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Full-Text Articles in Physical Sciences and Mathematics

Magnetic-Field-Induced Alignment-To-Orientation Conversion In Sodium, G. Schinn, Xianming Han Oct 2015

Magnetic-Field-Induced Alignment-To-Orientation Conversion In Sodium, G. Schinn, Xianming Han

Xianming Han

We report a detailed investigation of excited-state alignment-to-orientation conversion in the presence of an external magnetic field. This counterintuitive phenomenon occurs under intermediate-coupling conditions. A weak, linearly polarized, cw laser beam was used to excite and align the Na 3P3/2 state in an atomic beam along the z direction. The degree of circular polarization of the resulting fluorescence was detected along the z direction as a function of magnetic-field strength. The spectrally integrated transitions originating from individual F levels of the 3S1/2 state yield a maximum circular-polarization fraction of ∼40%; integrating the circular polarization over all the allowed 3S1/2-3P3/2 transitions …


Collision Induced Superfluorescence, A. Kumarakrishnan, Siddharaj Chudasama, Xianming Han Oct 2015

Collision Induced Superfluorescence, A. Kumarakrishnan, Siddharaj Chudasama, Xianming Han

Xianming Han

We have studied superfluorescence (SF) in Ca vapor evolving on the 3d4s3DJ-4s4p3PJ−1 transitions at 1.9 mm by exciting the 4s21S0-4s4p1P1 with a pulsed dye laser. SF is generated following population transfer by spinchanging collisions with an inert gas Ar from the 4s4p1P1 and 3d4s1D2 levels. We show for the first time to our knowledge that the time delay for SF evolution follows the 1/ÎN dependence expected for the case of uniform excitation of the vapor column by collisional transfer. Here, N is the number of participating atoms that was measured directly from the photon yield. The measured photon yield for …


Diamond Growth Reactor Chemistry And Film Nucleation Enhancement Using Chlorinated Hydrocarbons, James Chenault, Charles Feigerle, Xianming Han, Robert Shaw Oct 2015

Diamond Growth Reactor Chemistry And Film Nucleation Enhancement Using Chlorinated Hydrocarbons, James Chenault, Charles Feigerle, Xianming Han, Robert Shaw

Xianming Han

The chemistry of diamond film growth from chlorinated hydrocarbons has been investigated using a hot filament reactor coupled to an orifice sampling mass spectrometer. The relative concentrations of the species present near the growth surface have been determined as a function of filament temperature for dilute mixtures of CH4, CH3Cl, CH2Cl2 and CHCl3 in H2. Mass spectral analysis indicated that chlorinated hydrocarbons are sequentially dechlorinated in the presence of hydrogen at moderate reactor temperatures. A dark film was deposited on all surfaces of the reactor during studies of this dechlorination of CHCl3. Raman analysis indicated that these deposits are small …


Collisional Dynamics Of The First Excited States Of Neon In The 590-670 Nm Region Using Laser Optogalvanic Spectroscopy, Xianming Han, M. Su, C. Haridass, P. Misra Oct 2015

Collisional Dynamics Of The First Excited States Of Neon In The 590-670 Nm Region Using Laser Optogalvanic Spectroscopy, Xianming Han, M. Su, C. Haridass, P. Misra

Xianming Han

A mathematical rate equation model, incorporating the various processes contributing to the generation of optogalvanic signals in a discharge plasma, has been used to analyze the time-resolved waveforms of neon in the wavelength region 590–670 nm. Amplitudes, decay rates and the appropriate instrumental time constant have been determined using a non-linear least-squares fit of the observed time-resolved optogalvanic waveforms.


Abrupt Change In Neon Discharge Plasma Detected Through Optogalvanic Effects, Xianming Han, Michael Blosser, Prabhakar Misra, Haridass Chandran Oct 2015

Abrupt Change In Neon Discharge Plasma Detected Through Optogalvanic Effects, Xianming Han, Michael Blosser, Prabhakar Misra, Haridass Chandran

Xianming Han

When a laser is tuned between two excited energy levels of a gas in a Direct Current discharge lamp, the discharge current will experience a temporary disturbance lasting tens or hundreds of microseconds known as the optogalvanic effect. We have carried out extensive studies of optogalvanic effects in neon discharge plasmas for transitions at 621.7 nm, 630.5 nm, 638.3 nm, 650.7 nm and 659.9 nm. A nonlinear least-squares Monte Carlo technique has been used to determine the relevant amplitude coefficients, decay rates and the instrumental time constant. We discovered an abrupt change in the neon discharge plasma at a discharge …


Collisional Ionization Of Excited State Neon In A Gas Discharge Plasma, Xianming Han, Verl Wiseheart, Scott Conner, Meng-Chih Su, David Monts Oct 2015

Collisional Ionization Of Excited State Neon In A Gas Discharge Plasma, Xianming Han, Verl Wiseheart, Scott Conner, Meng-Chih Su, David Monts

Xianming Han

We report the first case where it is possible to clearly identify and quantitatively characterize the dominant physical processes contributing to production of the optogalvanic effect (OGE) signal in a discharge plasma. This work concentrates on the simplest case where only two states are involved in the optical transition. The theoretical model with only four parameters is in excellent agreement with the experimentally obtained time-resolved OGE waveforms. The collisional ionization rate in the upper state is twice as fast as that in the lower state although the two states are only separated by 1.94 eV. We conclude that the optogalvanic …


Investigations Of Superfluorescent Cascades, A. Kumarakrishnan, Xianming Han Oct 2015

Investigations Of Superfluorescent Cascades, A. Kumarakrishnan, Xianming Han

Xianming Han

We report our studies of superfluorescent cascades in atomic calcium which result from two-photon excitation of several levels reasonably close to the ionization limit. We have observed significant conversion efficiencies for some of these transitions which result in subnanosecond pulses particularly in the visible wavelengths. We report the discovery of a novel two-photon scattering mechanism which could prove to be a useful method for determining collisional broadening rates. In addition, a hyper Raman transition near 17 μm is discovered which appears to be a promising candidate for a tunable source.


Production And Diagnosis Of A Highly Spin-Polarized Na Beam, G. Schinn, Xianming Han, A. Gallagher Oct 2015

Production And Diagnosis Of A Highly Spin-Polarized Na Beam, G. Schinn, Xianming Han, A. Gallagher

Xianming Han

We describe optically pumping a beam of sodium atoms to >96% mS and >92% mS, mI state selection. (We have accurately measured the population of every mS, mI state in the optically pumped beam.) For the optical pumping both ground hyperfine states are pumped, using single-mode cw dye-laser radiation tuned to the 3S1/2–3P1/2 transition that is phase modulated in a LiTaO3 crystal to produce first-order sidebands at approximately the 1772-MHz hyperfine splitting of the ground state. The z-directed optical pumping is performed in a z-directed magnetic field of ~5 G. The state-selected atoms then move, in ~1 cm, into an …