dou
La And Nb Codoped Bifeo3 Multiferroic Thin Films On Lanio3/Si And Iro2/Si Substrates, Zhenxiang Cheng, Xiaolin Wang, Hideo Kimura, Kiyoshi Ozawa, S X. Dou
Shi Xue Dou
Nb and La codoped BiFeO3 thin films were fabricated on oxide bottom electrodes, LaNiO3/Si and IrO2/Si, by pulsed laser deposition method. The doped BiFeO3 thin film capacitor on LaNiO3showed a remnant polarization of more than 75 µC/cm2 in a saturated hysteresis loop. The same La and Nb codoped BiFeO3 thin film capacitors on IrO2 showed a larger remnant polarization, while with a significant contribution from the leakage current. Furthermore, the doped BiFeO3 capacitor on the LaNiO3 bottom electrode showed worse fatigue resistance than the film on IrO2. All the doped BiFeO3 thin films showed weak ferromagnetism at room temperature.
Magnetic Phase Transition In Mnfep0.5as0.4si 0.1, Jianli Wang, Stewart J. Campbell, O Tegus, E Bruck, S X. Dou
Magnetic Phase Transition In Mnfep0.5as0.4si 0.1, Jianli Wang, Stewart J. Campbell, O Tegus, E Bruck, S X. Dou
Shi Xue Dou
We have carried out a detailed investigation of the magnetic phase transition in MnFeP0.5As0.4Si0.1. Temperature hysteresis has been observed in the variable temperature magnetization curves (Bappl = 0.01 T) with TC W ~ 302 K on warming and TC C ~ 292 K on cooling. The first order nature of this transition in MnFeP0.5As0.4Si0.1 is confirmed by the negative slope obtained from isotherms of M2 versus B/M around the critical temperature. Linear thermal expansion measurements reveal a large volume change, ΔV/V∼8.7×10-3, at the magnetic phase transition and that this magnetovolume effect is suppressed to ΔV/V ∼ 5.5×10-3 in an applied …
Superconducting Properties Of Carbonaceous Chemical Doped Mgb2, Wenxian Li, S X. Dou
Superconducting Properties Of Carbonaceous Chemical Doped Mgb2, Wenxian Li, S X. Dou
Shi Xue Dou
The discovery of superconductivity in magnesium diboride (MgB2: 39 K, in January 2001) (Nagamatsu et al., 2001) has generated enormous interest and excitement in the superconductivity community and the world in general, but especially among researchers into superconductivity in non-oxide and boron related compounds.
Single-Crystal Growth And Anisotropic Magnetic Properties Of Nonstoichiometric Three-Layer Sodium Cobalt Oxides, Dapeng Chen, Xiaolin Wang, C T Lin, S X. Dou
Single-Crystal Growth And Anisotropic Magnetic Properties Of Nonstoichiometric Three-Layer Sodium Cobalt Oxides, Dapeng Chen, Xiaolin Wang, C T Lin, S X. Dou
Shi Xue Dou
Large single crystals of α-NaxCoO2 (x=0.91, 0.92, and 0.93) have been successfully fabricated by using the traveling solvent floating zone method. Details on the crystal growth are discussed. The crystal structures were characterized using powder x-ray diffraction and Rietveld refinement. The magnetic susceptibility measurements show that the magnetic properties depend strongly on x. The compound was found to be antiferromagnetic at TN ≈ 20 K for x=0.91 and x=0.92, and paramagnetic for x=0.93. The in-plane and out-of-plane anisotropies were observed for the x=0.91 crystals. In addition, the derived anisotropic g-factor ratios (gab /gc) from the anisotropic susceptibility along H||ab and …
Microscopic Role Of Carbon On Mgb2 Wire For Critical Current Density Comparable To Nbti, Jung Ho Kim, Sangjun Oh, Yoon-Uk Heo, Satoshi Hata, Hiroaki Kumakura, Akiyoshi Matsumoto, Masatoshi Mitsuhara, Seyong Choi, Yusuke Shimada, Minoru Maeda, Judith Macmanus-Driscoll, S X. Dou
Microscopic Role Of Carbon On Mgb2 Wire For Critical Current Density Comparable To Nbti, Jung Ho Kim, Sangjun Oh, Yoon-Uk Heo, Satoshi Hata, Hiroaki Kumakura, Akiyoshi Matsumoto, Masatoshi Mitsuhara, Seyong Choi, Yusuke Shimada, Minoru Maeda, Judith Macmanus-Driscoll, S X. Dou
Shi Xue Dou
Increasing dissipation-free supercurrent has been the primary issue for practical application of superconducting wires. For magnesium diboride, MgB2, carbon is known to be the most effective dopant to enhance high-field properties. However, the critical role of carbon remains elusive, and also low-field critical current density has not been improved. Here, we have undertaken malic acid doping of MgB2 and find that the microscopic origin for the enhancement of high-field properties is due to boron vacancies and associated stacking faults, as observed by high-resolution transmission electron microscopy and electron energy loss spectroscopy. The carbon from the malic acid almost uniformly encapsulates …
Correlation Between Doping Induced Disorder And Superconducting Properties In Carbohydrate Doped Mgb2, Jung Ho Kim, S X. Dou, Sangjun Oh, M Jercinovic, E Babic, T Nakane, Hiroaki Kumakura
Correlation Between Doping Induced Disorder And Superconducting Properties In Carbohydrate Doped Mgb2, Jung Ho Kim, S X. Dou, Sangjun Oh, M Jercinovic, E Babic, T Nakane, Hiroaki Kumakura
Shi Xue Dou
A comprehensive study of the effects of carbohydrate doping on the superconductivity of MgB2 has been conducted. In accordance with the dual reaction model, more carbon substitution is achieved at lower sintering temperature. As the sintering temperature is lowered, lattice disorder is increased. Disorder is an important factor determining the transition temperature for the samples studied in this work, as evidenced from the correlations among the lattice strain, the resistivity, and the transition temperature. It is further shown that the increased critical current density in the high field region can be understood by a recently-proposed percolation model [M. Eisterer et …
A Sign Of Field-Induced First Order Magnetic State Transition And Giant Reversible Magnetocaloric Effect In Cobalt Hydroxide Nanosheets, Precious Shamba, Rong Zeng, J Q Wang, S X. Dou
A Sign Of Field-Induced First Order Magnetic State Transition And Giant Reversible Magnetocaloric Effect In Cobalt Hydroxide Nanosheets, Precious Shamba, Rong Zeng, J Q Wang, S X. Dou
Shi Xue Dou
We report the synthesis of β−Co(OH)2 nanosheets using microwave assisted hydrothermal and conventional chemical reaction methods. A magnetic transition at an onset temperature, T1 ~ 96 K, and a sign of antiferromagnetic state transition at the Néel temperature, TN=9~10 K, can be determined from M-T curves and M-H curves magnetic properties investigation. It is found that a sign of field-induced first order transition below 9 K, act as a role of reversing the magnetocaloric effect from negative to positive value. The large reversible magnetic-entropy change (∆SM) of 17 J/kg K around 11 K for a field change of 5 T …
Ferroelectric And Ferromagnetic Nanofibers: Synthesis, Properties And Applications, A Jalalian, A M. Grishin, S X. Dou
Ferroelectric And Ferromagnetic Nanofibers: Synthesis, Properties And Applications, A Jalalian, A M. Grishin, S X. Dou
Shi Xue Dou
As first time, ferroelectric (Ba0.85Ca0.15)(Ti0.9Zr0.1)O3 (BCTZ), biocompatible (Na0.5K0.5)NbO3 (NKN), and ferromagnetic Y3Fe5O12 (YIG) nanofibers were synthesized by sol-gel assisted electrospining technique. Non-woven, bead-free 100 μm long fiber mat was formed from close-packed nanocrystals after calcination in air at 800°C (BCTZ and NKN) and 1100°C (YIG). BCTZ fibers are 200 nm in width whereas NKN and YIG fibers have smaller 50-100 nm diameter. X-ray diffraction and Raman spectroscopy show that BCTZ and NKN crystallized in tetragonal and rhombohedral polar phases in the vicinity of morphotropic phase boundary. Room temperature ferromagnetism in YIG fibers is indicated by a well formed M-H hysteresis …
Magnetocapacitance Effect In Nonmultiferroic Yfe03 Single Crystal, Z X. Cheng, H Shen, J Xu, Peng Liu, S J. Zhang, Jianli Wang, Xiaolin Wang, S X. Dou
Magnetocapacitance Effect In Nonmultiferroic Yfe03 Single Crystal, Z X. Cheng, H Shen, J Xu, Peng Liu, S J. Zhang, Jianli Wang, Xiaolin Wang, S X. Dou
Shi Xue Dou
YFeO3 single crystal displays two relaxor-like dielectric relaxations, one at low temperature (170300 K) and one at high temperature (370520 K), which are attributed to the activation of electrons and oxygen vacancies, respectively. Above the temperature at which electrons are activated, the sample displays a large magnetocapacitance effect. Comparison of the impedance Cole-Cole plots measured with and without applied magnetic field reveals that the occurrence of magnetocapacitance effect is accompanied with an increasing in DC conductivity under magnetic field after the activation of electrons, which is explained by the enhancement of electron jumping in Fe2b-O-Fe3b chains by magnetic field. Thus …
Structure, Ferroelectric Properties, And Magnetic Properties Of The La-Doped Bismuth Ferrite, Zhenxiang Cheng, Aihua Li, Xiaolin Wang, S X. Dou, Kiyoshi Ozawa, Hideo Kimura, S Zhang, Thomas R. Shrout
Structure, Ferroelectric Properties, And Magnetic Properties Of The La-Doped Bismuth Ferrite, Zhenxiang Cheng, Aihua Li, Xiaolin Wang, S X. Dou, Kiyoshi Ozawa, Hideo Kimura, S Zhang, Thomas R. Shrout
Shi Xue Dou
Bi1-xLaxFeO3 ceramics with x=0, 0.1, 0.2, and 0.3 have been synthesized by solid state reaction, starting from metal oxides. A series of structure transformations is found to depend upon the doping level. Below 10% La doping, Bi1-xLaxFeO3 maintains the rhombohedral structure of BiFeO3. However, for Bi0.8La0.2FeO3 and Bi0.7La0.3FeO3, the structures change to the orthorhombic and tetragonal, respectively. La doping significantly reduces electric leakage and leads to successful observation of electrical polarization hysteresis loops. Doping with La also enhances the ferromagnetic moment, due to the broken cycloid spin structure caused by the changes in the crystalline structure.
Structure, Magnetic, And Thermal Properties Of Nd1-Xlaxcro3 (0 ≤ X ≤ 1.0), Yi Du, Zhenxiang Cheng, Xiaolin Wang, S X. Dou
Structure, Magnetic, And Thermal Properties Of Nd1-Xlaxcro3 (0 ≤ X ≤ 1.0), Yi Du, Zhenxiang Cheng, Xiaolin Wang, S X. Dou
Shi Xue Dou
Perovskite-type Nd1−xLaxCrO3(0 ≤ x ≤1.0) polycrystalline samples were synthesized using solid state reaction. Structural studies indicate that the lattice parameters, metal–oxygen bond lengths, and angles of Nd1−xLaxCrO3 strongly depend on the La content. Two magnetic transition temperatures, Cr3+ antiferromagnetic ordering temperature (TN) and the spin reorientation phase transition temperature (TSRPT), have been observed in the M-T curves. The increase in TN and decrease in TSRPT with increasing x value can be explained by the change in the magnetic interactions due to La doping. The heat capacity of Nd1−xLaxCrO3 measured from 2 to 300 K reveals that the lattice, electronic, and …
Morphology-Controllable 1d-3d Nanostructured Tio2 Bilayer Photoanodes For Dye-Sensitized Solar Cells, Ziqi Sun, Jung Ho Kim, Yue Zhao, Darren Attard, S X. Dou
Morphology-Controllable 1d-3d Nanostructured Tio2 Bilayer Photoanodes For Dye-Sensitized Solar Cells, Ziqi Sun, Jung Ho Kim, Yue Zhao, Darren Attard, S X. Dou
Shi Xue Dou
Morphology-controlled bilayer TiO2 nanostructures consisting of one-dimensional (1D) nanowire bottom arrays and a three-dimensional (3D) dendritic microsphere top layer were synthesized via a one-step hydrothermal method. These novel 1D-3D bilayer photoanodes demonstrated the highest energy conversion efficiency of 7.2% for rutile TiO2 dye-sensitized solar cells to date, with TiCl4 post-treatment.
Nano-Structured Sno2-Carbon Composites Obtained By In Situ Spray Pyrolysis Method As Anodes In Lithium Batteries, Ling Yuan, Konstantin Konstantinov, Guoxiu Wang, Hua-Kun Liu, S X. Dou
Nano-Structured Sno2-Carbon Composites Obtained By In Situ Spray Pyrolysis Method As Anodes In Lithium Batteries, Ling Yuan, Konstantin Konstantinov, Guoxiu Wang, Hua-Kun Liu, S X. Dou
Shi Xue Dou
In this paper, we report on a series of SnO2-carbon nano-composites synthesized by in situ spray pyrolysis of a solution of SnCl2·2H2O and sucrose at 700 °C. The process results in super fine nanocrystalline SnO2, which is homogeneously distributed inside the amorphous carbon matrix. The SnO2 was revealed as a structure of broken hollow spheres with porosity on both the inside and outside particle surfaces. This structure promises a highly developed specific surface area. X-ray diffraction (XRD) patterns and transmission electron microscope (TEM) images revealed the SnO2 crystal size is about 5–15 nm. These composites show a reversible lithium storage …