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Full-Text Articles in Physical Sciences and Mathematics
Atmospheric Chemistry Of A 33–34 Hour Old Volcanic Cloud From Hekla Volcano (Iceland): Insights From Direct Sampling And The Application Of Chemical Box Modeling, William I. Rose, Genevieve A. Millard, Tamsin A. Mather, Donald E. Hunton, Bruce Anderson, Clive Oppenheimer, Brett F. Thornton, Terrence M. Gerlach, Albert A. Viggiano, Yutaka Kondo, Thomas M. Miller, John O. Ballenthin
Atmospheric Chemistry Of A 33–34 Hour Old Volcanic Cloud From Hekla Volcano (Iceland): Insights From Direct Sampling And The Application Of Chemical Box Modeling, William I. Rose, Genevieve A. Millard, Tamsin A. Mather, Donald E. Hunton, Bruce Anderson, Clive Oppenheimer, Brett F. Thornton, Terrence M. Gerlach, Albert A. Viggiano, Yutaka Kondo, Thomas M. Miller, John O. Ballenthin
Department of Geological and Mining Engineering and Sciences Publications
On 28 February 2000, a volcanic cloud from Hekla volcano, Iceland, was serendipitously sampled by a DC-8 research aircraft during the SAGE III Ozone Loss and Validation Experiment (SOLVE I). It was encountered at night at 10.4 km above sea level (in the lower stratosphere) and 33–34 hours after emission. The cloud is readily identified by abundant SO2 (≤1 ppmv), HCl (≤70 ppbv), HF (≤60 ppbv), and particles (which may have included fine silicate ash). We compare observed and modeled cloud compositions to understand its chemical evolution. Abundances of sulfur and halogen species indicate some oxidation of sulfur gases but …
Halogen Emissions From A Small Volcanic Eruption: Modeling The Peak Concentrations, Dispersion, And Volcanically Induced Ozone Loss In The Stratosphere, G. A. Millard, T. A. Mather, D. M. Pyle, William I. Rose, B. Thornton
Halogen Emissions From A Small Volcanic Eruption: Modeling The Peak Concentrations, Dispersion, And Volcanically Induced Ozone Loss In The Stratosphere, G. A. Millard, T. A. Mather, D. M. Pyle, William I. Rose, B. Thornton
Department of Geological and Mining Engineering and Sciences Publications
Aircraft measurements in the Hekla, Iceland volcanic plume in February 2000 revealed large quantities of hydrogen halides within the stratosphere correlated to volcanic SO2. Investigation of the longer-term stratospheric impact of these emissions, using the 3D chemical transport model, SLIMCAT suggests that volcanic enhancements of H2O and HNO3 increased HNO3·3H2O particle availability within the plume. These particles activated volcanic HCl and HBr, enhancing model plume concentrations of ClOx (20 ppb) and BrOx (50 ppt). Model O3 concentrations decreased to near-zero in places, and plume average O3 remained 30% lower after two weeks. Reductions in the model O3column reduced UV shielding …
Effects Of Carbonation On The Mineral Composition Of Cement Kiln Dust, Cecilia P. Anderson
Effects Of Carbonation On The Mineral Composition Of Cement Kiln Dust, Cecilia P. Anderson
Dissertations, Master's Theses and Master's Reports - Open
Due to their relatively high calcium oxide content, industrial mineral oxide wastes are potential candidates for mineral sequestration of carbon dioxide (CO2). Cement kiln dust (CKD), a byproduct of cement manufacturing contains 20-60% CaO making it a possible candidate for CO2 sequestration. In this study, three types of CKD are characterized, before and after carbonation, using environmental scanning electron microscopy and energy dispersive x-ray microanalysis to determine the mineralogical and morphological changes occurring due to carbonation. The reactants, products, and precipitation mechanisms were investigated to enhance understanding of the governing processes and allow better utilization of CKD …
Carbon Dioxide Sequestration In Cement Kiln Dust Through Miner Carbonation, Deborah N. Huntzinger
Carbon Dioxide Sequestration In Cement Kiln Dust Through Miner Carbonation, Deborah N. Huntzinger
Dissertations, Master's Theses and Master's Reports - Open
The feasibility of carbon sequestration in cement kiln dust (CKD) was investigated in a series of batch and column experiments conducted under ambient temperature and pressure conditions. The significance of this work is the demonstration that alkaline wastes, such as CKD, are highly reactive with carbon dioxide (CO2). In the presence of water, CKD can sequester greater than 80% of its theoretical capacity for carbon without any amendments or modifications to the waste. Other mineral carbonation technologies for carbon sequestration rely on the use of mined mineral feedstocks as the source of oxides. The mining, pre-processing and reaction …
Analyzing The Effects Of Vertical Acceleration And Deceleration In Multi-Phase, Debris-Flow Sediment-Column Experiments / By Christine Marie Williams., Christine Marie Williams
Analyzing The Effects Of Vertical Acceleration And Deceleration In Multi-Phase, Debris-Flow Sediment-Column Experiments / By Christine Marie Williams., Christine Marie Williams
Dissertations, Master's Theses and Master's Reports - Open
Water-saturated debris flows are among some of the most destructive mass movements. Their complex nature presents a challenge for quantitative description and modeling. In order to improve understanding of the dynamics of these flows, it is important to seek a simplified dynamic system underlying their behavior. Models currently in use to describe the motion of debris flows employ depth-averaged equations of motion, typically assuming negligible effects from vertical acceleration. However, in many cases debris flows experience significant vertical acceleration as they move across irregular surfaces, and it has been proposed that friction associated with vertical forces and liquefaction merit inclusion …