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Full-Text Articles in Physical Sciences and Mathematics
The Generation Of Terahertz Light And Its Applications In The Study Of Vibrational Motion, Aldair Alejandro
The Generation Of Terahertz Light And Its Applications In The Study Of Vibrational Motion, Aldair Alejandro
Theses and Dissertations
Terahertz (THz) spectroscopy is a powerful tool that uses ultrashort pulses of light to study the properties of materials on picosecond time scales. THz light can be generated through a variety of methods. In our lab, we generate THz through the process of optical rectification in nonlinear optical (NLO) organic crystals. THz light can be used to study several phenomena in materials, such as spin precession, electron acceleration, vibrational and rotational motion. The work presented in this dissertation is divided into two parts: (1) the generation of THz light and (2) applications of THz light. The first portion of this …
Nonlinear Ultrafast Excitation And Two-Dimensional Terahertz Spectroscopy Of Solids, Brittany E. Knighton
Nonlinear Ultrafast Excitation And Two-Dimensional Terahertz Spectroscopy Of Solids, Brittany E. Knighton
Theses and Dissertations
Ultrafast spectroscopy allows us to probe and understand material properties. With it, we can measure phonon-polaritons (optical phonons coupled with light) and the resulting dispersion curve in lithium niobate. Customizing the excitation source in ultrafast measurements can excite phonon modes to large amplitudes, allowing the experimental exploration of the Potential Energy Surface in solids. However, stronger pump fluences and bigger signal isn't always the answer in ultrafast spectroscopy. When sample signals and their nonlinear and mechanisms cannot be distinguished with 1D measurements, simple 2D THz measurements are a great place to start searching for distinct factors as was the case …