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Physical Sciences and Mathematics Commons™
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Full-Text Articles in Physical Sciences and Mathematics
First Results From The High-Brightness X-Ray Spectroscopy Beamline 9.3.1 At Als, W. Ng, G. Jones, Rupert C. Perera, D. Hansen, J. Daniels, Oliver Hemmers, P. Glans, S. B. Whitfield, H. Wang, Dennis W. Lindle
First Results From The High-Brightness X-Ray Spectroscopy Beamline 9.3.1 At Als, W. Ng, G. Jones, Rupert C. Perera, D. Hansen, J. Daniels, Oliver Hemmers, P. Glans, S. B. Whitfield, H. Wang, Dennis W. Lindle
Environmental Studies Faculty Publications
Beamline 9.3.1 at the Advanced Light Source (ALS) is a windowless beamline, covering the 1–6 keV photon energy range. This beamline is designed to achieve the goal of high brightness at the sample for use in the x‐ray atomic and molecular spectroscopy (XAMS) science, surface and interface science, biology and x‐ray optical development programs at ALS. X‐ray absorption and time‐of‐flight photoemission measurements in 2–5 keV photon energy range along with the flux, resolution, spot size and stability of the beamline will be discussed. Prospects for future XAMS measurements will also be presented.
Kinetic-Energy- And Angular-Resolved Fragmentation Of Co In Vibrational-Resolved C 1s Excitation, N. Saito, Franz Heiser, Oliver Hemmers, K. Wieliczek, J. Viefhaus, U. Becker
Kinetic-Energy- And Angular-Resolved Fragmentation Of Co In Vibrational-Resolved C 1s Excitation, N. Saito, Franz Heiser, Oliver Hemmers, K. Wieliczek, J. Viefhaus, U. Becker
Environmental Studies Faculty Publications
Angular distributions of C++O+ from CO were measured, following vibrationally resolved C 1s excitations into the 2pπ, 3sσ, and 3pπ orbitals as well as into higher unresolved orbitals. A time-of-flight mass spectrometer, with a multihit-type position-sensitive anode, was used for the measurements. The anisotropy parameters (β) of C++O+ approach their theoretically expected values as the released kinetic energy in the fragmentation increases. The value of the β parameters remains constant for all vibrational states within each orbital.
Auger Resonant Raman Spectroscopy Used To Study The Angular Distributions Of The Xe 4d5/2 → 6p Decay Spectrum, B. Langer, N. Berrah, A. Farhat, Oliver Hemmers, J. Bozek
Auger Resonant Raman Spectroscopy Used To Study The Angular Distributions Of The Xe 4d5/2 → 6p Decay Spectrum, B. Langer, N. Berrah, A. Farhat, Oliver Hemmers, J. Bozek
Environmental Studies Faculty Publications
The Auger resonant Raman effect can be used as a method to eliminate natural lifetime broadening in resonant Auger spectra. We have coupled this method with high-resolution photons from the Advanced Light Source to study angular distributions and decay rates of the Xe4d5/2→6p resonant Auger lines. The angular distribution parameters β of almost all possible final ionic 5p4(3P, 1D, 1S)6p states have been determined. Our data, which remove the discrepancy between previous lower-resolution experimental results, are compared to different theoretical results.