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Articles 1 - 9 of 9
Full-Text Articles in Physical Sciences and Mathematics
A New Interpretation Of Total Column Bro During Arctic Spring, R J. Salawitch, T Canty, T P. Kurosu, K Chance, Q Liang, Arlindo Da Silva, S Pawson, J E. Neilsen, J. V. Rodriguez, P K. Bhartia, X Liu, L Gregory Huey, J Liao, R E. Stickel, D Tanner, Jack E. Dibb, W R. Simpson, D Donohue, Andrew Weinheimer, F Flocke, D Knapp, D Montzka, J A. Neuman, J Nowak, Thomas B. Ryerson, S J. Oltmans, D R. Blake, E L. Atlas, D Kinnison, S Tilmes, L L. Pan, F Hendrick, R Bradley Pierce, M Van Roozendael, K Kreher, P V. Johnston, R S. Gao, B Johnson, T P. Bui, G Chen, R B. Pierce, J H. Crawford, D J. Jacob
A New Interpretation Of Total Column Bro During Arctic Spring, R J. Salawitch, T Canty, T P. Kurosu, K Chance, Q Liang, Arlindo Da Silva, S Pawson, J E. Neilsen, J. V. Rodriguez, P K. Bhartia, X Liu, L Gregory Huey, J Liao, R E. Stickel, D Tanner, Jack E. Dibb, W R. Simpson, D Donohue, Andrew Weinheimer, F Flocke, D Knapp, D Montzka, J A. Neuman, J Nowak, Thomas B. Ryerson, S J. Oltmans, D R. Blake, E L. Atlas, D Kinnison, S Tilmes, L L. Pan, F Hendrick, R Bradley Pierce, M Van Roozendael, K Kreher, P V. Johnston, R S. Gao, B Johnson, T P. Bui, G Chen, R B. Pierce, J H. Crawford, D J. Jacob
Earth Sciences
Emission of bromine from sea-salt aerosol, frost flowers, ice leads, and snow results in the nearly complete removal of surface ozone during Arctic spring. Regions of enhanced total column BrO observed by satellites have traditionally been associated with these emissions. However, airborne measurements of BrO and O3 within the convective boundary layer (CBL) during the ARCTAS and ARCPAC field campaigns at times bear little relation to enhanced column BrO. We show that the locations of numerous satellite BrO “hotspots” during Arctic spring are consistent with observations of total column ozone and tropopause height, suggesting a stratospheric origin to these …
Bromide And Other Ions In The Snow, Firn Air, And Atmospheric Boundary Layer At Summit During Gshox, Jack E. Dibb, Luke D. Ziemba, J Luxford, P Beckman
Bromide And Other Ions In The Snow, Firn Air, And Atmospheric Boundary Layer At Summit During Gshox, Jack E. Dibb, Luke D. Ziemba, J Luxford, P Beckman
Earth Sciences
Measurements of gas phase soluble bromide in the boundary layer and in firn air, and Br− in aerosol and snow, were made at Summit, Greenland (72.5° N, 38.4° W, 3200 m a.s.l.) as part of a larger investigation into the influence of Br chemistry on HOx cycling. The soluble bromide measurements confirm that photochemical activation of Br− in the snow causes release of active Br to the overlying air despite trace concentrations of Br− in the snow (means 15 and 8 nmol Br− kg−1 of snow in 2007 and 2008, respectively). Mixing ratios of …
The Production And Persistence Of Σrono2 In The Mexico City Plume, A E. Perring, T H. Bertram, D K. Farmer, Paul J. Wooldridge, Jack E. Dibb, N J. Blake, D R. Blake, H B. Singh, H Fuelberg, Glenn Diskin, G W. Sachse, Robert C. Cohen
The Production And Persistence Of Σrono2 In The Mexico City Plume, A E. Perring, T H. Bertram, D K. Farmer, Paul J. Wooldridge, Jack E. Dibb, N J. Blake, D R. Blake, H B. Singh, H Fuelberg, Glenn Diskin, G W. Sachse, Robert C. Cohen
Earth Sciences
Alkyl and multifunctional nitrates (RONO2, ΣANs) have been observed to be a significant fraction of NOy in a number of different chemical regimes. Their formation is an important free radical chain termination step ending production of ozone and possibly affecting formation of secondary organic aerosol. ΣANs also represent a potentially large, unmeasured contribution to OH reactivity and are a major pathway for the removal of nitrogen oxides from the atmosphere. Numerous studies have investigated the role of nitrate formation from biogenic compounds and in the remote atmosphere. Less attention has been paid to the role ΣANs may …
Synthesis Of Satellite (Modis), Aircraft (Icartt), And Surface (Improve, Epa-Aqs, Aeronet) Aerosol Observations Over Eastern North America To Improve Modis Aerosol Retrievals And Constrain Surface Aerosol Concentrations And Sources, Easan Drury, Daniel J. Jacob, Robert J.D. Spurr, Jun Wang, Yohei Shinozuka, Bruce E. Anderson, A D. Clarke, Jack E. Dibb, Cameron Mcnaughton, Rodney J. Weber
Synthesis Of Satellite (Modis), Aircraft (Icartt), And Surface (Improve, Epa-Aqs, Aeronet) Aerosol Observations Over Eastern North America To Improve Modis Aerosol Retrievals And Constrain Surface Aerosol Concentrations And Sources, Easan Drury, Daniel J. Jacob, Robert J.D. Spurr, Jun Wang, Yohei Shinozuka, Bruce E. Anderson, A D. Clarke, Jack E. Dibb, Cameron Mcnaughton, Rodney J. Weber
Earth Sciences
We use an ensemble of satellite (MODIS), aircraft, and ground-based aerosol observations during the ICARTT field campaign over eastern North America in summer 2004 to (1) examine the consistency between different aerosol measurements, (2) evaluate a new retrieval of aerosol optical depths (AODs) and inferred surface aerosol concentrations (PM2.5) from the MODIS satellite instrument, and (3) apply this collective information to improve our understanding of aerosol sources. The GEOS-Chem global chemical transport model (CTM) provides a transfer platform between the different data sets, allowing us to evaluate the consistency between different aerosol parameters observed at different times and …
The Arctic Research Of The Composition Of The Troposphere From Aircraft And Satellites (Arctas) Mission: Design, Execution, And First Results, D J. Jacob, J H. Crawford, H Maring, A D. Clarke, Jack E. Dibb, L K. Emmons, R A. Ferrare, C A. Hostetler, Phil Russell, H B. Singh, A M. Thompson, G E. Shaw, E Mccauley, Judith Pederson, Jenny Fisher
The Arctic Research Of The Composition Of The Troposphere From Aircraft And Satellites (Arctas) Mission: Design, Execution, And First Results, D J. Jacob, J H. Crawford, H Maring, A D. Clarke, Jack E. Dibb, L K. Emmons, R A. Ferrare, C A. Hostetler, Phil Russell, H B. Singh, A M. Thompson, G E. Shaw, E Mccauley, Judith Pederson, Jenny Fisher
Earth Sciences
The NASA Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) mission was conducted in two 3-week deployments based in Alaska (April 2008) and western Canada (June–July 2008). Its goal was to better understand the factors driving current changes in Arctic atmospheric composition and climate, including (1) influx of mid-latitude pollution, (2) boreal forest fires, (3) aerosol radiative forcing, and (4) chemical processes. The June–July deployment was preceded by one week of flights over California (ARCTAS-CARB) focused on (1) improving state emission inventories for greenhouse gases and aerosols, (2) providing observations to test and improve models …
Convective Distribution Of Tropospheric Ozone And Tracers In The Central American Itcz Region: Evidence From Observations During Tc4, M A. Avery, Cynthia Twohy, David Mccabe, J Joiner, Kurt Severance, E L. Atlas, D R. Blake, T P. Bui, John D. Crounse, Jack E. Dibb, Glenn Diskin, Paul Lawson, Matthew Mcgill, David Rogers, G W. Sachse, Eric Scheuer, A M. Thompson, Charles Trepte, Paul Wennberg, Jerald Ziemke
Convective Distribution Of Tropospheric Ozone And Tracers In The Central American Itcz Region: Evidence From Observations During Tc4, M A. Avery, Cynthia Twohy, David Mccabe, J Joiner, Kurt Severance, E L. Atlas, D R. Blake, T P. Bui, John D. Crounse, Jack E. Dibb, Glenn Diskin, Paul Lawson, Matthew Mcgill, David Rogers, G W. Sachse, Eric Scheuer, A M. Thompson, Charles Trepte, Paul Wennberg, Jerald Ziemke
Earth Sciences
During the Tropical Composition, Clouds and Climate Coupling (TC4) experiment that occurred in July and August of 2007, extensive sampling of active convection in the ITCZ region near Central America was performed from multiple aircraft and satellite sensors. As part of a sampling strategy designed to study cloud processes, the NASA ER‐2, WB‐57 and DC‐8 flew in stacked “racetrack patterns” in convective cells. On July 24, 2007, the ER‐2 and DC‐8 probed an actively developing storm and the DC‐8 was hit by lightning. Case studies of this flight, and of convective outflow on August 5, 2007 reveal a significant anti‐correlation …
Evidence Of Nitric Acid Uptake In Warm Cirrus Anvil Clouds During The Nasa Tc4 Campaign, Eric Scheuer, Jack E. Dibb, Cynthia Twohy, David Rogers, Andrew J. Heymsfield, Aaron Bansemer
Evidence Of Nitric Acid Uptake In Warm Cirrus Anvil Clouds During The Nasa Tc4 Campaign, Eric Scheuer, Jack E. Dibb, Cynthia Twohy, David Rogers, Andrew J. Heymsfield, Aaron Bansemer
Earth Sciences
Uptake of HNO3 onto cirrus ice may play an important role in tropospheric NOx cycling. Discrepancies between modeled and in situ measurements of gas-phase HNO3 in the troposphere suggest that redistribution and removal mechanisms by cirrus ice have been poorly constrained. Limited in situ measurements have provided somewhat differing results and are not fully compatible with theory developed from laboratory studies. We present new airborne measurements of HNO3 in cirrus clouds from anvil outflow made during the Tropical Composition, Cloud, and Climate Coupling Experiment (TC4). Upper tropospheric (>9 km) measurements made during three flights while repeatedly traversing the same …
Impact Of Mineral Dust On Nitrate, Sulfate, And Ozone In Transpacific Asian Pollution Plumes, T D. Fairlie, D J. Jacob, Jack E. Dibb, B Alexander, M A. Avery, Aaron Van Donkelaar, L Zhang
Impact Of Mineral Dust On Nitrate, Sulfate, And Ozone In Transpacific Asian Pollution Plumes, T D. Fairlie, D J. Jacob, Jack E. Dibb, B Alexander, M A. Avery, Aaron Van Donkelaar, L Zhang
Earth Sciences
We use a 3-D global chemical transport model (GEOS-Chem) to interpret aircraft observations of nitrate and sulfate partitioning in transpacific dust plumes during the INTEX-B campaign of April–May 2006. The model includes explicit transport of size-resolved mineral dust and its alkalinity, nitrate, and sulfate content. The observations show that particulate nitrate is primarily associated with dust, sulfate is primarily associated with ammonium, and Asian dust remains alkaline across the Pacific. This can be reproduced in the model by using a reactive uptake coefficient for HNO3 on dust (γ(HNO3) ~10−3) much lower than commonly assumed in …
A Regional Scale Modeling Analysis Of Aerosol And Trace Gas Distributions Over The Eastern Pacific During The Intex-B Field Campaign, B Adhikary, Gregory R. Carmichael, S Kulkarni, C Wei, Y Tang, A D'Allura, M Mena-Carrasco, David G. Streets, Q Zhang, R B. Pierce, J Al-Saadi, L K. Emmons, G G. Pfister, M A. Avery, J D. Barrick, D R. Blake, William H. Brune, Robert C. Cohen, Jack E. Dibb, A Fried, B J. Heikes, L Gregory Huey, D W. O'Sullivan, G W. Sachse, R E. Shetter, H B. Singh, T L. Campos, C A. Cantrell, F Flocke, E J. Dunlea, Jose L. Jimenez, Andrew Weinheimer, John D. Crounse, Paul Wennberg, James J. Schauer, E A. Stone, D A. Jaffe, D R. Reidmiller
A Regional Scale Modeling Analysis Of Aerosol And Trace Gas Distributions Over The Eastern Pacific During The Intex-B Field Campaign, B Adhikary, Gregory R. Carmichael, S Kulkarni, C Wei, Y Tang, A D'Allura, M Mena-Carrasco, David G. Streets, Q Zhang, R B. Pierce, J Al-Saadi, L K. Emmons, G G. Pfister, M A. Avery, J D. Barrick, D R. Blake, William H. Brune, Robert C. Cohen, Jack E. Dibb, A Fried, B J. Heikes, L Gregory Huey, D W. O'Sullivan, G W. Sachse, R E. Shetter, H B. Singh, T L. Campos, C A. Cantrell, F Flocke, E J. Dunlea, Jose L. Jimenez, Andrew Weinheimer, John D. Crounse, Paul Wennberg, James J. Schauer, E A. Stone, D A. Jaffe, D R. Reidmiller
Earth Sciences
The Sulfur Transport and dEposition Model (STEM) is applied to the analysis of observations obtained during the Intercontinental Chemical Transport Experiment-Phase B (INTEX-B), conducted over the eastern Pacific Ocean during spring 2006. Predicted trace gas and aerosol distributions over the Pacific are presented and discussed in terms of transport and source region contributions. Trace species distributions show a strong west (high) to east (low) gradient, with the bulk of the pollutant transport over the central Pacific occurring between ∼20° N and 50° N in the 2-6 km altitude range. These distributions are evaluated in the eastern Pacific by comparison with …