Physical Sciences and Mathematics Commons^™

Quantum Chaos, Integrability, And Hydrodynamics In Nonequilibrium Quantum Matter, Javier Lopez Piqueres

Doctoral Dissertations

It is well-known that the Hilbert space of a quantum many-body system grows exponentially with the number of particles in the system. Drive the system out of equilibrium so that the degrees of freedom are now dynamic and the result is an extremely complicated problem. With that comes a vast landscape of new physics, which we are just recently starting to explore. In this proposal, we study the dynam- ics of two paradigmatic classes of quantum many-body systems: quantum chaotic and integrable systems. We leverage certain tools commonly employed in equilibrium many-body physics, as well as others tailored to the …

Development Of An Integrated Workflow For Nucleosome Modeling And Simulations, Ran Sun

Doctoral Dissertations

Nucleosomes are the building blocks of eukaryotic genomes and thus fundamental to to all genetic processes. Any protein or drug that binds DNA must either cooperate or compete with nucleosomes. Given that a nucleosome contains 147 base pairs of DNA, there are approximately 4^147 or 10^88 possible sequences for a single nucleosome. Exhaustive studies are not possible. However, genome wide association studies can identify individual nucleosomes of interest to a specific mechanism, and today's supercomputers enable comparative simulation studies of 10s to 100s of nucleosomes. The goal of this thesis is to develop and present and end-to-end workflow that serves …

Synthesis And Characterization Of Quantum Materials, Yunsheng Qiu

Doctoral Dissertations

"In this study, attempts were made to grow quantum materials that have recently undergone a profound change of perspective. These materials are involved in intricate macroscopic properties rooted in the subtle nature of quantum physics. To explore our understanding of quantum materials, this study includes three projects: Magnetic Topological Insulators, Topological Superconductors, and high-temperature superconductors.

A Cr-doped Sb₂Te₃ is added to the category for the magnetic topological insulators project. Their transport properties are studied, and the origin of ferromagnetism is studied. Anomalous Hall effect is observed in the Hall measurements, and serval factors (cooling rate, dopant deficiency) …

The Science Of Gravitational-Wave Sources And Beyond Compact Binary Coalescences, Yanyan Zheng

Doctoral Dissertations

"This work focuses on the field of gravitational-wave astronomy by extending the scope of detectable sources beyond compact binary coalescences, All the gravitational-wave detections so far come from compact binary coalescences. Focusing on core-collapse supernovae as promising sources for short gravitational-wave transients, this work reports optically targeted searches for gravitational-wave emitted by core-collapse supernovae during the third observing run of the LIGO and Virgo detectors. It also predicts the search sensitivity for the ongoing fourth and forthcoming fifth observing runs. Moreover, the work introduces a novel computational framework for testing the spatial distribution of binary black hole sources, allowing for …

Atomic-Level Mechanisms Of Fast Relaxation In Metallic Glasses, Leo W. Zella

Doctoral Dissertations

Glasses are ubiquitous in daily life and have unique properties which are a consequence of the underlying disordered structure. By understanding the fundamental processes that govern these properties, we can modify glasses for desired applications. Key to understanding the structure-dynamics relationship in glasses is the variety of relaxation processes that exist below the glass transition temperature. Though these relaxations are well characterized with macroscopic experimental techniques, the microscopic nature of these relaxations is difficult to elucidate with experimental tools due to the requirements of timescale and spatial resolution. There remain many questions regarding the microscopic nature of relaxation in glass …

A Measurement Of Neutron Polarization And Transmission For The Nedm@Sns Experiment, Kavish Imam

Doctoral Dissertations

The D.O.E Nuclear Science Advisory Committee Long Range Plan has called for experimental programs to explore fundamental symmetry violations and their implications in nuclear, particle and cosmological physics. The neutron electric dipole moment experiment at the Spallation Neutron Source (nEDM@SNS) aims to search for new physics in the Time-reversal (T) and Charge-Parity (CP) symmetry violating sector by setting a new limit on the nEDM down to a few x 10^-28 e·cm using a novel cryogenic technique, which combines the unique properties of polarized Ultracold Neutrons (UCN), polarized ³He, and superfluid ⁴He. The experiment will employ a cryogenic …

Short Range Correlation Measurements In The Quasielastic Region With An 11 Gev Beam, Casey Morean

Doctoral Dissertations

Electron scattering is a significant means of studying internal high momentum
nucleon and quark distributions in nuclei. Thomas Jefferson National Accelerator
Facility (JLab) with its 11GeV beam is capable of studying high momentum nucleons
with unmatched precision. The role of short range nucleon configurations and
quark distributions is significant for understanding the dynamics of nuclei and their
underlying components. Scattering cross section measurements in the kinematic
regime x > 1, where the free nucleon is forbidden, are sensitive to high momentum
nucleons, which are believed to come from short range correlations (SRCs). SRCs are
strongly interacting, high momentum nucleons with a …

Generative Adversarial Game With Tailored Quantum Feature Maps For Enhanced Classification, Anais Sandra Nguemto Guiawa

Doctoral Dissertations

In the burgeoning field of quantum machine learning, the fusion of quantum computing and machine learning methodologies has sparked immense interest, particularly with the emergence of noisy intermediate-scale quantum (NISQ) devices. These devices hold the promise of achieving quantum advantage, but they grapple with limitations like constrained qubit counts, limited connectivity, operational noise, and a restricted set of operations. These challenges necessitate a strategic and deliberate approach to crafting effective quantum machine learning algorithms.

This dissertation revolves around an exploration of these challenges, presenting innovative strategies that tailor quantum algorithms and processes to seamlessly integrate with commercial quantum platforms. A …

When To Hold And When To Fold: Studies On The Topology Of Origami And Linkages, Mary Elizabeth Lee

Doctoral Dissertations

Linkages and mechanisms are pervasive in physics and engineering as models for a
variety of structures and systems, from jamming to biomechanics. With the increase
in physical realizations of discrete shape-changing materials, such as metamaterials,
programmable materials, and self-actuating structures, an increased understanding
of mechanisms and how they can be designed is crucial. At a basic level, linkages
or mechanisms can be understood to be rigid bars connected at pivots around which
they can rotate freely. We will have a particular focus on origami-like materials, an
extension to linkages with the added constraint of faces. Self-actuated versions typ-
ically start …

Search For Exotic Higgs Boson Decay To Multiple B-Quarks With The Atlas Detector At Lhc Using Machine Learning Methods, Yuan-Tang Chou

Doctoral Dissertations

The discovery of the Higgs boson has opened up new possibilities for investigating physics beyond the Standard Model (SM). New particles may interact with the SM through the Higgs boson, and deviations from SM predictions can indicate the presence of new physics. This dissertation focuses on the search for exotic Higgs decay, $H\rightarrow aa \rightarrow (b\bbar)(b\bbar)$ where a is a new scalar boson and focuses on the case where the Higgs boson is produced in association with a Z boson. The data were collected by the ATLAS detector at the Large Hadron Collider at center-of-mass energy $\sqrt{s} =~13~\TeV$ from 2015 …

Experiments With Monopoles, Rings And Knots In Spinor Bose-Einstein Condensates, Alina A. Blinova

Doctoral Dissertations

Topological excitations are ubiquitous in nature, their charge being a naturally-quantized, conserved quantity that can exhibit particle-like behavior. Spinor Bose-Einstein condensates (BECs) are an exceptionally versatile system for the study and exploration of topological excitations. Between the spin-1 and spin-2 ⁸⁷Rb condensates there are seven possible broken-symmetry magnetic phases, with each one hosting unique opportunities for topological defects. We have created and observed several novel topological excitations in a spinor ⁸⁷Rb BEC. In this dissertation I present and discuss three principal experimental findings: (1) The discovery of an Alice ring, or a half-quantum vortex ring, emerging from a …

Tev-Scale Lepton Number Violation: 0Νββ Decay, The Origin Of Matter, And Energy Frontier Probes, Sebastian Urrutia Quiroga

Doctoral Dissertations

Lepton number violation (LNV) offers promising theoretical pathways to several unresolved problems in particle and nuclear physics and unveils a diverse range of phenomenology across different energy scales. TeV-scale LNV is especially relevant for both its experimental accessibility and its broad-ranging impact, making it a key area of interest for both theoretical and experimental physicists. In this thesis, we explore three distinct scenarios within the LNV research landscape. Our first analysis concerns the implications of TeV-scale LNV effects in thermal leptogenesis and its complementary sensitivity in neutrinoless double beta (0νββ) decay and collider experiments. We employed a simplified model to …

The Fate Of The Crossbridge After Phosphate Rebinding: Implications For Fatigue, Christopher P. Marang

Doctoral Dissertations

In response to repeated intense contractile activity, a muscle’s ability to generate force decreases due to the created state of muscular fatigue. This compromised force production state is dependent on changes within the microenvironment of muscle thought to alter the function of the force generating, contractile protein myosin. For example, phosphate (P_i), elevated during fatigue, has been suggested to alter how myosin generates force. However, the effects of P_i are not straightforward, as muscle fiber data suggest that P_i's interaction with myosin may be force-dependent. In particular, P_i has no effect on maximal shortening …

Deformations Of Geometrically Frustrated Elastic Sheets, Meng Xin

Doctoral Dissertations

The wrinkling and buckling of thin solids are common phenomena in our daily life and can be observed in many situations, such as crumpled papers, stretched plastics, compressed metals, clothes on our bodies and even furrowed human skin. Understanding of these phenomena has therefore long drawn interest of scholars. In this thesis, we discuss two buckling problems numerically and analytically. First, we study the wrinkling mechanism of stretched sheets with clamped edges. A central puzzle underlying this canonical example of “tensional wrinkling” has been the origin of compressive stress, which eventually leads to buckling instability. We elucidate the source of …

Dinitrogen Functionalization Using A Molybdenum Atom: Bridging The Gap Between Small And Coordination Complexes Via Quantum Mechanical Methods, Maria Virginia White

Doctoral Dissertations

Chemistry devotes a significant amount of its research to understanding small molecule activation from an electronic structure perspective to help with the investigation of the reaction pathways of catalytically active substances that can promote biomimetic catalysis. A large portion of the energy used annually in our planet is used for the artificial nitrogen fixation (Haber-Bosch process), which renders dinitrogen activation a subject of study. Molybdenum, a fourth row transitional metal, has demonstrated its effectiveness as an essential component of the dinitrogen reduction catalytic process. To better understand the multiple dinitrogen molybdenum binding modes, the work described herein combines wave function …

Chirality, Symmetry-Breaking, And Chemical Substitution In Multiferroics, Kiman Park

Doctoral Dissertations

Multiferroic materials attract significant attention due to their potential utility in a broad range of device applications. The inclusion of heavy metal centers in these materials enhances their magnetoelectric properties, yielding fascinating physical phenomena such as the Dzyaloshinskii–Moriya interaction, nonreciprocal directional dichroism, enhancement of spin-phonon coupling, and spin-orbit-entangled ground states. This dissertation provides a comprehensive survey of magnetoelectric multiferroics containing heavy metal centers and explores spectroscopic techniques under extreme conditions. A microscopic examination of phase transitions, symmetry-breaking, and structure-property relationships enhances the fundamental understanding of coupling mechanisms.

In A2Mo3O8 (A = Fe, Zn, Ni, and Mn), we use optical spectroscopy …

Exploring Skyrmions Dynamics And Structure Using Neutron Scattering, W-L-Namila Chandula Liyanage

Doctoral Dissertations

Magnetic skyrmions are topologically protected chiral spin textures with great potential for next-generation consumer technologies. These magnetic structures can be described as spins continuously wrapping into a closed coplanar loop, featuring a core and fencing perimeter with opposite out-of-plane orientations. While conventional depictions of magnetic skyrmions use a two-dimensional projection, recent research underscores the importance of their three-dimensional structure in determining their topology and stability. Magnetic skyrmions typically emerge just below the curie temperature of a magnetic material, creating what is known as a skyrmion pocket. In most materials the stability pocket is at low temperatures and finite fields, however …

Sub-Chandrasekhar Type Ia Supernovae Scenarios With Increased Pathways For Neutronization, Fernando Hernan Rivas

Doctoral Dissertations

Type Ia supernovae are thermonuclear explosions of white dwarfs (WD), electron-degenerate cores of old intermediate mass stars(under 8$M_{\odot}$). Reaching energies of $10^{51}$\si{\erg}, they outshine whole galaxies as they synthesize and distribute most of the iron group elements (IGE; V, Cr, Mn, Fe, Co, Ni) into the interstellar medium, thus being one of the main agents in cosmic chemical evolution. Also, given their notably homogeneous lightcurves, they form the last step in the cosmic distance ladder outdistancing Cepheid variables by orders of magnitude. Though calibration of said lightcurves is dependent on a high number of confirmed events, the limits of statistical …

Fabrication, Measurements, And Modeling Of Semiconductor Radiation Detectors For Imaging And Detector Response Functions, Corey David Ahl

Doctoral Dissertations

In the first part of this dissertation, we cover the development of a diamond semiconductor alpha-tagging sensor for associated particle imaging to solve challenges with currently employed scintillators. The alpha-tagging sensor is a double-sided strip detector made from polycrystalline CVD diamond. The performance goals of the alpha-tagging sensor are 700-picosecond timing resolution and 0.5 mm spatial resolution. A literature review summarizes the methodology, goals, and challenges in associated particle imaging. The history and current state of alpha-tagging sensors, followed by the properties of diamond semiconductors are discussed to close the literature review. The materials and methods used to calibrate the …

Path Integral Monte Carlo For Entanglement In Bosonic Lattices At T = 0, Emanuel Casiano-Diaz

Doctoral Dissertations

Path-Integral Monte Carlo Worm Algorithm is one of many Quantum Monte Carlo (QMC) methods that serve as powerful tools for the simulation of quantum many-body systems. Developed in the late 90’s, this algorithm has been used with great success to study a wide array of physical models where exact calculation of observables is not possible due to the exponential size of the Hilbert space. One type of systems that have eluded PIMC-WA implementation are lattice models at zero temperature, which are of relevance in experimental settings, such as in optical lattices of ultra-cold atoms. In this thesis, we develop a …

Pointing Control And Stabilization Of The High-Energy Uv Laser For Laser-Assisted Charge Exchange, Martin Joseph Kay

Doctoral Dissertations

Laser-Assisted Charge Exchange (LACE) is an experimental method of charge exchange injection into a proton accumulator ring that is being developed at the Spallation Neutron Source (SNS) in Oak Ridge National Laboratory (ORNL) as an alternative to hazardous injection foils. The current scheme of LACE requires a high-energy, low-repetition-rate UV (355 nm) laser beam (140 mJ pulses at 10 Hz) to be transported over 65 meters to the laser-particle interaction point (IP) in a high-radiation area of the accelerator. Thermal effects and other disturbances along the free-space laser transport line cause the beam to slowly drift away from the IP …

Total Absorption Spectroscopy Of Mo-106 And Tc-106, Michael Cooper

Doctoral Dissertations

Total absorption spectroscopy is a method of gamma-ray spectroscopy that has gained prominence in the past several decades, as nuclear data revisions are performed on older nuclear data, which is often incomplete. A strong understanding of underlying nuclear data, particularly fission and beta decay data, is essential for nuclear reactors and nuclear fuel decay heat. This PhD work involves the analysis of fission fragments 106Mo [Mo-106] and 106Tc [Tc-106]. These neutron rich isotopes contribute upwards of 6% of the cumulative fission yield of 241Pu [Pu-241] fission, and 4% of 239Pu [Pu-239] fission. Prior data for these two fission fragments only …

Neutrino Physics At A Research Reactor: Backgrounds And Analysis, Blaine Alexander Heffron

Doctoral Dissertations

The field of neutrino physics has a rich history and is currently the subject of much active research. The discovery of neutrino oscillations led to the conclusion that neutrinos have mass which was in contradiction to the Standard Model. Now researchers are investigating a number of open questions regarding neutrino properties such as their mass values or the existence of CP violation in the weak interaction. In order to answer these questions experimental and analytical techniques of neutrino detection are becoming more advanced, entering into an era of precision neutrino detection.

Nuclear reactors as a source of antineutrinos have played …

Unlocking The Potential Of Machine Learning In The Derivation Of Low-Energy Models For Metallic Magnets, Vikram Sharma

Doctoral Dissertations

Condensed matter physics often grapples with complex many-particle problems lacking definitive closed-form solutions, necessitating approximation strategies to investigate low-energy sectors of the Hilbert space. Perturbation theory, though widely used for this purpose, is limited when expansion terms diverge. This work introduces a machine learning (ML) assisted protocol to extract effective low-energy models for lattice models of fermions interacting with classical fields, specifically focusing on the Kondo Lattice Model (KLM).

Skyrmions, featuring whirling spin texture and topological protection, are promising candidates for future spintronic devices. Materials featuring conduction electrons coupled to localized $f$-electrons' net moment are ideal for realizing skyrmions and …

Fourth Order Dispersion In Nonlinear Media, Georgios Tsolias

Doctoral Dissertations

In recent years, there has been an explosion of interest in media bearing quartic
dispersion. After the experimental realization of so-called pure-quartic solitons, a
significant number of studies followed both for bright and for dark solitonic struc-
tures exploring the properties of not only quartic, but also setic, octic, decic etc.
dispersion, but also examining the competition between, e.g., quadratic and quartic
dispersion among others.
In the first chapter of this Thesis, we consider the interaction of solitary waves in
a model involving the well-known φ⁴ Klein-Gordon theory, bearing both Laplacian and biharmonic terms with different prefactors. As a …

Self-Limiting Morphologies In Geometrically Frustrated Assemblies, Douglas M. Hall

Doctoral Dissertations

Geometrically frustrated assembly, where locally preferred motifs are incompatible with constraints on global ordering of the assembly, may result in a super-extensive energy penalty to assembly growth and self-limitation of the assembly size. Using theory and simulation, we study how this mechanism may also shape the assembly's boundary and its interior packing, which are distinct morphological changes. In Chapter 1, we provide some background and a theoretical framework for understanding self-limiting behavior due to geometric frustration. Three distinct projects are detailed in the subsequent chapters: original numerical results are presented on competing responses to frustration in helical bundles made of …

Novel Quantum Materials For Spintronic And Opto-Electronic Applications, Ali Sarikhani

Doctoral Dissertations

"Multi-functional quantum materials play a crucial role in the development of spintronics and opto-electronics, as their properties can greatly influence device performance. For instance, in spintronics, materials such as ferromagnetic half-metals, Giant Magnetoresistants (GMR), and magnetic semiconductors have been extensively studied due to their ability to manipulate the spin of electrons for applications in magnetic storage. In opto-electronics, materials such as Diluted Magnetic Semiconductors (DMS) and non-oxide Transparent Conductors (TC) offer advantages such as tunable bandgap and high absorption coefficients, which enable improved device performance.

For this purpose, we have experimentally investigated the compounds that have shown theoretically interesting physical …

Near-Ir Spectroscopic Analysis Of The Primary Volatile Composition Of Long And Short-Period Comets, Younas Khan

Doctoral Dissertations

"Comets are among the most well-preserved objects that formed in the protosolar nebula ∼4.5 Gyr ago. Hence, they are important for understanding various aspects of the formation, evolution, and habitability of the solar system. Multiple primary volatiles (molecules directly sublimating into the coma from the nucleus) emit via rovibrational transitions in the near-IR, providing opportunities to calculate their abundances. To date, only ∼50 comets have been characterized for their primary volatiles, with the short-period Jupiter-family comets (JFCs) being significantly underrepresented. In contrast, hundreds of comets have been sampled at optical/UV wavelengths, primarily for the composition of daughter species, leading to …

Core-Collapse Supernova Simulations With Spectral Two-Moment Neutrino Transport, Ran Chu

Doctoral Dissertations

The primary focus of this dissertation is to develop a next-generation, state-of-the-art neutrino kinetics capability that will be used in the context of the next-generation, state-of-the-art core-collapse supernova (CCSN) simulation frameworks \thornado\ and \FLASH.\index{CCSN} \thornado\ is a \textbf{t}oolkit for \textbf{h}igh-\textbf{or}der \textbf{n}eutrino-r\textbf{ad}iation hydr\textbf{o}dynamics, which is a collection of modules that can be incorporated into a simulation code/framework, such as \FLASH, together with a nuclear equation of state (EOS)\index{EOS} library, such as the \WeakLib\ EOS tables. The first part of this work extends the \WeakLib\ code to compute neutrino interaction rates from~\cite{Bruenn_1985} and produce corresponding opacity tables.\index{Bruenn 1985} The processes of emission, …

Development Of A New High-Resolution Neutron Detector And Beta-Delayed Neutron Spectroscopy Of 24o., Shree K. Neupane

Doctoral Dissertations

An efficient neutron detection system with good energy resolution is needed to correctly characterize the decays of neutron-rich nuclei where beta-delayed neutron emission is a dominant decay mode. Precision neutron spectroscopy probes nuclear structure effects in neutron-rich nuclei and is essential to exploit the opportunities in new-generation radioactive beam facilities. A new high-resolution neutron detector, Neutron dEtector with Xn Tracking (NEXT), has been constructed, characterized, and tested in decay and reaction experiments. Its essential capability is the neutron interaction position localization, which enables improvement in energy resolution without compromising detection efficiency in the time-of-flight measurements. Neutron-gamma discrimination capability of NEXT …

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