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Full-Text Articles in Physical Sciences and Mathematics
Applications Of Voltammetric Ion Selective Electrodes To Complex Matrices, Alexander R. Harris, Jie Zhang, Robert W. Cattrall, Alan M. Bond
Applications Of Voltammetric Ion Selective Electrodes To Complex Matrices, Alexander R. Harris, Jie Zhang, Robert W. Cattrall, Alan M. Bond
Australian Institute for Innovative Materials - Papers
The practical application of two different voltammetric ion selective electrodes (VISE) to measure ion activity in complex solutions has been explored. 7,7,8,8-tetracyanoquinodimethane (TCNQ) and tetrathiafulvalene (TTF) microcrystals adhered to an electrode surface act as a low selectivity voltammetric ion sensor. Resistance drop effects and pH artifacts were minimised by the addition of an "innocent" supporting electrolyte (buffer) to the analyte solution. In this format, addition of an ionophore to improve selectivity resulted in a reduction in current magnitude, due to competition for the ion. In contrast, voltammetry of a thin film containing a redox active species, electrolyte, ionophore and membrane …
A Preliminary Investigation Of Complex Adaptive Systems As A Model For Explaining Organisational Change Caused By The Introduction Of Health Information Systems, Kieren Diment, Ping Yu, Karin Garrety
A Preliminary Investigation Of Complex Adaptive Systems As A Model For Explaining Organisational Change Caused By The Introduction Of Health Information Systems, Kieren Diment, Ping Yu, Karin Garrety
Faculty of Informatics - Papers (Archive)
This paper documents the preliminary development of a framework for evaluating organisational change processes during the implementation of an electronic nursing documentation system in residential aged care facilities. It starts with a brief outline of organisational change processes. This is followed by a more detailed exposition of the principles underlying complex adaptive systems (CAS) theory, where we explain how mathematical concepts can be used to illuminate qualitative research approaches. Finally we present some preliminary findings on the facilitators and barriers for the introduction of the electronic documentation system, explained with reference to the CAS theory, based on analysis of interviews …
Supporting Developers In Complex Systems Modelling, Antonio A. Lopez-Lorca, Ghassan Beydoun, Rodrigo Martinez-Bejar, Holly Tootell
Supporting Developers In Complex Systems Modelling, Antonio A. Lopez-Lorca, Ghassan Beydoun, Rodrigo Martinez-Bejar, Holly Tootell
Faculty of Informatics - Papers (Archive)
Development of complex systems often requires building a large number of models with many interconnections and dependencies among them. The success of a project can be compromised by cognitive overload or limits of developers, who might miss relationships between elements of the models. Developing Multi-Agent Systems (MAS) is a typical example of where this may occur. Despite of its potential, this technology has not yet been widely adopted by industry due to its complexity and frequent errors in modelling activities. These errors typically propagate to later phases of the MAS development lifecycle, becoming costlier to fix and then lowering the …
Rotationally Resolved Infrared Spectrum Of The Na+-D2 Complex: An Experimental And Theoretical Study, Berwyck L. Poad, V Dryza, J Klos, A A. Buchachenko, E J. Bieske
Rotationally Resolved Infrared Spectrum Of The Na+-D2 Complex: An Experimental And Theoretical Study, Berwyck L. Poad, V Dryza, J Klos, A A. Buchachenko, E J. Bieske
Faculty of Science - Papers (Archive)
The infrared spectrum of mass-selected Na+-D2 complexes is recorded in the D-D stretch vibration region (2915-2972 cm−1) by detecting Na+ photofragments resulting from photo-excitation of the complexes. Analysis of the rotationally resolved spectrum confirms a T-shaped equilibrium geometry for the complex and a vibrationally averaged intermolecular bond length of 2.461 Å. The D-D stretch band centre occurs at 2944.04 cm−1, representing a −49.6 cm−1 shift from the Q1(0) transition of the free D2 molecule. Variational rovibrational energy level calculations are performed for Na+-D2 utilising an ab initio potential energy surface developed previously for investigating the Na+-H2 complex [B. L. J. …
The Molecular Level Modification Of Surfaces: From Self-Assembled Monolayers To Complex Molecular Assemblies, J Justin Gooding, Simone Ciampi
The Molecular Level Modification Of Surfaces: From Self-Assembled Monolayers To Complex Molecular Assemblies, J Justin Gooding, Simone Ciampi
Australian Institute for Innovative Materials - Papers
The modification of surfaces with self-assembled monolayers (SAMs) containing multiple different molecules, or containing molecules with multiple different functional components, or both, has become increasingly popular over the last two decades. This explosion of interest is primarily related to the ability to control the modification of interfaces with something approaching molecular level control and to the ability to characterise the molecular constructs by which the surface is modified. Over this time the level of sophistication of molecular constructs, and the level of knowledge related to how to fabricate molecular constructs on surfaces have advanced enormously. This critical review aims to …
Li2b12h12·7nh3: A New Ammine Complex For Ammonia Storage Or Indirect Hydrogen Storage, Zhenguo Huang, Judith C. Gallucci, Xuenian Chen, Teshome B. Yisgedu, Hima Kumar Lingam, Sheldon G. Shore, Ji-Cheng Zhao
Li2b12h12·7nh3: A New Ammine Complex For Ammonia Storage Or Indirect Hydrogen Storage, Zhenguo Huang, Judith C. Gallucci, Xuenian Chen, Teshome B. Yisgedu, Hima Kumar Lingam, Sheldon G. Shore, Ji-Cheng Zhao
Australian Institute for Innovative Materials - Papers
A new ammine complex, Li2B12H12$7NH3, that can reversibly release all the NH3 at below 200oC and reabsorb NH3 at room temperature and 0.5 bar was synthesized and investigated for reversible ammonia storage or indirect hydrogen storage.
Lead-Free Potassium Bismuth Titanate Thin Film With Complex Aurivillius Layer Structure, Zhenxiang Cheng, Xiaolin Wang, Hongyang Zhao, Hideo Kimura
Lead-Free Potassium Bismuth Titanate Thin Film With Complex Aurivillius Layer Structure, Zhenxiang Cheng, Xiaolin Wang, Hongyang Zhao, Hideo Kimura
Australian Institute for Innovative Materials - Papers
A ferroelectric thin film of Aurivillius phase K0.5Bi4.5Ti4O15 (KBT) with a complex bismuth layer-structure was fabricated using the pulsed laser deposition method. The thin film grown on Pt/Ti/SiO2/ Si substrate shows a strong c-axis orientation, as revealed by x-ray diffraction results, and platelike growth of grains. A Pt/KBT/Pt capacitor shows a maximum polarization of about 20 µC/cm2. In addition, the capacitor also shows good fatigue resistance, with a decrease of 14.5% in the remanent polarization after 107 switching cycles. This Aurivillius phase with four layers of TiO6 …
Some Complex Systems Engineering Principles, Matthew J. Berryman, Peter Campbell
Some Complex Systems Engineering Principles, Matthew J. Berryman, Peter Campbell
SMART Infrastructure Facility - Papers
Complex adaptive systems can be characterised by many adaptively changing parts, with a large number of interactions, and adaptation at the system level. This body of research can inform the large engineering projects that are characterised by large systems of systems, where interactions to achieve end goals matters, and where designs and the technology of parts in service undergo many adaptive changes. A number of key lessons can be drawn from the complex adaptive systems literature. Firstly, that the use of design patterns, as traditionally applied in software engineering, can also be applied to wider systems engineering and systems integration …
Shell Artefacts And Shell-Working Within The Lapita Cultural Complex, Katherine A. Szabo
Shell Artefacts And Shell-Working Within The Lapita Cultural Complex, Katherine A. Szabo
Faculty of Science - Papers (Archive)
Despite a consistent presence in the archaeological record of the Lapita cultural complex, and their omnipresence in the associated literature, the nature and range of shell artefacts recovered from Lapita sites has only been partially summarized at best. Considering the categories of raw material choice, working techniques, formal artefact types and curation, this article summarizes our current knowledge and points to areas for further research.
Average Mass Scan Of The Total Ion Chromatogram Versus Percentage Chemical Composition In Multivariate Statistical Comparison Of Complex Volatile Mixtures, Niko Radulovic, Polina Blagojevic, Danielle Skropeta
Average Mass Scan Of The Total Ion Chromatogram Versus Percentage Chemical Composition In Multivariate Statistical Comparison Of Complex Volatile Mixtures, Niko Radulovic, Polina Blagojevic, Danielle Skropeta
Faculty of Science - Papers (Archive)
The analysis of complex volatile mixtures by gas chromatography-mass spectrometry (GC-MS) is a time-consuming process. It involves separation and identification of the components based on their retention times and fragmentation patterns, followed by determination of their relative percentages from integration of their peak areas. Herein we show that multivariate statistical analysis of the relative abundances of the m/z values obtained from the average mass scans (AMS) of the complex mixture is a faster and potentially more reliable method of assessing these mixtures. To achieve this, 15 model complex mixtures, were prepared comprising varying amounts of 10 different constituents. The AMS …
Site-Specific Covalent Attachment Of Dna To Proteins Using A Photoactivatable Tus-Ter Complex, Dahdah B. Dahdah, Isabelle Morin, Morgane Moreau, Nicholas E. Dixon, Patrick M. Schaeffer
Site-Specific Covalent Attachment Of Dna To Proteins Using A Photoactivatable Tus-Ter Complex, Dahdah B. Dahdah, Isabelle Morin, Morgane Moreau, Nicholas E. Dixon, Patrick M. Schaeffer
Faculty of Science - Papers (Archive)
Investigations into the photocrosslinking kinetics of the protein Tus with various bromodeoxyuridine-substituted Ter DNA variants highlight the potential use of this complex as a photoactivatable connector between proteins of interest and specific DNA sequences.
Detrital Zircon Sedimentary Provenance Ages For The Eoarchaean Isua Supracrustal Belt Southern West Greenland: Juxtaposition Of An Imbricated Ca. 3700 Ma Juvenile Arc Against An Older Complex With 3920-3760 Ma Components, Allen P. Nutman, Clark R L Friend, Shane Paxton
Detrital Zircon Sedimentary Provenance Ages For The Eoarchaean Isua Supracrustal Belt Southern West Greenland: Juxtaposition Of An Imbricated Ca. 3700 Ma Juvenile Arc Against An Older Complex With 3920-3760 Ma Components, Allen P. Nutman, Clark R L Friend, Shane Paxton
Faculty of Science - Papers (Archive)
The amphibolite facies Eoarchaean Isua supracrustal belt (northern part of the Nuuk region, southern West Greenland) is dominated by strongly deformed metabasalts, with chert, banded iron formation, felsic volcanic and volcano-sedimentary rocks and minor gabbro and sedimentary carbonates. It comprises a suture zone between a northern terrane formed at ca. 3700 Ma and a southern one formed at ca. 3800 Ma. At the junction between these two terranes is a strongly tectonised, thin unit of metachert, BIF and carbonate-bearing rocks with minor detrital components, named the dividing sedimentary unit. Away from the belt, the northern terrane is dominated by ca. …
Eoarchaean Crustal Growth In West Greenland (Itsaq Gneiss Complex) And In Northeastern China (Anshan Area): Review And Synthesis, Allen P. Nutman, Vickie C. Bennett, Clark R L Friend, Frances Jenner, Yusheng Wan, Dunyi Liu
Eoarchaean Crustal Growth In West Greenland (Itsaq Gneiss Complex) And In Northeastern China (Anshan Area): Review And Synthesis, Allen P. Nutman, Vickie C. Bennett, Clark R L Friend, Frances Jenner, Yusheng Wan, Dunyi Liu
Faculty of Science - Papers (Archive)
Eoarchaean crust in West Greenland (the Itsaq Gneiss Complex, 3870-3600 Ma) is >80% by volume orthogneisses derived from plutonic tonalite-trondhjemite-granodiorite (TTG) suites,3850, c. 3810 and c. 3710 Mahave some compositional similarities to modern island arc basalts (IAB), suggesting their origin by hydrous fluxing of a suprasubduction-zone upper mantle wedge. Most of the Eoarchaean tonalites match in composition high-silica, low-magnesian adakites, whose petrogenesis is dominated by partial melting of garnetiferous mafic rocks at high pressure. However, associated with the tonalites are volumetrically minor more magnesian quartz diorites, whose genesis probably involved melting of depleted mantle to which some slab-derived component had …
Spectroscopic Study Of The Benchmark Mn+-H2 Complex, Viktoras Dryza, Berwyck L. J Poad, Evan J. Bieske
Spectroscopic Study Of The Benchmark Mn+-H2 Complex, Viktoras Dryza, Berwyck L. J Poad, Evan J. Bieske
Faculty of Science - Papers (Archive)
We have recorded the rotationally resolved infrared spectrum of the weakly bound Mn+-H2 complex in the H-H stretch region (4022-4078 cm(-1)) by monitoring Mn+ photodissociation products. The band center of Mn+-H2, the H-H stretch transition, is shifted by -111.8 cm(-1) from the transition of the free H2 molecule. The spectroscopic data suggest that the Mn+-H2 complex consists of a slightly perturbed H2 molecule attached to the Mn+ ion in a T-shaped configuration with a vibrationally averaged intermolecular separation of 2.73 A. Together with the measured Mn+...H2 binding energy of 7.9 kJ/mol (Weis, P.; et al. J. Phys. Chem. A 1997, …
Embracing Social Uncertainties With Complex Systems Science, Pascal Perez
Embracing Social Uncertainties With Complex Systems Science, Pascal Perez
SMART Infrastructure Facility - Papers
Human ecosystems are real-life systems characterized by very strong and longterm interactions between human communities and their environment; as such they constitute an expansion of the ecological concept of ecosystem. According to Stepp and colleagues (2003), human ecosystems not only process matter and energy flows, but - and more specifically - information flows as well. Therefore, they display very specific characteristics due to our ability to communicate and learn from others, creating the conditions for co-evolutionary processes in which chance lends a hand to necessity. Bradbury (2006) argues that, until recently, human beings had been able to adapt to changes …
The Largest Eigenvalue Characteristic Of Correlated Complex Wishart Matrices And Its Application To Mimo Mrc Systems, Xianyi Rui, Ronghong Jin, Junping Geng, Xiaojing Huang
The Largest Eigenvalue Characteristic Of Correlated Complex Wishart Matrices And Its Application To Mimo Mrc Systems, Xianyi Rui, Ronghong Jin, Junping Geng, Xiaojing Huang
Faculty of Informatics - Papers (Archive)
In this paper, we analyze statistical properties of the largest eigenvalue of correlated complex Wishart matrices. The results provide an analytical tool for the study of multiple-input multiple-output (MIMO) maximal ratio combining (MRC) systems in the presence of spatial fading correlation at the transmitter or receiver. Based on them, the exact closed-form expressions for the cumulative distribution function and the probability density function of the output signal-to-noise ratio are presented. The analytical results are validated by Monte Carlo simulations.
The Itsaq Gneiss Complex Of Southern West Greeland And The Construction Of Eoarchaean Crust At Convergent Plate Boundaries, Allen P. Nutman, Clark R. L Friend, Kenji Horie, Hiroshi Hidaka
The Itsaq Gneiss Complex Of Southern West Greeland And The Construction Of Eoarchaean Crust At Convergent Plate Boundaries, Allen P. Nutman, Clark R. L Friend, Kenji Horie, Hiroshi Hidaka
Faculty of Science - Papers (Archive)
The ca. 3000 km2ItsaqGneissComplex of the Nuuk region, southernWestGreenland was the first body of pre-3600 Ma crust discovered. Such ancient gneisses are now also known elsewhere, but in total form only about a millionth of the modern crust. The other 99.9999% of ancient crust was destroyed by melting and erosion over billions of years. Understanding the origin of this oldest crust is hampered by metamorphism (repeatedly) in the amphibolite or granulite facies, and most of it having been strongly deformed. The ItsaqGneissComplex is dominated by polyphase grey gneisses derived from several suites of tonalites, granites and subordinate quartz-diorites and ferro-gabbros …
~3,850 Ma Tonalites In The Nuuk Region, Greenland: Geochemistry And Their Reworking Within An Eoarchaean Gneiss Complex, Allen P. Nutman, Vickie C. Bennett, Clark R. L Friend, Kenji Horie, Hiroshi Hidaka
~3,850 Ma Tonalites In The Nuuk Region, Greenland: Geochemistry And Their Reworking Within An Eoarchaean Gneiss Complex, Allen P. Nutman, Vickie C. Bennett, Clark R. L Friend, Kenji Horie, Hiroshi Hidaka
Faculty of Science - Papers (Archive)
The Eoarchaean (>3,600 Ma) Itsaq Gneiss Complex of southern West Greenland is dominated by polyphase orthogneisses with a complex Archaean tectonothermal history. Some of the orthogneisses have c. 3,850 Ma zircons, and they vary from rare single phase metatonalites to more common complexly banded migmatites. This is due to heterogeneous strain, in situ anatexis and granitic veining superimposed during younger tectonothermal events. In the single-phase tonalites with c. 3,850 Ma zircon, oscillatory-zoned prismatic zircon is all 3,850 Ma old, but shows patchy ancient loss of radiogenic Pb. SHRIMP spot analyses and laser ablation ICP-MS depth profiling show that thin …
An Ontology-Based Approach For Expert And Knowledge Mining In Complex Multi-Agent Systems, Minjie Zhang, Xijin Tang, Quan Bai, Jifa Gu
An Ontology-Based Approach For Expert And Knowledge Mining In Complex Multi-Agent Systems, Minjie Zhang, Xijin Tang, Quan Bai, Jifa Gu
Faculty of Informatics - Papers (Archive)
Complex problems require diverse expertise and multiple techniques to solve. In order to solve such problems, complex multi-agent systems include numbers of heterogeneous agents, which may include both of human experts and autonomous agents, to work together toward some complex problems. Most complex multi-agent systems are working in open domains. Due to heterogeneities and dynamic working environments, expertise and capabilities of agents might not be well estimated and presented in the system. Therefore, how to discover useful knowledge from human and autonomous experts, make more accurate estimation for experts' capabilities and to find out suitable expert(s) to solve incoming problems …
Rotationally Resolved Infrared Spectrum Of The Li+_D2 Cation Complex, C D. Thompson, C Emmeluth, B L. J Poad, G H. Weddle, E J. Bieske
Rotationally Resolved Infrared Spectrum Of The Li+_D2 Cation Complex, C D. Thompson, C Emmeluth, B L. J Poad, G H. Weddle, E J. Bieske
Faculty of Science - Papers (Archive)
The infrared spectrum of mass selected Li +-D 2 cations is recorded in the D-D stretch region (2860-2950 cm -1) in a tandem mass spectrometer by monitoring Li + photofragments. The D-D stretch vibration of Li +-D 2 is shifted by -79 cm -1 from that of the free D 2 molecule indicating that the vibrational excitation of the D 2 subunit strengthens the effective Li +-D 2 intermolecular interaction. Around 100 rovibrational transitions, belonging to parallel K a=0-0, 1-1, and 2-2 subbands, are fitted to a Watson A-reduced Hamiltonian to yield effective molecular parameters. The infrared spectrum shows that …
Complex Science For A Complex World: An Introduction, Pascal Perez, David Batten
Complex Science For A Complex World: An Introduction, Pascal Perez, David Batten
SMART Infrastructure Facility - Papers
No abstract provided.
Age, Petrogenesis And Metamorphism Of The Syn-Collisional Proven Igneous Complex, West Greenland, Kristine Thrane, J Baker, J Connelly, Allen Phillip Nutman
Age, Petrogenesis And Metamorphism Of The Syn-Collisional Proven Igneous Complex, West Greenland, Kristine Thrane, J Baker, J Connelly, Allen Phillip Nutman
Faculty of Science - Papers (Archive)
The Paleoproterozoic Prøven Igneous Complex (PIC) in West Greenland extends from ca. 72°15′ to 73°10′N, approximately 500 km north of the subduction-related intrusive complex in the core of the +1100 km wide, asymmetric collisional Nagssugtoqidian-Rinkian Orogen. A new U-Pb SHRIMP age for the PIC of 1869±9 Ma indicates that it intruded synchronously with the main collisional phase of the orogen into the passive margin side of the collision. Sm-Nd and Lu-Hf isotopic and A-type geochemical signatures are compatible with its derivation from melted Archean lower crustal material contaminated to varying degrees by pelitic sedimentary rocks of the Karrat Group. The …
The Epididymal Soluble Prion Protein Forms A High-Molecular-Mass Complex In Association With Hydrophobic Proteins, Heath W. Ecroyd, Maya Belghazi, Jean-Louis Dacheux, Jean-Luc Gatti
The Epididymal Soluble Prion Protein Forms A High-Molecular-Mass Complex In Association With Hydrophobic Proteins, Heath W. Ecroyd, Maya Belghazi, Jean-Louis Dacheux, Jean-Luc Gatti
Faculty of Science - Papers (Archive)
We have shown previously that a 'soluble' form of PrP (prion protein), not associated with membranous vesicles, exists in the male reproductive fluid [Ecroyd, Sarradin, Dacheux and Gatti (2004) Biol. Reprod. 71, 993-1001]. Attempts to purify this 'soluble' PrP indicated that it behaves like a high-molecular-mass complex of more than 350 kDa and always co-purified with the same set of proteins. The main associated proteins were sequenced by MS and were found to match to clusterin (apolipoprotein J), BPI (bacterial permeability-increasing protein), carboxylesterase-like urinary excreted protein (cauxin), beta-mannosidase and beta-galactosidase. Immunoblotting and enzymatic assay confirmed the presence of clusterin and …
New Pieces To The Archaean Terrane Jigsaw Puzzle In The Nuuk Region, Southern West Greeland: Steps In Transforming A Simple Insight Into A Complex Regional Tectonothermal Model, Clark R L Friend, Allen Phillip Nutman
New Pieces To The Archaean Terrane Jigsaw Puzzle In The Nuuk Region, Southern West Greeland: Steps In Transforming A Simple Insight Into A Complex Regional Tectonothermal Model, Clark R L Friend, Allen Phillip Nutman
Faculty of Science - Papers (Archive)
In the south of the Nuuk region of West Greenland our 1980s mapping recognized four Archaean gneiss terranes (Færingehavn, Tre Brødre, Tasiusarsuaq and Akia terranes) with different protolith ages and separate early tectonothermal histories. Later in the Archaean these were juxtaposed and then experienced the same 2700-2500 Ma tectonothermal events. Here we abandon extrapolation of only these four terranes across the whole region, and distinguish two new terranes in the NE. The northernmost Isukasia terrane (previously regarded as the northernmost exposure of the Færingehavn terrane) consists of Palaeoarchaean rocks (>3600 Ma) tectonically bounded on its south by the 3075-2960 …
Complex 3670-3500 Ma Orogenic Episodes Superimposed On Juvenile Crust Accreted Between 3850 And 3690 Ma, Itsaq Gneiss Complex, Southern West Greenland, Clark R L Friend, Allen Phillip Nutman
Complex 3670-3500 Ma Orogenic Episodes Superimposed On Juvenile Crust Accreted Between 3850 And 3690 Ma, Itsaq Gneiss Complex, Southern West Greenland, Clark R L Friend, Allen Phillip Nutman
Faculty of Science - Papers (Archive)
The Itsaq Gneiss Complex of the Nuuk region, southern West Greenland, is dominated by 3850-3690 Ma tonalites intruded into and intercalated with lesser amounts of different ≥3850-3700 Ma supracrustal units. Published wholerock Sr and Nd isotopic studies demonstrate that the tonalites are juvenile crustal additions from a depleted mantle source. From our field studies and SHRIMP U/Pb zircon dating, we argue that this juvenile crustal accretion was spread over ca. 170 m.yr. (≥3850-3690 Ma). Following 3850-3690 Ma juvenile crustal accretion events, the evolution of the Itsaq Gneiss Complex continued with numerous crustal-reworking events between 3670 and 3500 Ma. Examples of …
An Automated Gis Method For Modeling Relative Wave Exposure Within Complex Reef-Island Systems: A Case Study Of The Great Barrier Reef, Marjetta L. Puotinen
An Automated Gis Method For Modeling Relative Wave Exposure Within Complex Reef-Island Systems: A Case Study Of The Great Barrier Reef, Marjetta L. Puotinen
Faculty of Science - Papers (Archive)
Patterns of wave energy play a significant role in shaping the long-term structure of coral reef communities worldwide. For example, sections of reefs have been shown to vary greatly in morphology (dominant size class, growth form) as coral colonies adapt in response to local-scale differences in the wave heights typically experienced. These differences result in zonation (crest, lagoon, and slope), producing characteristic growth forms and species assemblages that vary in their vulnerability to damage from waves (Done 1993). Those communities experiencing the greatest typical wave energy align themselves parallel to the water flow, adopt stream-lined forms and are usually smaller …