Physical Sciences and Mathematics Commons^™

Probing Symmetry And Disorder Effects In The Fractional Quantum Hall States Of The Second Landau Level, Ethan I. Kleinbaum

Open Access Dissertations

Electrons confined to two dimensions, cooled to cryogenic temperatures, and placed in a strong perpendicular magnetic field exhibit a set of ground states referred to as the fractional quantum Hall states (FQHS). The FQHSs forming in the region called the second Landau level are some of the most exciting states as several theories predict that they are very different from the well understood FQHS in the lowest Landau level. Nonetheless, the nature of these FQHSs continue to evade understanding. In this thesis, a unique ultra-low temperature setup is used to examine the FQHSs of the second Landau level in regimes …

Localization And Delocalization In Two-Dimensional Quantum Percolation, Brianna S. Dillon Thomas

Open Access Dissertations

Quantum percolation is one of several disorder-only models that address the question of whether conduction, or more generally, delocalization, is possible in two dimensional disordered systems. Whether quantum percolation exhibits a delocalization-localization phase transition in two dimensions is an ongoing debate, but many recent studies point toward there being a delocalized phase at non-zero disorder, in contradiction to the behavior of the Anderson model, another disorder-only model. In this dissertation, I present my research on quantum percolation that shows a delocalized state is possible, both on isotropic lattices and on highly anisotropic lattices, and shows that the essential characteristics of …

Energy Transfer And Localization In Molecular Crystals, Mitchell A. Wood

Open Access Dissertations

With the aim of developing new technologies for the detection and defeat of energetic materials, this collection of work was focused on using simulations to characterize materials at extremes of temperature, pressure and radiation. Each branch of the work here is collected by which material response is potentially used as the detectable signal.

Where the chemical response is of interest, this work will explore the possibility of non-statistical chemical reactions in condensed-phase energetic materials via reactive molecular dynamics (MD) simulations. We characterize the response of three unique high energy density molecular crystals to different means of energy input: electric fields …

Fabrication And Photonics Properties Of Iii-V Semiconductor Nanowire Structures, Tzu-Ging Lin

Open Access Dissertations

III-V semiconductor nanowires (NWs) have shown great potential to be building blocks for optical, optoelectronic, and electronic devices due to their special transverse confinement of electrons and photons along the nanowire axis. In addition, semiconductor nanowires with subwavelength structures exhibit strong optical Mie resonance, making them ideal platforms for realizing novel optical devices, such as extreme solar energy absorbers and broadband light trapping devices. This special 1D optical Mie resonance can be enhanced by using semiconductor-core dielectric-shell (CS) and metal-core semiconductor-shell dielectric-outer shell (CSS) nanowire heterostructures. Those advantages can be even leveraged up by utilizing nanowire arrays, attributing to the …

Transport Studies In Graphene-Based Materials And Structures, Jiuning Hu

Open Access Dissertations

Graphene, a single atomic layer of graphite, has emerged as one of the most attractive materials in recent years for its many unique and excellent properties, inviting a broad area of fundamental studies and applications. In this thesis, we present some theoretical/experimental studies about the thermal, electronic and thermoelectric transport properties in graphene-based systems. We employ the molecular dynamic simulations to study the thermal transport in graphene nanoribbons (GNRs) exhibiting various properties, including chirality dependent thermal conductivity, thermal rectification in asymmetric GNRs, defects and isotopic engineering of the thermal conductivity and negative differential thermal conductance (NDTC) at large temperature biases. …

Growth Of Low Disorder Gaas/Algaas Heterostructures By Molecular Beam Epitaxy For The Study Of Correlated Electron Phases In Two Dimensions, John D. Watson

Open Access Dissertations

The unparalleled quality of GaAs/AlGaAs heterostructures grown by molecular beam epitaxy has enabled a wide range of experiments probing interaction effects in two-dimensional electron and hole gases. This dissertation presents work aimed at further understanding the key material-related issues currently limiting the quality of these 2D systems, particularly in relation to the fractional quantum Hall effect in the 2^nd Landau level and spin-based implementations of quantum computation.^ The manuscript begins with a theoretical introduction to the quantum Hall effect which outlines the experimental conditions necessary to study the physics of interest and motivates the use of the semiconductor growth …

Structural Characterization Of Multimetallic Nanoparticles, Vineetha Mukundan

Open Access Dissertations

Bimetallic and trimetallic alloy nanoparticles have enhanced catalytic activities due to their unique structural properties. Using in situ time-resolved synchrotron based x-ray diffraction, we investigated the structural properties of nanoscale catalysts undergoing various heat treatments. Thermal treatment brings about changes in particle size, morphology, dispersion of metals on support, alloying, surface electronic properties, etc. First, the mechanisms of coalescence and grain growth in PtNiCo nanoparticles supported on planar silica on silicon were examined in detail in the temperature range 400-900°C. The sintering process in PtNiCo nanoparticles was found to be accompanied by lattice contraction and L1₀chemical ordering. …

Transport Studies Of Reentrant Integer Quantum Hall States Forming In The Two-Dimensional Electron Gas, Nianpei Deng

Open Access Dissertations

The two dimensional electron gas subjected to a magnetic field has been a model system in contemporary condensed matter physics which generated many beautiful experiments as well as novel fundamental concepts. These novel concepts are of broad interests and have benefited other fields of research. For example, the observations of conventional odd-denominator fractional quantum Hall states have enriched many-body physics with important concepts such as fractional statistics and composite fermions. The subsequent discovery of the enigmatic even-denominator ν=5/2 fractional quantum Hall state has led to more interesting concepts such as non-Abelian statistics and pairing of composite fermions which can be …

Modeling The Atomic And Electronic Structure Of Metal-Metal, Metal-Semiconductor And Semiconductor-Oxide Interfaces, Ganesh Krishna Hegde

Open Access Dissertations

The continuous downward scaling of electronic devices has renewed attention on the importance of the role of material interfaces in the functioning of key components in electronic technology in recent times. It has also brought into focus the utility of

atomistic modeling in providing insights from a materials design perspective. In this thesis, a combination of Semi Empirical Tight-Binding (TB), first-principles Density

Functional Theory and Reactive Molecular Dynamics (MD) modeling is used to study aspects of the electronic and atomic structure of three such 'canonical' material interfaces - Metal-Metal, Metal-Semiconductor and Semiconductor oxide interfaces.

An important contribution of this thesis …

Characterization And Interactions Of Ultrafast Surface Plasmon Pulses, Sibel Ebru Yalcin

Open Access Dissertations

Surface Plasmon Polaritons (SPPs) are considered to be attractive components for plasmonics and nanophotonic devices due to their sensitivity to interface changes, and their ability to guide and confine light beyond the diffraction limit. They have been utilized in SPP resonance sensors and near field imaging techniques and, more recently, SPP experiments to monitor and control ultrafast charge carrier and energy relaxation dynamics in thin films. In this thesis, we discuss excitation and propagation properties of ultrafast SPPs on thin extended metal films and SPP waveguide structures. In addition, localized and propagating surface plasmon interactions in functional plasmonic nanostructures will …