Physical Sciences and Mathematics Commons^™

Cloud Microphysical Response To Entrainment And Mixing Is Locally Inhomogeneous And Globally Homogeneous: Evidence From The Lab, Jaemin Yeom, Ian Helman, Prasanth Prabhakaran, Jesse Anderson, Fan Yang, Raymond Shaw, Will Cantrell

Michigan Tech Research Data

The effects of entrainment-mixing on the cloud droplet size distribution are examined in the Pi cloud chamber that creates a turbulent supersaturated environment for cloud formation. The experiments are conducted with a temperature-controlled flange to mimic the entrainment-mixing process. The entrainment zone is created at the center of the top surface of the chamber, allowing dry air of controlled temperature (T_e) and flow rate (Q_e) to flow into the mixing cloud region. Due to the large-scale circulation, the downwind region is directly affected by entrained dry air from the flange, whereas the upwind region is representative …

Molecular Dynamics Simulation Data: Mw And Mlmw Water Model Ice Nucleation On A Hydrophilic Substrate With Negative Pressure, Will Cantrell, Tianshu Li, Issei Nakamura, Elise Rosky, Raymond Shaw

Michigan Tech Research Data

This dataset contains the data supporting Figures in the study by Rosky et al., "Molecular simulations reveal that heterogeneous ice nucleation occurs at higher temperatures in water under capillary tension", submitted for publication in Atmospheric Chemistry and Physics in February 2023. Input files for reproducing the molecular dynamics simulations are included.

The abstract from the paper reads: Using a molecular model of water freezing on a hydrophilic substrate, it is found that heterogeneous ice nucleation rates occur at higher temperatures in water that is under tension, in other words under negative pressure. For pressures ranging from from 1 atm to …

Physical, Optical, And Chemical Properties Of Light Absorbing Aerosols And Their Climatic Impacts, Susan Mathai

Dissertations, Master's Theses and Master's Reports

Aerosols are particles suspended in the atmosphere; they are emitted during natural phenomena such as dust storms, wildfires, and volcanic eruptions, and during anthropogenic activities like household wood burning, vehicles operations, and industrial productions, or they can form in the atmosphere from gas to particle partition. Aerosols impact earth’s weather and climate by absorbing and scattering the incoming solar and the outgoing earth thermal radiation and interacting with clouds. The optical properties of aerosols evolve as the chemical and physical properties vary during their residence in the atmosphere. In addition, the aerosols’ properties strongly depend on the vertical distribution in …

An Intercomparison Of Large-Eddy Simulations Of A Convection Cloud Chamber Using Haze-Capable Bin And Lagrangian Cloud Microphysics Schemes, Fan Yang, Fabian Hoffmann, Raymond Shaw, Mikhail Ovchinnikov, Andrew Vogelmann

Michigan Tech Research Data

Recent in-situ observations show that haze particles exist in a convection cloud chamber. The microphysics schemes previously used for large-eddy simulations of the cloud chamber could not fully resolve haze particles and the associated processes, including their activation and deactivation. Specifically, cloud droplet activation is modeled based on Twomey-type parameterizations, wherein cloud droplets are formed when a critical supersaturation for the available cloud condensation nuclei (CCN) is exceeded and haze particles are not explicitly resolved. Here, we develop and adapt haze-capable bin and Lagrangian microphysics schemes to properly resolve the activation and deactivation processes. Results are compared with the Twomey-type …

Data Supporting The Paper "Is The Water Vapor Supersaturation Distribution Gaussian?", Subin Thomas, Prasanth Prabhakaran, W. Cantrell, Raymond Shaw

Michigan Tech Research Data

The data in this file are from the MTU Pi Cloud Chamber and large eddy simulations. This work was supported by NSF grant AGS-1754244. Data are made available in support of the above publication by Thomas et al.. For any further use, e.g., for publication elsewhere, the authors should be contacted to ensure the appropriate use of the data and proper acknowledgment.

Understanding The Effects Of Water Vapor And Temperature On Aerosol Using Novel Measurement Methods, Tyler Jacob Capek

Dissertations, Master's Theses and Master's Reports

Aerosol and water are inexorably linked, and both are ubiquitous within our atmosphere and required components for cloud formation. Relative humidity (RH), a temperature dependent quantity, can have a significant influence on the size, shape, and ultimately, the optical properties of the aerosol. RH can vary substantially on small spatial and short temporal scales in turbulent conditions due to rapid fluctuations in temperature and water vapor mixing ratio. Accurate assessment of optical enhancements due to an increase in RH is key for determining the particles’ impact on the climate and visibility.

A humidity-controlled cavity attenuated phase-shift albedometer (H-CAPS-PM_SSA) …

Investigating Ice Nucleation At Negative Pressures Using Molecular Dynamics: A First Order Approximation Of The Dependence Of Ice Nucleation Rate On Pressure, Elise Rosky

Dissertations, Master's Theses and Master's Reports

Atmospheric scientists and climate modelers are faced with uncertainty around the process of ice production in clouds. While significant progress has been made in predicting homogeneous and heterogeneous ice nucleation rates as a function of temperature, recent experiments have shown that ice nucleation rates can be enhanced without decreasing temperature, through various mechanical agitations. One hypothesis for these findings is that mechanisms of stretching water and thereby inducing negative pressure in the liquid could lead to an increase in freezing rate. To better understand the viability of this concept, the effect of negative pressure on ice nucleation rates needs to …

Modeling And Numerical Simulations Of The Michigan Tech Convection Cloud Chamber, Subin Thomas

Dissertations, Master's Theses and Master's Reports

Understanding atmospheric clouds is essential for human progress, ranging from short-term effects such as when and how much it rains to long-term effects such as how much temperatures would rise due to global climate change. Clouds vary globally and seasonally; also they have length scales ranging from a few nanometers to a few kilometers and timescales from a few nanoseconds to a few weeks. Knowledge gaps in aerosol-cloud-turbulence interactions and a lack of sufficient resolution in observations pose a challenge in understanding cloud systems.

Experimental facilities like the Michigan Tech Cloud Chamber can provide a suitable platform for studying aerosol-cloud …

Activation Scavenging Of Aerosol : Effect Of Turbulence And Aerosol-Composition, Abu Sayeed Md Shawon

Dissertations, Master's Theses and Master's Reports

The interaction of aerosol particles with solar radiation significantly contributes to the global radiation balance. The magnitude of this aerosol-radiation interaction, among other parameters, depends on different aerosol properties, including how readily these particles would act as cloud condensation nuclei (CCN). These properties are governed by the formation and scavenging processes of aerosol. This dissertation explores some of these scavenging processes.

Favorable humidity and preexisting aerosol particles acting as CCN are the sine qua non conditions to form cloud droplets in Earth’s atmosphere. Forming cloud droplets (known as activation), meanwhile, acts as a wet scavenging mechanism for those CCN. Given …

Data In Support Of The Paper "Dependence Of Aerosol-Droplet Partitioning On Turbulence In A Laboratory Cloud", Abu Sayeed Md Shawon, Prasanth Prabhakaran, Gregory Kinney, Raymond Shaw, Will Cantrell

Michigan Tech Research Data

No abstract provided.

Extensive Soot Compaction By Cloud Processing From Laboratory And Field Observations, Janarjan Bhandari, Swarup China, Kamal Kant Chandrakar, Greg Kinney, Will Cantrell, Raymond Shaw, Lynn Mazzoleni, Giulia Girotto, Noopur Sharma, Kyle Gorkowski, Stefania Gilardoni, Stefano Decesari, Maria Cristina Facchini, Nicola Zanca, Giulia Pavese, Francesco Esposito, Manvendra K Dubey, Allison C Aiken, Rajan K Chakrabarty, Hans Moosmüller, Timothy B Onasch, Rahul A Zaveri, Barbara V Scarnato, Paulo Fialho, Claudio Mazzoleni

Michigan Tech Publications

Soot particles form during combustion of carbonaceous materials and impact climate and air quality. When freshly emitted, they are typically fractal-like aggregates. After atmospheric aging, they can act as cloud condensation nuclei, and water condensation or evaporation restructure them to more compact aggregates, affecting their optical, aerodynamic, and surface properties. Here we survey the morphology of ambient soot particles from various locations and different environmental and aging conditions. We used electron microscopy and show extensive soot compaction after cloud processing. We further performed laboratory experiments to simulate atmospheric cloud processing under controlled conditions. We find that soot particles sampled after …

Data Supporting The Paper "Extensive Soot Compaction By Cloud Processing From Laboratory And Field Observations", Janarjan Bhandari, Swarup China, Kamal Kant Chandrakar, Greg Kinney, Will Cantrell, Raymond Shaw, Lynn R. Mazzoleni, Giulia Girotto, Noopur Sharma, Kyle Gorkowski, Stefania Gilardoni, Stefano Decesari, Maria Cristina Facchini, Nicola Zanca, Giulia Pavese, Francesco Esposito, Manvendra Dubey, Allison Aiken, Rajan K. Chakrabarty, Hans Moosmüller, Timothy B. Onasch, Rahul A. Zaveri, Barbara Scarnato, Paolo Fialho, Claudio Mazzoleni

Department of Physics Publications

No abstract provided.

Data Supporting The Paper "Scaling Of An Atmospheric Model To Simulate Turbulence And Cloud Microphysics In The Pi Chamber", Subin Thomas, Mikhail S. Ovchinnikov, Fan Yang, Dennis Van Der Voort, Will Cantrell, Steven K. Krueger, Raymond Shaw

Department of Physics Publications

No abstract provided.

Molecular Characterization Of Free Tropospheric Organic Aerosol And The Development Of Computational Tools For Molecular Formula Assignment, Simeon Schum

Dissertations, Master's Theses and Master's Reports

Organic aerosol affects human health and climate. These effects are largely determined by the composition of the organic aerosol, which is a complex mixture of species. Understanding the complexity of organic aerosol is critical to determining its effect on human health and climate. In this study, long range transported organic aerosol collected at the Pico Mountain Observatory was analyzed using ultrahigh resolution mass spectrometry. Organic aerosol transported in the free troposphere had an overall lower extent of oxidation than aerosol transported in the boundary layer. It was hypothesized that the lower oxidation was related to a more viscous phase state …

Aerosol-Cloud Interactions In Turbulent Clouds: A Combined Cloud Chamber And Theoretical Study, Kamal Kant Chandrakar

Dissertations, Master's Theses and Master's Reports

The influence of aerosol concentration on the cloud droplet size distribution is investigated in a laboratory chamber that enables turbulent cloud formation through moist convection. In chapter 2, moist Rayleigh-Bénard convection with water saturated boundaries is explored using a one-dimensional-turbulence model. This study provides some background about supersaturation statistics in moist convection. Chapters 3 - 7 discuss the experimental and theoretical investigation of aerosol-cloud interactions and cloud droplet size-distributions in turbulent conditions. The experiments are performed in a way so that steady-state microphysics are achieved, with aerosol input balanced by cloud droplet growth and fallout. As aerosol concentration is increased …

Light Propagation Through A Turbulent Cloud: Comparison Of Measured And Computed Extinction, Eduardo Rodriguez-Feo Bermudez

Dissertations, Master's Theses and Master's Reports

Remote sensing techniques used for measurement of atmospheric cloud properties operate under the notion that light extinction caused by scattering and absorption is exponential due to Beer-Lambert law. This is expected to be valid for a uni-form medium with no spatial correlations between particle position. The aim of this research was to show that under turbulent conditions, cloud droplets cannot be interpreted as non-correlated, and in turn will exhibit a lower than exponential light decay from scattering. The research took place at the MTU π-Chamber laboratory. A temperature difference between the floor and ceiling of the chamber was applied to …

Extreme Molecular Diversity In Biomass Burning Atmospheric Organic Aerosol Observed Through Ultrahigh Resolution Mass Spectrometry, Matthew Brege

Dissertations, Master's Theses and Master's Reports

Ambient atmospheric aerosol is ubiquitous in the atmosphere, originating from a variety of natural and man-made sources. These microscopic particles have profound impacts on the global climate system as well as human health. The organic fraction of atmospheric aerosol is an extremely complex mixture which is not yet fully characterized. These unknown organic aerosol species contribute to the uncertainty in the effect of aerosol on climate and uncertainty in overall ambient aerosol toxicity. Light absorbing organic aerosol can interact with incoming solar radiation and contribute to atmospheric heating; however, the source apportionment and overall fate of these absorbing organic aerosol …

Investigation Of Light Transport And Scattering In Turbulent Clouds: Simulations And Laboratory Measurements, Corey D. Packard

Dissertations, Master's Theses and Master's Reports

A better understanding of light transport and scattering in turbulent clouds is needed for more accurate remote sensing, improved imaging and signal transmission through atmospheric aerosol and fog, and deeper understanding of cloud optical properties relevant to weather and climate. In this study, we investigate the impact of light scattering in clouds on two problems of atmospheric relevance.

In the first part, we examine deleterious effects of the atmosphere on remotely acquired images including signal attenuation and potential blurring due to forward-scattered light accepted by the imaging system. A prior proposed aerosol scattering model provides a method for calculating the …

Fine-Scale Droplet Clustering In Atmospheric Clouds: 3d Radial Distribution Function From Airborne Digital Holography, Michael L. Larsen, Raymond Shaw, Alexander Kostinski, Susanne Glienke

Department of Physics Publications

The extent of droplet clustering in turbulent clouds has remained largely unquantified, and yet is of possible relevance to precipitation formation and radiative transfer. To that end, data gathered by an airborne holographic instrument are used to explore the three-dimensional spatial statistics of cloud droplet positions in homogeneous stratiform boundary-layer clouds. The three-dimensional radial distribution functions g(r) reveal unambiguous evidence of droplet clustering. Three key theoretical predictions are observed: the existence of positive correlations, onset of correlation in the turbulence dissipation range, and monotonic increase of g(r) with decreasing r. This implies that current theory captures the essential processes contributing …

Turbulence Induced Cloud Voids: Observation And Interpretation, Katarzyna Karpinska, Jonathan F. E. Bodenschatz, Szymon P. Malinowski, Jakub L. Nowak, Steffen Risius, Tina Schmeissner, Raymond Shaw, Holger Siebert, Hengdong Xi, Haitao Xu, Eberhard Bodenschatz

Department of Physics Publications

The phenomenon of cloud voids, i.e., elongated volumes inside a cloud that are devoid of droplets, was observed with laser sheet photography in clouds at a mountain-top station. Two experimental cases, similar in turbulence conditions yet with diverse droplet size distributions and cloud void prevalence, are reported. A theoretical explanation is proposed based on the study of heavy inertial sedimenting particles inside a Burgers vortex. A general conclusion regarding void appearance is drawn from theoretical analysis. Numerical simulations of polydisperse droplet motion with realistic vortex parameters and Mie scattering visual effects accounted for can explain the presence of voids with …

Molecular And Physical Characteristics Of Aerosol At A Remote Free Troposphere Site: Implications For Atmospheric Aging, Simeon Schum, Bo Zhang, Katja Džepina, Paolo Fialho, Claudio Mazzoleni, Lynn Mazzoleni

Department of Chemistry Publications

Aerosol properties are transformed by atmospheric processes during long-range transport and play a key role in the Earth's radiative balance. To understand the molecular and physical characteristics of free tropospheric aerosol, we studied samples collected at the Pico Mountain Observatory in the North Atlantic. The observatory is located in the marine free troposphere at 2225m above sea level, on Pico Island in the Azores archipelago. The site is ideal for the study of long-range-transported free tropospheric aerosol with minimal local influence. Three aerosol samples with elevated organic carbon concentrations were selected for detailed analysis. FLEXPART retroplumes indicated that two of …

Data Supporting The Paper "Turbulence Induced Cloud Voids: Observation And Interpretation", Katarzyna Karpinska, Jonathan F. E. Bodenschatz, Szymon P. Malinowski, Jakub L. Nowak, Steffen Risius, Tina Schmeissner, Raymond Shaw, Holger Siebert, Hengdong Xi, Haitao Xu, Eberhard Bodenschatz

Department of Physics Publications

No abstract provided.

Dispersion Aerosol Indirect Effect In Turbulent Clouds: Laboratory Measurements Of Effective Radius, K. K. Chandrakar, Will Cantrell, A. Kostinski, Raymond Shaw

Department of Physics Publications

Cloud optical properties are determined not only by the number density n_d and mean radius ṝ of cloud droplets but also by the shape of the droplet size distribution. The change in cloud optical depth with changing n_d, due to the change in distribution shape, is known as the dispersion effect. Droplet relative dispersion is defined as d=σ_r / ṝ . For the first time, a commonly used effective radius parameterization is tested in a controlled laboratory environment by creating a turbulent cloud. Stochastic condensation growth suggests d independent of n_d for a nonprecipitating cloud, …

Data Supporting The Paper "Dispersion Aerosol Indirect Effect In Turbulent Clouds: Laboratory Measurements Of Effective Radius", K. K. Chandrakar, Will Cantrell, A. Kostinski, R. A. Shaw

Department of Physics Publications

No abstract provided.

Simulation Data Supporting The Paper "Optical Properties And Radiative Forcing Of Fractal-Like Tar Ball Aggregates From Biomass Burning", Janarjan Bhandari, Swarup China, Giulia Girotto, Barbara Scarnato, Kyle Gorkowski, Allison Aiken, Manvendra Dubey, C. Mazzoleni

Department of Physics Publications

Simulations data supporting the paper "Optical properties and radiative forcing of fractal-like tar ball aggregates from biomass burning," to be submitted to the Journal of Quantitative Spectroscopy and Radiative Transfer.

Measurement And Modeling Of The Multiwavelength Optical Properties Of Uncoated Flame-Generated Soot, Sara D. Forestieri, Taylor M. Helgestad, Andrew T. Lambe, Lindsay Renbaum-Wolff, Paulo Massoli, Eben S. Cross, Claudio Mazzoleni, Et. Al.

Michigan Tech Publications

Optical properties of flame-generated black carbon (BC) containing soot particles were quantified at multiple wavelengths for particles produced using two different flames: a methane diffusion flame and an ethylene premixed flame. Measurements were made for (i) nascent soot particles, (ii) thermally denuded nascent particles, and (iii) particles that were coated and then thermally denuded, leading to the collapse of the initially lacy, fractal-like morphology. The measured mass absorption coefficients (MACs) depended on soot maturity and generation but were similar between flames for similar conditions. For mature soot, here corresponding to particles with volume-equivalent diameters >∼160 nm, the MAC and absorption …

Observation Of A Link Between Energy Dissipation Rate And Oscillation Frequency Of The Large-Scale Circulation In Dry And Moist Rayleigh-Bénard Turbulence, Dennis Niedermeier, Kelken Chang, Will Cantrell, Kamal Kant Chandrakar, David Ciochetto, Raymond Shaw

Department of Physics Publications

In this study both the small- and large-scale flow properties of turbulent Rayleigh-Bénard convection are investigated. Experiments are carried out using the Π chamber (aspect ratio Γ=2) for Rayleigh number range Ra∼10⁸–10⁹ and Prandtl number Pr≈0.7. Furthermore, experiments are run for dry and wet conditions, i.e., top and bottom surfaces of the chamber are dry and wet, respectively. For wet conditions we further distinguish between conditions with and without the presence of sodium chloride aerosol particles which, if supersaturated conditions are achieved, lead to cloud droplet formation. We therefore refer to these conditions as moist and cloudy, …

Identification And Characterization Of An Anomaly In Two-Dimensional Video Disdrometer Data, Michael L. Larsen, Michael Schönhuber

Michigan Tech Publications

The two-dimensional video distrometer (2DVD) is a well known ground based point-monitoring precipitation gauge, often used as a ground truth instrument to validate radar or satellite rainfall retrieval algorithms. This instrument records a number of variables for each detected hydrometeor, including the detected position within the sample area of the instrument. Careful analyses of real 2DVD data reveal an artifact—there are time periods where hydrometeor detections within parts of the sample area are artificially enhanced or diminished. Here, we (i) illustrate this anomaly with an exemplary 2DVD data set, (ii) describe the origin of this anomaly, (iii) develop and present …

The Interactive Stratospheric Aerosol Model Intercomparison Project (Isa-Mip): Motivation And Experimental Design, Claudio Timmreck, Graham W. Mann, Valentina Aquila, Rene Hommel, Lindsay A. Lee, Simon Carn, Et. Al.

Michigan Tech Publications

The Stratospheric Sulfur and its Role in Climate (SSiRC) Interactive Stratospheric Aerosol Model Intercomparison Project (ISA-MIP) explores uncertainties in the processes that connect volcanic emission of sulfur gas species and the radiative forcing associated with the resulting enhancement of the stratospheric aerosol layer. The central aim of ISA-MIP is to constrain and improve interactive stratospheric aerosol models and reduce uncertainties in the stratospheric aerosol forcing by comparing results of standardized model experiments with a range of observations. In this paper we present four co-ordinated inter-model experiments designed to investigate key processes which influence the formation and temporal development of stratospheric …

Development Of The Wrf-Co2 4d-Var Assimilation System V1.0, Tao Zheng, Nancy H. F. French, Martin Baxter

Michigan Tech Publications

Regional atmospheric CO2 inversions commonly use Lagrangian particle trajectory model simulations to calculate the required influence function, which quantifies the sensitivity of a receptor to flux sources. In this paper, an adjoint-based four-dimensional variational (4D-Var) assimilation system, WRF-CO2 4D-Var, is developed to provide an alternative approach. This system is developed based on the Weather Research and Forecasting (WRF) modeling system, including the system coupled to chemistry (WRF-Chem), with tangent linear and adjoint codes (WRFPLUS), and with data assimilation (WRFDA), all in version 3.6. In WRF-CO2 4D-Var, CO2 is modeled as a tracer and its feedback to meteorology is ignored. This …