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Full-Text Articles in Physical Sciences and Mathematics

Spectral Aerosol Extinction (Spex): A New Instrument For In Situ Ambient Aerosol Extinction Measurements Across The Uv/Visible Wavelength Range, C. E. Jordan, B E. Anderson, A J. Beyersdorf, C A. Corr, Jack E. Dibb, Margaret E. Greenslade, R F. Martin, R H. Moore, Eric Scheuer, M A. Shook, Kenn L. Thornhill, D Troop, Luke D. Ziemba, E L. Winstead Nov 2015

Spectral Aerosol Extinction (Spex): A New Instrument For In Situ Ambient Aerosol Extinction Measurements Across The Uv/Visible Wavelength Range, C. E. Jordan, B E. Anderson, A J. Beyersdorf, C A. Corr, Jack E. Dibb, Margaret E. Greenslade, R F. Martin, R H. Moore, Eric Scheuer, M A. Shook, Kenn L. Thornhill, D Troop, Luke D. Ziemba, E L. Winstead

Earth Sciences

We introduce a new instrument for the measurement of in situ ambient aerosol extinction over the 300– 700 nm wavelength range, the spectral aerosol extinction (SpEx) instrument. This measurement capability is envisioned to complement existing in situ instrumentation, allowing for simultaneous measurement of the evolution of aerosol optical, chemical, and physical characteristics in the ambient environment. In this work, a detailed description of the instrument is provided along with characterization tests performed in the laboratory. Measured spectra of NO2 and polystyrene latex spheres (PSLs) agreed well with theoretical calculations. Good agreement was also found with simultaneous aerosol extinction measurements at …


Neither Dust Nor Black Carbon Causing Apparent Albedo Decline In Greenland's Dry Snow Zone: Implications For Modis C5 Surface Reflectance, Chris Polashenski, Jack E. Dibb, Mark G. Flanner, Justin Y. Chen, Zoe R. Courville, Alexandra M. Lai, James J. Schauer, Martin M. Shafer, Mike Bergin Nov 2015

Neither Dust Nor Black Carbon Causing Apparent Albedo Decline In Greenland's Dry Snow Zone: Implications For Modis C5 Surface Reflectance, Chris Polashenski, Jack E. Dibb, Mark G. Flanner, Justin Y. Chen, Zoe R. Courville, Alexandra M. Lai, James J. Schauer, Martin M. Shafer, Mike Bergin

Earth Sciences

Remote sensing observations suggest Greenland ice sheet (GrIS) albedo has declined since 2001, even in the dry snow zone. We seek to explain the apparent dry snow albedo decline. We analyze samples representing 2012–2014 snowfall across NW Greenland for black carbon and dust light-absorbing impurities (LAI) and model their impacts on snow albedo. Albedo reductions due to LAI are small, averaging 0.003, with episodic enhancements resulting in reductions of 0.01–0.02. No significant increase in black carbon or dust concentrations relative to recent decades is found. Enhanced deposition of LAI is not, therefore, causing significant dry snow albedo reduction or driving …


Brown Carbon Aerosol In The North American Continental Troposphere: Sources, Abundance, And Radiative Forcing, J. Liu, Eric Scheuer, Jack E. Dibb, G S. Diskin, L D. Ziemba, K L. Thornhill, B E. Anderson, A Whisthaler, T Mikoviny, J J. Devi, M Bergin, A E. Perring, M Z. Markovic, J P. Schwarz, P Campuzano-Jost, D A. Day, J L. Jimenez, R J. Weber Jul 2015

Brown Carbon Aerosol In The North American Continental Troposphere: Sources, Abundance, And Radiative Forcing, J. Liu, Eric Scheuer, Jack E. Dibb, G S. Diskin, L D. Ziemba, K L. Thornhill, B E. Anderson, A Whisthaler, T Mikoviny, J J. Devi, M Bergin, A E. Perring, M Z. Markovic, J P. Schwarz, P Campuzano-Jost, D A. Day, J L. Jimenez, R J. Weber

Earth Sciences

Chemical components of organic aerosol (OA) selectively absorb light at short wavelengths. In this study, the prevalence, sources, and optical importance of this so called brown carbon (BrC) aerosol component are investigated throughout the North American continental tropospheric column during a summer of extensive biomass burning. Spectrophotometric absorption measurements on extracts of bulk aerosol samples collected from an aircraft over the central USA were analyzed to directly quantify BrC abundance. BrC was found to be prevalent throughout the 1 to 12 km altitude measurement range, with dramatic enhancements in biomass-burning plumes. BrC to black carbon (BC) ratios, under background tropospheric …


Modeling Impacts Of Changes In Temperature And Water Table On C Gas Fluxes In An Alaskan Peatland, Jia Deng, Changsheng Li, Steve Frolking Jul 2015

Modeling Impacts Of Changes In Temperature And Water Table On C Gas Fluxes In An Alaskan Peatland, Jia Deng, Changsheng Li, Steve Frolking

Earth Sciences

Northern peatlands have accumulated a large amount of organic carbon (C) in their thick peat profile. Climate change and associated variations in soil environments are expected to have significant impacts on the C balance of these ecosystems, but the magnitude is still highly uncertain. Verifying and understanding the influences of changes in environmental factors on C gas fluxes in biogeochemical models are essential for forecasting feedbacks between C gas fluxes and climate change. In this study, we applied a biogeochemical model, DeNitrification-DeComposition (DNDC), to assess impacts of air temperature (TA) and water table (WT) on C gas fluxes …


The Polarcat Model Intercomparison Project (Polmip): Overview And Evaluation With Observations, L K. Emmons, S R. Arnold, S A. Monks, V Huijnen, S Tilmes, K S. Law, J L. Thomas, J C. Raut, I Bouarar, S Turquety, Y Long, B Duncan, S Steenrod, S Strode, J Flemming, J Mao, J Langner, A M. Thompson, D Tarasick, E C. Apel, D R. Blake, Robert C. Cohen, Jack E. Dibb, Glenn Diskin, A Fried, S R. Hall, L Gregory Huey, Andrew Weinheimer, Armin Wisthaler, Tomas Mikoviny, J Nowak, Jeff Peischl, J M. Roberts, Thomas B. Ryerson, C Warneke, D Helmig Jun 2015

The Polarcat Model Intercomparison Project (Polmip): Overview And Evaluation With Observations, L K. Emmons, S R. Arnold, S A. Monks, V Huijnen, S Tilmes, K S. Law, J L. Thomas, J C. Raut, I Bouarar, S Turquety, Y Long, B Duncan, S Steenrod, S Strode, J Flemming, J Mao, J Langner, A M. Thompson, D Tarasick, E C. Apel, D R. Blake, Robert C. Cohen, Jack E. Dibb, Glenn Diskin, A Fried, S R. Hall, L Gregory Huey, Andrew Weinheimer, Armin Wisthaler, Tomas Mikoviny, J Nowak, Jeff Peischl, J M. Roberts, Thomas B. Ryerson, C Warneke, D Helmig

Earth Sciences

A model intercomparison activity was inspired by the large suite of observations of atmospheric composition made during the International Polar Year (2008) in the Arctic. Nine global and two regional chemical transport models participated in this intercomparison and performed simulations for 2008 using a common emissions inventory to assess the differences in model chemistry and transport schemes. This paper summarizes the models and compares their simulations of ozone and its precursors and presents an evaluation of the simulations using a variety of surface, balloon, aircraft and satellite observations. Each type of measurement has some limitations in spatial or temporal coverage …


Revealing Important Nocturnal And Day-To-Day Variations In Fire Smoke Emissions Through A Multiplatform Inversion, Pablo E. Saide, David A. Peterson, Arlindo Da Silva, Bruce Anderson, Luke D. Ziemba, Glenn Diskin, Glen Sachse, Jonathan Hair, Carolyn Butler, Marta Fenn, Jose L. Jimenez, Pedro Campuzano-Jost, Anne E. Perring, Joshua P. Schwarz, Milos Z. Markovic, Phil Russell, Jens Redemann, Yohei Shinozuka, David G. Streets, Fang Yan, Jack E. Dibb, Robert Yokelson, O Brian Toon, Edward Hyer, Gregory R. Carmichael Jun 2015

Revealing Important Nocturnal And Day-To-Day Variations In Fire Smoke Emissions Through A Multiplatform Inversion, Pablo E. Saide, David A. Peterson, Arlindo Da Silva, Bruce Anderson, Luke D. Ziemba, Glenn Diskin, Glen Sachse, Jonathan Hair, Carolyn Butler, Marta Fenn, Jose L. Jimenez, Pedro Campuzano-Jost, Anne E. Perring, Joshua P. Schwarz, Milos Z. Markovic, Phil Russell, Jens Redemann, Yohei Shinozuka, David G. Streets, Fang Yan, Jack E. Dibb, Robert Yokelson, O Brian Toon, Edward Hyer, Gregory R. Carmichael

Earth Sciences

We couple airborne, ground-based, and satellite observations; conduct regional simulations; and develop and apply an inversion technique to constrain hourly smoke emissions from the Rim Fire, the third largest observed in California, USA. Emissions constrained with multiplatform data show notable nocturnal enhancements (sometimes over a factor of 20), correlate better with daily burned area data, and are a factor of 2-4 higher than a priori estimates, highlighting the need for improved characterization of diurnal profiles and day-to-day variability when modeling extreme fires. Constraining only with satellite data results in smaller enhancements mainly due to missing retrievals near the emissions source, …


Evolution Of Brown Carbon In Wildfire Plumes, Haviland Forrister, Jiumeng Liu, Jack E. Dibb, Eric Scheuer, Luke D. Ziemba, Kenn L. Thornhill, Bruce Anderson, Glenn Diskin, Anne E. Perring, Joshua P. Schwarz, Pedro Campuzano-Jost, Douglas A. Day, Brett B. Palm, Jose L. Jimenez, Athanasios Nenes, Rodney J. Weber Jun 2015

Evolution Of Brown Carbon In Wildfire Plumes, Haviland Forrister, Jiumeng Liu, Jack E. Dibb, Eric Scheuer, Luke D. Ziemba, Kenn L. Thornhill, Bruce Anderson, Glenn Diskin, Anne E. Perring, Joshua P. Schwarz, Pedro Campuzano-Jost, Douglas A. Day, Brett B. Palm, Jose L. Jimenez, Athanasios Nenes, Rodney J. Weber

Earth Sciences

Particulate brown carbon (BrC) in the atmosphere absorbs light at subvisible wavelengths and has poorly constrained but potentially large climate forcing impacts. BrC from biomass burning has virtually unknown lifecycle and atmospheric stability. Here, BrC emitted from intense wildfires was measured in plumes transported over 2 days from two main fires, during the 2013 NASA SEAC4RS mission. Concurrent measurements of organic aerosol (OA) and black carbon (BC) mass concentration, BC coating thickness, absorption Ångström exponent, and OA oxidation state reveal that the initial BrC emitted from the fires was largely unstable. Using back trajectories to estimate the transport time indicates …


Simulating Ice Core 10be On The Glacial–Interglacial Timescale, C Elsasser, D Wagenbach, I Levin, A Stanzick, Mark J. Christl, A Wallner, S Kipfstuhl, I K. Seietstad, H Wershofen, Jack E. Dibb Feb 2015

Simulating Ice Core 10be On The Glacial–Interglacial Timescale, C Elsasser, D Wagenbach, I Levin, A Stanzick, Mark J. Christl, A Wallner, S Kipfstuhl, I K. Seietstad, H Wershofen, Jack E. Dibb

Earth Sciences

10Be ice core measurements are an important tool for paleoclimate research, e.g., allowing for the reconstruction of past solar activity or changes in the geomagnetic dipole field. However, especially on multi-millennial timescales, the share of production and climate-induced variations of respective 10Be ice core records is still up for debate. Here we present the first quantitative climatological model of the 10Be ice concentration up to the glacial–interglacial timescale. The model approach is composed of (i) a coarse resolution global atmospheric transport model and (ii) a local 10Be air–firn transfer model. Extensive global-scale observational data of short-lived …