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Articles 1 - 5 of 5
Full-Text Articles in Physical Sciences and Mathematics
The Arctic Research Of The Composition Of The Troposphere From Aircraft And Satellites (Arctas) Mission: Design, Execution, And First Results, D J. Jacob, J H. Crawford, H Maring, A D. Clarke, J E. Dibb, L K. Emmons, R A. Ferrare, C A. Hostetler, P B. Russell, H B. Singh, A M. Thompson, G E. Shaw, E Mccauley, J R. Pederson, J A. Fisher
The Arctic Research Of The Composition Of The Troposphere From Aircraft And Satellites (Arctas) Mission: Design, Execution, And First Results, D J. Jacob, J H. Crawford, H Maring, A D. Clarke, J E. Dibb, L K. Emmons, R A. Ferrare, C A. Hostetler, P B. Russell, H B. Singh, A M. Thompson, G E. Shaw, E Mccauley, J R. Pederson, J A. Fisher
Jenny A Fisher
The NASA Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) mission was conducted in two 3-week deployments based in Alaska (April 2008) and western Canada (June–July 2008). Its goal was to better understand the factors driving current changes in Arctic atmospheric composition and climate, including (1) influx of mid-latitude pollution, (2) boreal forest fires, (3) aerosol radiative forcing, and (4) chemical processes. The June–July deployment was preceded by one week of flights over California (ARCTAS-CARB) focused on (1) improving state emission inventories for greenhouse gases and aerosols, (2) providing observations to test and improve models …
Sources, Distribution, And Acidity Of Sulfate-Ammonium Aerosol In The Arctic In Winter-Spring, Jenny A. Fisher, Daniel J. Jacob, Q Wang, Roya Bahreini, C C. Carouge, M J. Cubison, Jack E. Dibb, Thomas Diehl, J L. Jimenez, E M. Leibensperger, Zifeng Lu, Marcel B.J Meinders, H. O T. Pye, Patricia K. Quinn, Sangeeta Sharma, David G. Streets, Aaron Van Donkelaar, R M. Yantosca
Sources, Distribution, And Acidity Of Sulfate-Ammonium Aerosol In The Arctic In Winter-Spring, Jenny A. Fisher, Daniel J. Jacob, Q Wang, Roya Bahreini, C C. Carouge, M J. Cubison, Jack E. Dibb, Thomas Diehl, J L. Jimenez, E M. Leibensperger, Zifeng Lu, Marcel B.J Meinders, H. O T. Pye, Patricia K. Quinn, Sangeeta Sharma, David G. Streets, Aaron Van Donkelaar, R M. Yantosca
Jenny A Fisher
We use GEOS-Chem chemical transport model simulations of sulfate–ammonium aerosol data from the NASA ARCTAS and NOAA ARCPAC aircraft campaigns in the North American Arctic in April 2008, together with longer-term data from surface sites, to better understand aerosol sources in the Arctic in winter–spring and the implications for aerosol acidity. Arctic pollution is dominated by transport from mid-latitudes, and we test the relevant ammonia and sulfur dioxide emission inventories in the model by comparison with wet deposition flux data over the source continents. We find that a complicated mix of natural and anthropogenic sources with different vertical signatures is …
Sources Of Carbonaceous Aerosols And Deposited Black Carbon In The Arctic In Winter-Spring: Implications For Radiative Forcing, Q Wang, D J. Jacob, J A. Fisher, J Mao, E M. Leibensperger, C C. Carouge, P Le Sager, Y Kondo, J L. Jimenez, M J. Cubison, S J. Doherty
Sources Of Carbonaceous Aerosols And Deposited Black Carbon In The Arctic In Winter-Spring: Implications For Radiative Forcing, Q Wang, D J. Jacob, J A. Fisher, J Mao, E M. Leibensperger, C C. Carouge, P Le Sager, Y Kondo, J L. Jimenez, M J. Cubison, S J. Doherty
Jenny A Fisher
We use a global chemical transport model (GEOS-Chem CTM) to interpret observations of black carbon (BC) and organic aerosol (OA) from the NASA ARCTAS aircraft campaign over the North American Arctic in April 2008, as well as longer-term records in surface air and in snow (2007-2009). BC emission inventories for North America, Europe, and Asia in the model are tested by comparison with surface air observations over these source regions. Russian open fires were the dominant source of OA in the Arctic troposphere during ARCTAS but we find that BC was of prevailingly anthropogenic (fossil fuel and biofuel) origin, particularly …
Chemistry Of Hydrogen Oxide Radicals (Hox) In The Arctic Troposphere In Spring, J Mao, D J. Jacob, M J. Evans, J R. Olson, X Ren, W H. Brune, T M. St. Clair, J D. Crounse, K M. Spencer, M R. Beaver, P O. Wennberg, M J. Cubison, J L. Jimenez, A Fried, P Weibring, J G. Walega, S R. Hall, A J. Weinheimer, R C. Cohen, G Chen, J H. Crawford, C Mcnaughton, A D. Clarke, L Jaegle, Jenny A. Fisher, R M. Yantosca, P Le Sager, C C. Carouge
Chemistry Of Hydrogen Oxide Radicals (Hox) In The Arctic Troposphere In Spring, J Mao, D J. Jacob, M J. Evans, J R. Olson, X Ren, W H. Brune, T M. St. Clair, J D. Crounse, K M. Spencer, M R. Beaver, P O. Wennberg, M J. Cubison, J L. Jimenez, A Fried, P Weibring, J G. Walega, S R. Hall, A J. Weinheimer, R C. Cohen, G Chen, J H. Crawford, C Mcnaughton, A D. Clarke, L Jaegle, Jenny A. Fisher, R M. Yantosca, P Le Sager, C C. Carouge
Jenny A Fisher
We use observations from the April 2008 NASA ARCTAS aircraft campaign to the North American Arctic, interpreted with a global 3-D chemical transport model (GEOS-Chem), to better understand the sources and cycling of hydrogen oxide radicals (HOx≡H+OH+peroxy radicals) and their reservoirs (HOy≡HOx+peroxides) in the springtime Arctic atmosphere. We find that a standard gas-phase chemical mechanism overestimates the observed HO2 and H2O2 concentrations. Computation of HOx and HOy gas-phase chemical budgets on the basis of the aircraft observations also indicates a large missing sink for both. We hypothesize that this could reflect HO2 uptake by aerosols, favored by low temperatures and …
Source Attribution And Interannual Variability Of Arctic Pollution In Spring Constrained By Aircraft (Arctas, Arcpac) And Satellite (Airs) Observations Of Carbon Monoxide, J A. Fisher, D J. Jacob, M T. Purdy, M Kopacz, P Le Sager, C C. Carouge, C D. Holmes, R M. Yantosca, R L. Batchelor, K Strong, G S. Diskin, H E. Fuelberg, J S. Holloway, E J. Hyer, W. W Mcmillan, J Warner, D G. Streets, Q Zhang, Y Yang, S Wu
Source Attribution And Interannual Variability Of Arctic Pollution In Spring Constrained By Aircraft (Arctas, Arcpac) And Satellite (Airs) Observations Of Carbon Monoxide, J A. Fisher, D J. Jacob, M T. Purdy, M Kopacz, P Le Sager, C C. Carouge, C D. Holmes, R M. Yantosca, R L. Batchelor, K Strong, G S. Diskin, H E. Fuelberg, J S. Holloway, E J. Hyer, W. W Mcmillan, J Warner, D G. Streets, Q Zhang, Y Yang, S Wu
Jenny A Fisher
We use aircraft observations of carbon monoxide (CO) from the NASA ARCTAS and NOAA ARCPAC campaigns in April 2008 together with multiyear (2003– 2008) CO satellite data from the AIRS instrument and a global chemical transport model (GEOS-Chem) to better understand the sources, transport, and interannual variability of pollution in the Arctic in spring. Model simulation of the aircraft data gives best estimates of CO emissions in April 2008 of 26 Tg month−1 for Asian anthropogenic, 9.4 for European anthropogenic, 4.1 for North American anthropogenic, 15 for Russian biomass burning (anomalously large that year), and 23 for Southeast Asian biomass …