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Full-Text Articles in Physical Sciences and Mathematics

Long-Term Trends And Variability Of Pm₂.₅ Mass, Chemical Components, And Sources Over Nys, Hesham Abdelmonem Hassan May 2022

Long-Term Trends And Variability Of Pm₂.₅ Mass, Chemical Components, And Sources Over Nys, Hesham Abdelmonem Hassan

Legacy Theses & Dissertations (2009 - 2024)

Eighteen years of ambient PM2.5 mass and major components are used in this study to harmonize the carbonaceous fraction of PM2.5 data, and to examine long-term trends and seasonal variability changes. The major decreasing trend of PM2.5 mass and major inorganic ions reflects the ambient concentration response to clean air regulations and policies.Although elemental carbon shows a decreasing trend in agreement with most other PM2.5 components, organic carbon shows a different behavior of no-trend to slightly increasing trend in some sites. Organic carbon behavior indicates the growing role of non-combustion sources at the expense of decreasing combustion sources. Seasonal trends …


Aerosol And Terrain Effects On Winter Cloud And Precipitation Over New York State, Yuyi Du Jan 2021

Aerosol And Terrain Effects On Winter Cloud And Precipitation Over New York State, Yuyi Du

Legacy Theses & Dissertations (2009 - 2024)

Prediction of regional weather and climate regarding precipitation for a region such as the Northeast US with its complex terrain and aerosol environment constitutes a major challenge. Furthermore, complex thermodynamic structures occur in and around New York State (NYS) owing to its complex topography paired with its coastal regions, ultimately affecting cloud and precipitation microphysics. The microphysical processes within the weather systems that produce orographic precipitation are not fully understood. These processes include, but are not limited to, liquid-ice interactions, ice growth through vapor deposition, riming, and aggregation, cloud-aerosol interactions, and melting and refreezing upon sedimentation to the surface. These …


Physical Characteristics And Microphysical Processing Of Atmospheric Aerosol In Rural And Urban New York State, Joseph Marto Jan 2021

Physical Characteristics And Microphysical Processing Of Atmospheric Aerosol In Rural And Urban New York State, Joseph Marto

Legacy Theses & Dissertations (2009 - 2024)

Atmospheric aerosol has profound impacts on air quality, though particles of differing sizes can have profoundly different characteristics which are understated when measurements are reported as a single parameter (typically number concentration or total mass). To address some of these concerns and to better understand the nature of atmospheric aerosol, continuous particle size distributions have been measured at two sites in New York State. Measurement was performed for particle diameters between 7.6nm - 20µm at Pinnacle State Park (Addison, New York; March 2017-April 2018) and Queens College (May 2018-September 2019) at a 5-minute time resolution. At Pinnacle State Park, aerosol …


The Role Of Ammonia In Atmospheric New Particle Formation And Implications For Cloud Condensation Nuclei, Arshad Arjunan Nair Jan 2021

The Role Of Ammonia In Atmospheric New Particle Formation And Implications For Cloud Condensation Nuclei, Arshad Arjunan Nair

Legacy Theses & Dissertations (2009 - 2024)

Atmospheric ammonia has received recent attention due to (a) its increasing trend across various regions of the globe; (b) the associated direct and indirect (through PM2.5) effects on human health, the ecosystem, and climate; and (c) recent evidence of its role in significantly enhancing atmospheric new particle formation (NPF or nucleation) rates. The mechanisms behind nucleation in the atmosphere are not fully understood, although over the last decade there have been significant developments in our understanding. This dissertation aims at improving our understanding of atmospheric ammonia in the atmosphere, its spatiotemporal variability, its role in atmospheric new particle formation, and …


An Overview Of Handheld Sun Photometer Measurements Of Atmospheric Aerosols In New Orleans, Louisiana: A Case Study Of The Xavier University Study Site., M. Bradley, B. Sevalia, M. Gasseller Jul 2019

An Overview Of Handheld Sun Photometer Measurements Of Atmospheric Aerosols In New Orleans, Louisiana: A Case Study Of The Xavier University Study Site., M. Bradley, B. Sevalia, M. Gasseller

Faculty and Staff Publications

Aerosol optical depth (AOT) was measured at Xavier University of Louisiana (XULA, 29.96ᵒ N, 90.11° W and 3m above sea level) using a GLOBE handheld sun photometer. The measurements were done at two different wavelengths, 505nm and 625nm. The measured values were used to extrapolate the AOT values for wavelengths 667nm, 551nm, 532nm and 490nm at the XULA site. The measured and calculated AOT values were then compared with values from the nearest AERONET station at Wave CIS site 6 (AERONET, 28.87ᵒ N, 90.48° W and 33m above sea level), which is 60 miles south of XULA. In this study …


Contrasting Local And Long-Range-Transported Warm Ice-Nucleating Particles During An Atmospheric River In Coastal California, Usa, Andrew C. Martin, Gavin Cornwell, Charlotte M. Beall, Forest Cannon, Sean Reilly, Bas Schapp, Dolan Lucero, Jessie Creamean, F. Martin Ralph, Hari T. Mix, Kimberly Prather Apr 2019

Contrasting Local And Long-Range-Transported Warm Ice-Nucleating Particles During An Atmospheric River In Coastal California, Usa, Andrew C. Martin, Gavin Cornwell, Charlotte M. Beall, Forest Cannon, Sean Reilly, Bas Schapp, Dolan Lucero, Jessie Creamean, F. Martin Ralph, Hari T. Mix, Kimberly Prather

Geography Faculty Publications and Presentations

Ice-nucleating particles (INPs) have been found to influence the amount, phase and efficiency of precipitation from winter storms, including atmospheric rivers. Warm INPs, those that initiate freezing at temperatures warmer than −10ºC, are thought to be particularly impactful because they can create primary ice in mixed-phase clouds, enhancing precipitation efficiency. The dominant sources of warm INPs during atmospheric rivers, the role of meteorology in modulating transport and injection of warm INPs into atmospheric river clouds, and the impact of warm INPs on mixed-phase cloud properties are not well-understood. In this case study, time-resolved precipitation samples were collected during an atmospheric …


Characterization Of Ambient Aerosols And Their Evolution Under Various Atmospheric Conditions In The Northeast U.S, Jie Zhang Jan 2019

Characterization Of Ambient Aerosols And Their Evolution Under Various Atmospheric Conditions In The Northeast U.S, Jie Zhang

Legacy Theses & Dissertations (2009 - 2024)

The University at Albany Atmospheric Sciences Research Center (ASRC) mobile laboratory, which includes a High Resolution Time-of-Flight Aerosol Mass Spectrometer (HR-ToF-AMS), a Scanning Mobility Particle Sizer (SMPS), and several gas sensors, etc., has been used to characterize atmospheric aerosols and air quality at different locations in the Northeastern US (including urban, forest, and mountain areas) and the aerosol evolutions under a variety of atmospheric conditions (including extreme weather, fog, and cloud, etc.). In this dissertation, I present the findings of the several field measurements using the ASRC mobile lab, focusing on the influences of extreme events (including high O3, heatwave, …


Classification Of Aerosol Population Type And Cloud Condensation Nuclei Properties In A Coastal California Littoral Environment Using An Unsupervised Cluster Model, Samuel A. Atwood, Sonia M. Kreidenweis, Paul J. Demott, Markus D. Petters, Gavin Cornwell, Andrew C. Martin, Kathryn A. Moore Jan 2019

Classification Of Aerosol Population Type And Cloud Condensation Nuclei Properties In A Coastal California Littoral Environment Using An Unsupervised Cluster Model, Samuel A. Atwood, Sonia M. Kreidenweis, Paul J. Demott, Markus D. Petters, Gavin Cornwell, Andrew C. Martin, Kathryn A. Moore

Geography Faculty Publications and Presentations

Aerosol particle and cloud condensation nuclei (CCN) measurements from a littoral location on the northern coast of California at Bodega Bay Marine Laboratory (BML) are presented for approximately six weeks of observations during the boreal winter–spring as part of the CalWater-2015 field campaign. The nature and variability of surface (marine boundary layer, MBL) aerosol populations were evaluated by classifying observations into periods of similar aerosol and meteorological characteristics using an unsupervised cluster model to derive distinct littoral aerosol population types and link them to source regions. Such classifications support efforts to understand the impact of changing aerosol properties on precipitation …


Statistical Analysis And Comparison Of Optical Classification Of Atmospheric Aerosol Lidar Data, Kwasi Gyening Afrifa May 2018

Statistical Analysis And Comparison Of Optical Classification Of Atmospheric Aerosol Lidar Data, Kwasi Gyening Afrifa

Electrical & Computer Engineering Projects for D. Eng. Degree

This dissertation presents a new study for the analysis and classification of atmospheric aerosols in remote sensing LIDAR data. Information on particle size and associated properties are extracted from these remote sensing atmospheric data which are collected by a ground-based LIDAR system. This study first considers optical LIDAR parameter-based classification methods for clustering and classification of different types of harmful aerosol particles in the atmosphere. Since accurate methods for aerosol prediction behaviors are based upon observed data, computational approaches must overcome design limitations, and also consider appropriate calibration and estimation accuracy. Consequently, two statistical methods based on generalized linear models …


Aerosol Direct Radiative And Cloud Adjustment Effects On Surface Climate Over The Eastern China : Analyses Of Wrf Model Simulations, Yangyang Song Jan 2018

Aerosol Direct Radiative And Cloud Adjustment Effects On Surface Climate Over The Eastern China : Analyses Of Wrf Model Simulations, Yangyang Song

Legacy Theses & Dissertations (2009 - 2024)

Aerosol climate effects consist of the initial forcing of atmospheric radiation perturbation through both the direct radiative effect and the modulation of radiatively-important cloud microphysics, and the subsequent changes in meteorology that also affect cloud macro- and micro-physics. The aerosol-induced cloud adjustment therefore involves many couplings and interactions, and its quantitative evaluation requires the use of model simulations. This study uses WRF model simulated changes in clouds and meteorology due to anthropogenic aerosol increases (versus 1970s) for 2002−2008 summers over the eastern China to address two relevant issues: direct radiative vs. cloud adjustment effects, and their roles in affecting surface …


Dynamical Characteristics Of Atmospheric Aerosols Over Ig Region, Manish Sharma, Ramesh P. Singh, Rajesh Kumar May 2016

Dynamical Characteristics Of Atmospheric Aerosols Over Ig Region, Manish Sharma, Ramesh P. Singh, Rajesh Kumar

Mathematics, Physics, and Computer Science Faculty Articles and Research

The dynamical characteristics of atmospheric aerosols over the Indo-Gangetic (IG) region are primarily dependent on the geographical settings and meteorological conditions. Detailed analysis of multi satellite data and ground observations have been carried out over three different cities i.e. Kanpur, Greater Noida and Amritsar during 2010-2013. Level-3 Moderate Resolution Imaging Spectroradiometer (MODIS) terra daily global grid product with spatial resolution of 1° × 1° shows the mean AOD at 500 nm wavelength value of 0.73, 0.70 and 0.67 with the standard deviation of 0.43, 0.39 and 0.36 respectively over Amritsar, Greater Noida and Kanpur. Our detailed analysis shows characteristic behavior …


Retrival Of Atmospheric Aerosol Size Distributions Using Stochastic Particle Swarm Optimization, Benjamin D. Nault-Maurer Jan 2016

Retrival Of Atmospheric Aerosol Size Distributions Using Stochastic Particle Swarm Optimization, Benjamin D. Nault-Maurer

All College Thesis Program, 2016-2019

A stochastic particle swarm optimization (SPSO) technique’s robustness is studied in regards to atmospheric aerosol size distribution estimations for a bimodal distribution that focuses on Aitken and accumulation mode aerosols. The SPSO method is used to calculate a set of 11 aerosol optical depth (AOD) values based on a size distribution and match them to an inputted set of AOD values. This method is tested using computer generated AOD values with fixed distribution parameters, generated AOD values with varying distribution parameters, two sets of AOD measurements in clear conditions, and one set of AOD values in hazy conditions. The SPSO …


Distinguishing Molecular Characteristics Of Aerosol Water Soluble Organic Matter From The 2011 Trans-North Atlantic Us Geotraces Cruise, A. S. Wozniak, A. S. Willoughby, S. C. Gurganus, Patrick G. Hatcher Jan 2014

Distinguishing Molecular Characteristics Of Aerosol Water Soluble Organic Matter From The 2011 Trans-North Atlantic Us Geotraces Cruise, A. S. Wozniak, A. S. Willoughby, S. C. Gurganus, Patrick G. Hatcher

Chemistry & Biochemistry Faculty Publications

The molecular characteristics of aerosol organic matter (OM) determines to a large extent its impacts on the atmospheric radiative budget and ecosystem function in terrestrial and aquatic environments, yet the OM molecular details of aerosols from different sources are not well established. Aerosol particulate samples with North American-influenced, North African-influenced, and marine (minimal recent continental influence) air mass back trajectories were collected as part of the 2011 trans-North Atlantic US GEOTRACES cruise and analyzed for their water soluble OM (WSOM) molecular characteristics using electrospray ionization Fourier transform ion cyclotron resonance mass spectrometry. Principal component analysis (PCA) separated the samples into …


A Molecular-Level Approach For Characterizing Water-Insoluble Components Of Ambient Organic Aerosol Particulates Using Ultrahigh-Resolution Mass Spectrometry, A. S. Willoughby, A. S. Wozniak, Patrick G. Hatcher Jan 2014

A Molecular-Level Approach For Characterizing Water-Insoluble Components Of Ambient Organic Aerosol Particulates Using Ultrahigh-Resolution Mass Spectrometry, A. S. Willoughby, A. S. Wozniak, Patrick G. Hatcher

Chemistry & Biochemistry Faculty Publications

The chemical composition of organic aerosols in the atmosphere is strongly influenced by human emissions. The effect these have on the environment, human health, and climate change is determined by the molecular nature of these chemical species. The complexity of organic aerosol samples limits the ability to study the chemical composition, and therefore the associated properties and the impacts they have. Many studies have addressed the watersoluble fraction of organic aerosols and have had much success in identifying specific molecular formulas for thousands of compounds present. However, little attention is given to the water-insoluble portion, which can contain most of …


Spatial And Seasonal Variability Of Cloud Condensation Nuclei Number Concentrations Over The Extended North African Continent And The Mediterranean, Hesham Abdel-Monem Afify Hassan Jan 2014

Spatial And Seasonal Variability Of Cloud Condensation Nuclei Number Concentrations Over The Extended North African Continent And The Mediterranean, Hesham Abdel-Monem Afify Hassan

Legacy Theses & Dissertations (2009 - 2024)

The spatiotemporal variability of cloud condensation nuclei (CCN) number concentration is investigated over the extended domain of the North African continent and Mediterranean which is an essential step for better understanding of aerosol-cloud interactions and associated climate impacts over the region. The study is performed by analyzing the output for the period from 2004 to 2011 from the well-validated global chemistry and aerosol transport model GEOS-Chem-APM. The analysis shows that the dominant aerosol type for CCN number concentration is secondary particles all over the domain. Spatial analysis reveals the existence of four characteristic subdomains of variability: over the Mediterranean and …


Solar Radiation Measurements And Their Applications In Climate Research, Bangsheng Yin Jan 2013

Solar Radiation Measurements And Their Applications In Climate Research, Bangsheng Yin

Legacy Theses & Dissertations (2009 - 2024)

Aerosols and clouds play important roles in the climate system through their radiative effects and their vital link in the hydrological cycle. Accurate measurements of aerosol and cloud optical and microphysical properties are crucial for the study of climate and climate change. This study develops/improves retrieval algorithms for aerosol single scattering albedo (SSA) and low liquid water path (LWP) cloud optical properties, evaluates a new spectrometer, and applies long-term measurements to establish climatology of aerosol and cloud optical properties. The following results were obtained.


Study Of Key Factors Influencing Dust Emission : An Assessment Of Geos-Chem And Dead Simulations With Observations, Kevin Scott Bartlett Jan 2013

Study Of Key Factors Influencing Dust Emission : An Assessment Of Geos-Chem And Dead Simulations With Observations, Kevin Scott Bartlett

Legacy Theses & Dissertations (2009 - 2024)

Mineral dust aerosols can impact air quality, climate change, biological cycles, tropical cyclone development and flight operations due to reduced visibility. Dust emissions are primarily limited to the extensive arid regions of the world, yet can negatively impact local to global scales, and are extremely complex to model accurately. Within this dissertation, the Dust Entrainment And Deposition (DEAD) model was adapted to run, for the first known time, using high temporal (hourly) and spatial (0.3°x0.3°) resolution data to methodically interrogate the key parameters and factors influencing global dust emissions. The dependence of dust emissions on key parameters under various conditions …


Research Poster: Measuring The Aerosol Asymmetry Parameter G Instrument Description And Initial Measurements, Guoxun Tian, Hans Moosmuller, W. Patrick Arnott Feb 2010

Research Poster: Measuring The Aerosol Asymmetry Parameter G Instrument Description And Initial Measurements, Guoxun Tian, Hans Moosmuller, W. Patrick Arnott

2010 Annual Nevada NSF EPSCoR Climate Change Conference

Research poster


Retrieval Of Atmospheric Elemental Carbon Records Using Lake Sediments : Implications In Radiative Forcing, Tanveer Ahmed Jan 2010

Retrieval Of Atmospheric Elemental Carbon Records Using Lake Sediments : Implications In Radiative Forcing, Tanveer Ahmed

Legacy Theses & Dissertations (2009 - 2024)

Elemental or black carbon (EC or BC) aerosols produced during incomplete combustion strongly absorb solar radiation and contribute to global warming, and cause cardiopulmonary disease. Long-term atmospheric EC measurements, [EC]atm, are needed to validate global climate models to estimate the impact of EC on earth's temperature. Such data is sparse.


Technical Note: Molecular Characterization Of Aerosol-Derived Water Soluble Organic Carbon Using Ultrahigh Resolution Electrospray Ionization Fourier Transform Ion Cyclotron Resonance Mass Spectrometry, A. S. Wozniak, J. E. Bauer, R. L. Sleighter, R. M. Dickhut, Patrick Hatcher Jan 2008

Technical Note: Molecular Characterization Of Aerosol-Derived Water Soluble Organic Carbon Using Ultrahigh Resolution Electrospray Ionization Fourier Transform Ion Cyclotron Resonance Mass Spectrometry, A. S. Wozniak, J. E. Bauer, R. L. Sleighter, R. M. Dickhut, Patrick Hatcher

Chemistry & Biochemistry Faculty Publications

Despite the acknowledged relevance of aerosol-derived water-soluble organic carbon (WSOC) to climate and biogeochemical cycling, characterization of aerosol WSOC has been limited. Electrospray ionization Fourier transform ion cyclotron resonance mass spectrometry (ESI FT-ICR MS) was utilized in this study to provide detailed molecular level characterization of the hi(,h molecular weight (HMW; m/z>223) component of aerosol-derived WSOC collected from rural sites in Virginia and New York, USA. More than 3000 peaks were detected by ESI FT-ICR MS within a m/z range of 223-600 for each sample. Approximately 86% (Virginia) and 78% (New York) of these peaks were assigned molecular formulas …