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Full-Text Articles in Physical Sciences and Mathematics

Arctic Air Pollution: New Insights From Polarcat-Ipy, Katherine S. Law, Andreas Stohl, Patricia K. Quinn, Charles A. Brock, John F. Burkhart, Jean-Daniel Paris, Gerard Ancellet, Hanwant B. Singh, Anke Roiger, Hans Schlager, Jack E. Dibb, Daniel J. Jacob, S R. Arnold, Jacques Pelon, Jennie L. Thomas Dec 2014

Arctic Air Pollution: New Insights From Polarcat-Ipy, Katherine S. Law, Andreas Stohl, Patricia K. Quinn, Charles A. Brock, John F. Burkhart, Jean-Daniel Paris, Gerard Ancellet, Hanwant B. Singh, Anke Roiger, Hans Schlager, Jack E. Dibb, Daniel J. Jacob, S R. Arnold, Jacques Pelon, Jennie L. Thomas

Earth Sciences

Given the rapid nature of climate change occurring in the Arctic and the difficulty climate models have in quantitatively reproducing observed changes such as sea ice loss, it is important to improve understanding of the processes leading to climate change in this region, including the role of short-lived climate pollutants such as aerosols and ozone. It has long been known that pollution produced from emissions at midlatitudes can be transported to the Arctic, resulting in a winter/spring aerosol maximum known as Arctic haze. However, many uncertainties remain about the composition and origin of Arctic pollution throughout the troposphere; for example, …


Assessing Effects Of Permafrost Thaw On C Fluxes Based On Multiyear Modeling Across A Permafrost Thaw Gradient At Stordalen, Sweden, Jia Deng, C Li, Steve Frolking, Y Zhang, K Backstrand, P Crill Aug 2014

Assessing Effects Of Permafrost Thaw On C Fluxes Based On Multiyear Modeling Across A Permafrost Thaw Gradient At Stordalen, Sweden, Jia Deng, C Li, Steve Frolking, Y Zhang, K Backstrand, P Crill

Earth Sciences

Northern peatlands in permafrost regions contain a large amount of organic carbon (C) in the soil. Climate warming and associated permafrost degradation are expected to have significant impacts on the C balance of these ecosystems, but the magnitude is uncertain. We incorporated a permafrost model, Northern Ecosystem Soil Temperature (NEST), into a biogeochemical model, DeNitrificationDeComposition (DNDC), to model C dynamics in highlatitude peatland ecosystems. The enhanced model was applied to assess effects of permafrost thaw on C fluxes of a subarctic peatland at Stordalen, Sweden. DNDC simulated soil freeze–thaw dynamics, net ecosystem exchange of CO2 (NEE), and CH4 fluxes across …


Atmospheric Oxidation Chemistry And Ozone Production: Results From Sharp 2009 In Houston, Texas, Katherine A. Duderstadt, Jack E. Dibb, Charles H. Jackman, Cora E. Randall, Stanley C. Solomon, Michael J. Mills, Nathan A. Schwadron, Harlan E. Spence Jun 2014

Atmospheric Oxidation Chemistry And Ozone Production: Results From Sharp 2009 In Houston, Texas, Katherine A. Duderstadt, Jack E. Dibb, Charles H. Jackman, Cora E. Randall, Stanley C. Solomon, Michael J. Mills, Nathan A. Schwadron, Harlan E. Spence

Earth Sciences

This study considers whether spikes in nitrate in snow sampled at Summit, Greenland, from August 2000 to August 2002 are related to solar proton events. After identifying tropospheric sources of nitrate on the basis of correlations with sulfate, ammonium, sodium, and calcium, we use the three-dimensional global Whole Atmosphere Community Climate Model (WACCM) to examine unaccounted for nitrate spikes. Model calculations confirm that solar proton events significantly impact HOx, NOx, and O3 levels in the mesosphere and stratosphere during the weeks and months following the major 9 November 2000 solar proton event. However, solar proton event (SPE)-enhanced NOy calculated within …


Intercomparison Of Field Measurements Of Nitrous Acid (Hono) During The Sharp Campaign, J R. Pinto, Jack E. Dibb, B H. Lee, B Rappengluck, E C. Wood, M Levy, R Y. Zhang, Barry Lefer, Xinrong Ren, J Stutz, C Tsai, L Ackermann, J Golovko, S C. Herndon, M Oakes, Q Y. Meng, J W. Munger, M Zahniser, J Zheng May 2014

Intercomparison Of Field Measurements Of Nitrous Acid (Hono) During The Sharp Campaign, J R. Pinto, Jack E. Dibb, B H. Lee, B Rappengluck, E C. Wood, M Levy, R Y. Zhang, Barry Lefer, Xinrong Ren, J Stutz, C Tsai, L Ackermann, J Golovko, S C. Herndon, M Oakes, Q Y. Meng, J W. Munger, M Zahniser, J Zheng

Earth Sciences

Because of the importance of HONO as a radical reservoir, consistent and accurate measurements of its concentration are needed. As part of SHARP (Study of Houston Atmospheric Radical Precursors), time series of HONO were obtained by six different measurement techniques on the roof of the Moody Tower at the University of Houston. Techniques used were long path differential optical absorption spectroscopy (DOAS), stripping coil-visible absorption photometry (SC-AP), long path absorption photometry (LOPAP® ), mist chamber/ion chromatography (MC-IC), quantum cascade-tunable infrared laser differential absorption spectroscopy (QC-TILDAS), and ion drift-chemical ionization mass spectrometry (ID-CIMS). Various combinations of techniques were in operation from …


Brown Carbon In The Continental Troposphere, Jiumeng Liu, Eric Scheuer, Jack E. Dibb, Luke D. Ziemba, Kenn L. Thornhill, Bruce Anderson, Armin Wisthaler, Tomas Mikoviny, J J. Devi, Mike Bergin, Rodney J. Weber Apr 2014

Brown Carbon In The Continental Troposphere, Jiumeng Liu, Eric Scheuer, Jack E. Dibb, Luke D. Ziemba, Kenn L. Thornhill, Bruce Anderson, Armin Wisthaler, Tomas Mikoviny, J J. Devi, Mike Bergin, Rodney J. Weber

Earth Sciences

No abstract provided.


Mercury Speciation At A Coastal Site In The Northern Gulf Of Mexico: Results From The Grand Bay Intensive Studies In Summer 2010 And Spring 2011, Xinrong Ren, Winston T. Luke, Paul Kelley, Mark Cohen, Fong Ngan, Richard Artz, Jake Walker, Steve Brooks, Christopher Moore, Phil Swartzendruber, Dieter Bauer, James Remeika, Anthony Hynes, Jack E. Dibb, John Rolison, Nishanth Krishnamurthy, William M. Landing, Arsineh Hecobian, Jeffery Shook, L Gregory Huey Apr 2014

Mercury Speciation At A Coastal Site In The Northern Gulf Of Mexico: Results From The Grand Bay Intensive Studies In Summer 2010 And Spring 2011, Xinrong Ren, Winston T. Luke, Paul Kelley, Mark Cohen, Fong Ngan, Richard Artz, Jake Walker, Steve Brooks, Christopher Moore, Phil Swartzendruber, Dieter Bauer, James Remeika, Anthony Hynes, Jack E. Dibb, John Rolison, Nishanth Krishnamurthy, William M. Landing, Arsineh Hecobian, Jeffery Shook, L Gregory Huey

Earth Sciences

During two intensive studies in summer 2010 and spring 2011, measurements of mercury species including gaseous elemental mercury (GEM), gaseous oxidized mercury (GOM), and particulate-bound mercury (PBM), trace chemical species including O3, SO2, CO, NO, NOY, and black carbon, and meteorological parameters were made at an Atmospheric Mercury Network (AMNet) site at the Grand Bay National Estuarine Research Reserve (NERR) in Moss Point, Mississippi. Surface measurements indicate that the mean mercury concentrations were 1.42 ± 0.12 ng∙m−3 for GEM, 5.4 ± 10.2 pg∙m−3 for GOM, and 3.1 ± 1.9 pg∙m−3 for …