Physical Sciences and Mathematics Commons^™

Time-Resolved, Near Atomic Resolution Structural Studies At The Free Electron Laser, Jason James Tenboer

Theses and Dissertations

Time-resolved serial femtosecond crystallography (TR-SFX) employs X-ray free electron lasers (XFELs) to provide X-ray pulses of femtosecond (fs) duration with 1012 photons per pulse. These XFELs are more than a billion times more brilliant than 3rd generation synchrotron X-ray sources. For structure determination, protein crystals on the micrometer length scale (microcrystals) are injected into the X-ray beam and the resulting diffraction patterns are recorded on fast-readout pixel detectors. Although these intense pulses deposit enough energy to ultimately destroy the protein, the processes that lead to diffraction occur before the crystal is destroyed. This so-called diffraction-before-destruction principle overcomes radiation damage, which …

Theoretical Investigation Of Interactions And Relaxation In Biological Macromolecules, Koki Yokoi

Theses and Dissertations

One of the major challenges posed to our quantitative understanding of structure, dynamics, and function of biological macromolecules has been the high level of complexity of biological structures. In the present work, we studied interactions between G protein-coupled receptors (GPCRs), and also introduced a theoretical model of relaxation in complex systems, in order to help understand interactions and relaxation in biological macromolecules.

GPCRs are the largest and most diverse family of membrane receptors that play key roles in mediating signal transduction between outside and inside of a cell. Oligomerization of GPCRs and its possible role in function and signaling currently …

Theoretical Study Of Magnetoelectric Effects In Noncentrosymmetric And Cuprate Superconductors, Manoj Kumar Kashyap

Theses and Dissertations

A century after the discovery of superconductivity at the lab of Kamerlingh Onnes

in 1911, it is noticeable that the phenomenon is quite ubiquitous in nature. In addi-

tion to a long list of superconducting alloys and compounds, almost half the elements

in the periodic table superconduct. By the late seventies, superconductivity was

thought to be well understood. This turned out to be a myth, with the discovery of

unconventional superconductors that defied Bardeen-Cooper-Schrieffer (BCS) theory.

Cuprates have been the most prominent example among them ever since their discov-

ery in 1986 by Bednorz and M ̈uller. Another example of …

Tunneling Experiments With Dirac Electrons In Graphene Heterojunctions, Shivani Rajput

Theses and Dissertations

This dissertation presents results of scanning tunneling microscopy/spectroscopy experiments performed on graphene, a two-dimensional membrane of carbon atoms arranged in a honeycomb lattice, where charge carriers behave like massless fermions described by the Dirac equation. Our findings demonstrate that interface engineering is a viable route to control and further enhance the electronic properties of graphene.

In the first experiment, by transferring chemical vapor deposited (CVD) graphene onto substrates of opposite polarization - H-terminated Si-face and C-faces of hexagonal silicon carbide (SiC), we show that the type of charge carrier in graphene can be controlled by substrate polarization. Furthermore, we find …

Gravitational Waves From Rotating Neutron Stars And Compact Binary Systems, Leslie Wade

Theses and Dissertations

It is widely anticipated that the first direct detections of gravitational waves will be made by advanced gravitational-wave detectors, such as the two Laser Interferometer Gravitational-wave Observatories (LIGO) and the Virgo interferometer. In preparation for the advanced detector era, I have worked on both detection and post-detection efforts involving two gravitational wave sources: isolated rotating neutron stars (NSs) and compact binary coalescences (CBCs). My dissertation includes three main research projects: 1) a population synthesis study assessing the detectability of isolated NSs, 2) a CBC search for intermediate-mass black-hole binaries (IMBHBs), and 3) new methods for directly measuring the neutron-star (NS) …

Novel Two-Dimensional Nanomaterials And Their Gas Sensing Properties, Haihui Pu

Theses and Dissertations

Graphene, an atomic thin two-dimensional (2D) material with C atoms arranged in a honeycomb lattice, has sparked an unprecedented research interest across various scientific communities since its initial mechanical isolation in 2004. The linear energy dispersion with respect to the momentum within 1 eV around the Fermi level at the high symmetric K (Dirac) points in the Brillouin zone renders graphene a wonder material for scientists. However, graphene’s semimetallic nature significantly limits its high-end applications, e.g., in digital logic circuits. Therefore, continued efforts in opening the band gap for graphene and in searching for novel 2D semiconducting materials are rewarding. …

Gravitational-Wave Science With The Laser Interferometer Gravitational-Wave Observatory, Madeline Wade

Theses and Dissertations

Gravitational-waves, as predicted by Einstein’s theory of general relativity, are oscillations of spacetime caused by the motion of masses. Although not yet directly detected, there is strong evidence for the existence of gravitational-waves. Detectable gravitational waves will come from dramatic astrophysical events, such as supernova explosions and collisions of black holes. The Laser Interferometer Gravitational-wave Observatory (LIGO) is a network of detectors designed to make the first direct detection of gravitational waves. The upgraded version of LIGO, Advanced LIGO (aLIGO), will offer a dramatic improvement in sensitivity that will virtually guarantee detections.

Gravitational-wave detections will not only illuminate mysterious astrophysical …

Self-Force On Accelerated Particles, Thomas Michael Linz

Theses and Dissertations

The likelihood that gravitational waves from stellar-size black holes spiraling into a supermassive black hole would be detectable by a space based gravitational wave observatory has spurred the interest in studying the extreme mass-ratio inspiral (EMRI) problem and black hole perturbation theory (BHP). In this approach, the smaller black hole is treated as a point particle and its trajectory deviates from a geodesic due to the interaction with its own field. This interaction is known as the gravitational self-force, and it includes both a damping force, commonly known as radiation reaction, as well as a conservative force. The computation of …

Topics In Broadband Gravitational-Wave Astronomy, Sydney Joanne Chamberlin

Theses and Dissertations

The direct detection of gravitational waves promises to open a new observational window onto the universe, and a number of large scale efforts are underway worldwide to make such a detection a reality. In this work, we attack some of the current problems in gravitational-wave detection over a wide range of frequencies.

In the first part of this work, low frequency gravitational-wave detection is considered using pulsar timing arrays (PTAs). PTAs are a promising tool for probing the universe through gravitational radiation. Supermassive black hole binaries (SMBHBs), cosmic strings, relic gravitational waves from inflation, and first order phase transitions in …