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Theses/Dissertations

William & Mary

Optics

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Full-Text Articles in Engineering

Nonlinear Optical Studies Of Photoelastic Effect And Magneto-Plasmonics, Wei Zheng Jan 2014

Nonlinear Optical Studies Of Photoelastic Effect And Magneto-Plasmonics, Wei Zheng

Dissertations, Theses, and Masters Projects

Nonlinear optical (NLO) processes are optical phenomena involving a nonlinear response to an applied light field. Two kinds of nonlinearities are studied in this dissertation: magnetic-induced second-harmonic generation (MSHG) interacting with surface plasmon, called "nonlinear magnetoplasmonics" (NMP), and the nonlinear index induced by a strong pump beam in Titanium doped sapphire crystal, referred to as population-induced nonlinear index effect.;The fundamentals of the major effects involved are discussed, which include: surface plasmon and its field enhancement effect, MSHG technique and phenomenological calculations, the contrast ratio of magnetic switching, the calculation of lensing effects, population induced strain, and photoelastic effect. Furthermore, the …


Optical Characterization Of Magnetism In Magnetic/Nonmagnetic Heterostructures, Yichun Fan Jan 2013

Optical Characterization Of Magnetism In Magnetic/Nonmagnetic Heterostructures, Yichun Fan

Dissertations, Theses, and Masters Projects

This thesis focuses on the study of the static and dynamic magnetic interactions in ferromagnetic/nonmagnetic heterostructures using interface-specific and time-resolved optical techniques. The goal of this thesis is to elucidate the interface exchange coupling, magnetic anisotropy, and coherent spin dynamics in these advanced material systems, crucial to the realization of high performance spintronic devices.;First, a pronounced exchange bias (EB) phenomenon is observed in Fe/MgO (001) by magnetic second harmonic generation. The bulk magnetization does not, in marked contrast to typical systems where EB is manifested only in the net magnetization. The magnitude of the exchange bias varies with interface oxygen …


Microscopic Dynamics And Transport Of Hydrogen In Proton Conducting Oxides, Erik J. Spahr Jan 2011

Microscopic Dynamics And Transport Of Hydrogen In Proton Conducting Oxides, Erik J. Spahr

Dissertations, Theses, and Masters Projects

The microscopic motion of hydrogen in solid oxides plays an important role in defect migration and reaction processes. Understanding the vibrational dynamics associated with both hydrogen-oxygen (O-H) bonds and the surrounding ionic environment allows one to better characterize these fundamental interactions. This thesis presents a comprehensive investigation into the vibrational decay dynamics of O-H and O-D stretch modes in crystalline oxides using time-resolved infrared pump-probe spectroscopy.;Measurements of the vibrational lifetimes of hydrogen related local modes in potassium tantalate (KTaO3) and titanium dioxide (TiO2 ) show that the localized O-H vibration is very closely tied to proton transport. In KTaO3 we …


Advancements In Dual-Pump Broadband Cars For Supersonic Combustion Measurements, Sarah Augusta. Tedder Jan 2010

Advancements In Dual-Pump Broadband Cars For Supersonic Combustion Measurements, Sarah Augusta. Tedder

Dissertations, Theses, and Masters Projects

Space- and time-resolved measurements of temperature and species mole fractions of nitrogen, oxygen, and hydrogen were obtained with a dual-pump coherent anti-Stokes Raman spectroscopy (CARS) system in hydrogen-fueled supersonic combustion free jet flows. These measurements were taken to provide time-resolved fluid properties of turbulent supersonic combustion for use in the creation and verification of computational fluid dynamic (CFD) models. CFD models of turbulent supersonic combustion flow currently facilitate the design of air- breathing supersonic combustion ramjet (scramjet) engines. Measurements were made in supersonic axi-symmetric free jets of two scales. First, the measurement system was tested in a laboratory environment using …


Time-Resolved Magnetic Flux And Ac-Current Distributions In Superconducting Yttrium Barium Copper Oxide Thin Films And Multifilaments, Ran Yang Jan 2008

Time-Resolved Magnetic Flux And Ac-Current Distributions In Superconducting Yttrium Barium Copper Oxide Thin Films And Multifilaments, Ran Yang

Dissertations, Theses, and Masters Projects

Time-resolved magneto-optical imaging (TRMOI) technique allows dynamic ac transport measurements on superconductors. The high time and spatial resolutions of the measurements also offer good quantitative data analysis of the MO images. YBa2Cu 3O7-delta (YBCO) was discovered as a high-temperature superconductor (HTSC) which has wide applications due to its high critical temperature of Tc = 91 K, and high critical current density Jc in the order of 106-7 Acm-2. Many of the applications require high ac current load and a high magnetic field. We study the interaction behavior of YBCO thin films in an ac transport current and a dc magnetic …


Fluorescence Imaging Study Of Free And Impinging Supersonic Jets: Jet Structure And Turbulent Transition, Jennifer Ann Inman Jan 2007

Fluorescence Imaging Study Of Free And Impinging Supersonic Jets: Jet Structure And Turbulent Transition, Jennifer Ann Inman

Dissertations, Theses, and Masters Projects

A series of experiments into the behavior of underexpanded jet flows has been conducted at NASA Langley Research Center. This work was conducted in support of the Return to Flight effort following the loss of the Columbia. The tests involved simulating flow through a hypothetical breach in the leading edge of the Space Shuttle Orbiter along its reentry trajectory, with the goal of generating a data set with which other researchers can test and validate computational modeling tools. Two nozzles supplied with high-pressure gas were used to generate axisymmetric underexpanded jets exhausting into a low-pressure chamber. These nozzles had exit …


Optical Characterization Of Ferromagnetic Heterostructure *Interfaces And Thin Films, Haibin Zhao Jan 2006

Optical Characterization Of Ferromagnetic Heterostructure *Interfaces And Thin Films, Haibin Zhao

Dissertations, Theses, and Masters Projects

This thesis presents optical characterizations of interfaces in ferromagnetic heterostructures and thin films used for spin polarized electronic devices. In these experiments, femtosecond laser spectroscopies are exploited to investigate the interface magnetization reversal, spin precession, and band offset, which are crucial in determining the performances of spintronic devices.;First, magnetization-induced second-harmonic-generation (MSHG) is applied to study interface magnetism in a hybrid structure containing a noncentrosymmetric semiconductor---Fe/AlGaAs. The reversal process of Fe interface layer magnetization is compared with the bulk magnetization reversal. In Fe/AlGaAs (001), the interface magnetization is found to be decoupled from the bulk magnetization based on the different switching …


Ultrafast Laser Spectroscopy Of Half -Metallic Chromium Dioxide, Hailong Huang Jan 2006

Ultrafast Laser Spectroscopy Of Half -Metallic Chromium Dioxide, Hailong Huang

Dissertations, Theses, and Masters Projects

This thesis presents ultrafast laser pump-probe differential transmission experiments on epitaxial CrO2 (110). The experiments were conducted at the wavelengths of 600 nm, 800 nm and 1200 nm, corresponding to the transition energies of 2 eV, 1.5 eV and 1 eV respectively. The wavelength dependent results, comparing with linear optical absorption, revealed the electronic structure of the material. The experimental results also showed polarization dependence of the probe beams. This is attributed to the electronic orbital anisotropy.;Temperature dependence was observed in the pump-probe experiments. The ultrafast transmission data show similar temperature dependence as ultrafast MOKE (Magneto-Optical Kerr Effect) data. A …


Vibrational Lifetimes Of Hydrogen And Oxygen Defects In Semiconductors, Baozhou Sun Jan 2005

Vibrational Lifetimes Of Hydrogen And Oxygen Defects In Semiconductors, Baozhou Sun

Dissertations, Theses, and Masters Projects

Characterization of defect and impurity reactions, dissociation, and migration in semiconductors requires a detailed understanding of the rates and pathways of vibrational energy flow and of the coupling mechanisms between local modes and the phonon bath of the host material. Information on the inelastic microscopic interaction can be obtained by measuring the lifetime of local vibrational modes. This dissertation presents lifetime measurements of hydrogen and oxygen defects in semiconductors by means of time-resolved infrared pump-probe spectroscopy.;First, we measured the vibrational lifetime of H- and D-related bending modes in Si and other semiconductors. Time-resolved pump-probe and linewidth measurements reveal that the …


Theoretical And Experimental Study Of Generation Mechanisms For Laser Ultrasound In Woven Graphite /Epoxy Composites With Translaminar Stitching, Adam D. Friedman Jan 2000

Theoretical And Experimental Study Of Generation Mechanisms For Laser Ultrasound In Woven Graphite /Epoxy Composites With Translaminar Stitching, Adam D. Friedman

Dissertations, Theses, and Masters Projects

The aerospace industry is beginning to use advanced composite materials for primary load bearing structures and their failure mechanisms must be better understood to predict their behavior in service. The Combined Loads Tests (COLTS) facility is being constructed at the NASA Langley Research Center to characterize these failure mechanisms. Laser based ultrasonic NDE can monitor the samples during dynamic loading without interfering with the structural tests. However, the constraints of implementing laser ultrasound in a structures laboratory reduces the efficiency of the technique. The system has to be "eye-safe" because many people will be present during the structural tests. Consequently, …