Physical Sciences and Mathematics Commons^™

Hallmarks Of The Mott-Metal Crossover In The Hole-Doped Pseudospin-1/2 Mott Insulator Sr2Iro4, Yue Cao, Qiang Wang, Justin A. Waugh, Theodore J. Reber, Haoxiang Li, Xiaoqing Zhou, Stephen Parham, S. -R. Park, Nicholas C. Plumb, Eli Rotenberg, Aaron Bostwick, Jonathan D. Denlinger, Tongfei Qi, Michael A. Hermele, Gang Cao, Daniel S. Dessau

Physics and Astronomy Faculty Publications

The physics of doped Mott insulators remains controversial after decades of active research, hindered by the interplay among competing orders and fluctuations. It is thus highly desired to distinguish the intrinsic characters of the Mott-metal crossover from those of other origins. Here we investigate the evolution of electronic structure and dynamics of the hole-doped pseudospin-1/2 Mott insulator Sr₂IrO₄. The effective hole doping is achieved by replacing Ir with Rh atoms, with the chemical potential immediately jumping to or near the top of the lower Hubbard band. The doped iridates exhibit multiple iconic low-energy features previously observed …