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Afci Quarterly Input – Unlv October Through December, 2003, Harry Reid Center For Environmental Studies. Nuclear Science And Technology Division

Transmutation Research Program Reports (TRP)

Quarterly report highlighting research projects and objectives of the Transmutation Research Program at the Nuclear Science & Technology Division, Harry Reid Research Center.

The University of Nevada, Las Vegas supports the AFCI through research and development of technologies for economic and environmentally sound refinement of spent nuclear fuel. The UNLV program has four components: infrastructure, international collaboration, student-based research, and management and program support.

Inside Unlv, Gian Galassi, Katrina Hudak, Carol C. Harter, Eric Sandgren, Tom Hagge

Inside UNLV

No abstract provided.

Modeling Corrosion In Oxygen Controlled Lbe Systems With Coupling Of Chemical Kinetics And Hydrodynamics-Task V: Fourth Quarterly Report 09/01/2003-11/30/2003, Samir Moujaes, Yitung Chen

Transmutation Sciences Materials (TRP)

The Lead-Bismuth eutectic (LBE) has been determined from previous experimental studies by the Russians and the European scientific community to be a potential material that can be used as a spallation target and coolant for the TRP proposed application. Properly controlling the oxygen content in LBE can drastically reduce the LBE corrosion to structural steels. However, existing knowledge of material corrosion performance was obtained from point-wise testing with only very sparse experimental data. Scientists have noticed that the concentration of oxygen dissolved in the liquid alloy could control the corrosion rate of steels exposed to Pb or Pb-Bi. At high …

Design And Evaluation Of Processes For Fuel Fabrication: Quarterly Progress Report #9, Georg F. Mauer

Fuels Campaign (TRP)

The ninth quarter of the project covered the following:

• Mr. Richard Silva continued the development of a simulation model with a Waelischmiller hot cell robot. Rich will continue to develop detailed 3-D process simulation models as his M.Sc. thesis project.

• A paper on hot cell robotics was presented at the ANS Winter Annual Meeting and published in the ANS 2003 conference proceedings.

• Further advances on Concepts and Methods for Vision-Based Hot Cell Supervision and control, focusing on rule-based object recognition (Ph.D. Student Jae-Kyu Lee)

• Graduate student Jamil Renno created simulations of more complex fuel manufacturing and …

Bomb-Pulse Chlorine-36 At The Proposed Yucca Mountain Repository Horizon: An Investigation Of Previous Conflicting Results And Collection Of New Data, Klaus J. Stetzenbach, Fred Phillips, Drew Coleman, Don Baepler, Amy J. Smiecinski

Publications (YM)

Previous studies by scientists at Los Alamos National Laboratory (LANL) and the United States Geological Survey (USGS) quantified ³⁶Cl/Cl to test for the presence of fast pathways at the proposed Yucca Mountain high-level nuclear waste repository. The goal of these studies was to determine whether or not fluids containing bomb-pulse ³⁶Cl/Cl traveled along fast travel pathways and reached the repository horizon, however, the two groups followed somewhat different procedures and produced conflicting results. The objective of this study is to attempt to determine the cause of the conflicting results and to obtain additional data to determine whether or …

Inside Unlv, Gian Galassi, Cayrn Key, Carol C. Harter, Patrick Ferrillo

Inside UNLV

No abstract provided.

Developing A Sensing System For The Measurement Of Oxygen Concentration In Liquid Pb-Bi Eutectic: Quarterly Progress Report (Aug. 01 – Oct. 31, 2003), Yingtao Jiang, Bingmei Fu

Transmutation Sciences Materials (TRP)

The experimental setup designed and manufactured in UNLV was shipped to LANL in early Aug. One student has been working in LANL to conduct the experiment since then. In the meantime, one new Ph. D. student has started to run the simulation for transport in oxygen mixing. In Oct., a professional has been hired to work in both experimental and the theoretical studies pertaining to the proposed work.

Environment-Induced Degradation And Crack-Growth Studies Of Candidate Target Materials: Quarterly Progress Report (June 1 – August 31, 2003), Ajit K. Roy, Brendan O'Toole

Transmutation Sciences Materials (TRP)

As indicated in the original proposal, the primary objective of this task is to evaluate the effect of hydrogen on environment-assisted cracking of candidate target materials for applications in spallationneutron- target (SNT) systems such as accelerator production of tritium (APT) and accelerator transmutation of waste (ATW). The materials selected for evaluation and characterization are martensitic stainless steels including Alloy HT-9, Alloy EP 823 and Type 422 stainless steel. The susceptibility to stress corrosion cracking (SCC) and hydrogen embrittlement (HE) of these materials are being evaluated in aqueous environments of interest using tensile specimens under constant load and slow-strain-rate (SSR) conditions. …

Development Of A Mechanistic Understanding Of High-Temperature Deformation Of Alloy Ep-823 For Transmutation Applications: Quarterly Progress Report (June 01 – Aug 31, 2003), Ajit K. Roy, Brendan O'Toole

Transmutation Sciences Materials (TRP)

The purpose of this project is to evaluate the elevated temperature tensile properties of Alloy EP-823, a leading target material for accelerator-driven waste transmutation applications. This Alloy has been proven to be an excellent structural material to contain the lead-bismuth-eutectic (LBE) nuclear coolant needed for fast spectrum operations. Very little data exist in the open literature on the tensile properties of this Alloy. The test material will be thermally treated prior to the evaluation of its tensile properties at temperatures relevant to the transmutation applications. The deformation characteristics of tensile specimens, upon completion of testing, will be evaluated by surface …

Use Of Positron Annihilation Spectroscopy For Stress-Strain Measurements: Quarterly Progress Report (June 01 – August 31, 2003), Ajit K. Roy

Transmutation Sciences Materials (TRP)

The purpose of this collaborative research project involving the University of Nevada Las Vegas (UNLV), the Idaho State University (ISU), and the Los Alamos National Laboratory (LANL) is to evaluate the feasibility of determining residual stresses in cold-worked, plastically-deformed (bent), and welded materials using a nondestructive method based on positron annihilation spectroscopy (PAS). This technique uses γ-rays from a small MeV electron Linac to generate positrons inside the sample via pair production. This method is known to have capabilities of characterizing defects in thick specimens that could not be accomplished by conventional positron technique or other nondestructive methods. The generated …

Development Of A Mechanistic Understanding Of High-Temperature Deformation Of Alloy Ep-823 For Transmutation Applications: Annual Progress Report (September 2002 – August 2003), Ajit K. Roy, Brendan O'Toole

Transmutation Sciences Materials (TRP)

The purpose of this project is to evaluate the elevated temperature tensile properties of Alloy EP-823, a leading structural target material for accelerator-driven waste transmutation applications. This alloy has been proven to be an excellent structural material to contain the molten lead-bismuth-eutectic (LBE) nuclear coolant needed for fast spectrum operations. Very little data exist in the open literature on the tensile properties of this martensitic alloy. Three different heats of this material, produced by vacuum induction melting, were thermally treated to produce fully-tempered martensitic microstructure without any retained austenite (Table I). Cylindrical specimens were fabricated from the heat-treated round bars …

Modeling, Fabrication, And Optimization Of Niobium Cavities: Phase Iii Quarterly Report, Robert A. Schill Jr., Mohamed Trabia

Transmutation Sciences Materials (TRP)

Niobium cavities are important parts of the integrated NC/SC high-power linacs. Over the years, researchers in several countries have tested various cavity shapes. They concluded that elliptically shaped cells are the most appropriate shape for superconducting cavities. The need for very clean surfaces lead to the use of a buffered chemical polishing produce for surface cleaning to get good performance of the cavities. The third phase concludes the experimental a fluid flow study and optimization study. The first quarter and second quarter of phase three also begins the experimental set-up of secondary emission studies from niobium in superconducting mode. This …

Inside Unlv, Cate Weeks, Diane Russell, Carol C. Harter, Martin Watson

Inside UNLV

No abstract provided.

Corrosion And Mass Transport Processes In Carbon Steel Miniature Waste Packages, James Cizdziel, Kaveh Zarrabi, Susan Lestrange, Amy J. Smiecinski

Publications (YM)

In this study, we have systematically investigated corrosion and mass transport processes in carbon steel miniature waste packages (MWP) in dynamic systems (water in, water out) under varying chemical conditions. The MWP were fabricated to have similar configuration to the DOE Spent Nuclear Fuel (SNF) waste package and that individual components to be in scale with each other compare to the SNF waste package. Two MWP configurations were studied: a "bathtub" model and a "flow-through" model. By slowly dripping 4 different solutions (groundwater obtained from well water J-13 located near Yucca Mountain, and J-13 water adjusted to low-pH, high-salinity, and …

Identification Of Dynamic Properties Of Materials For The Nuclear Waste Package, Brendan O'Toole, Mohamed Trabia, Amy J. Smiecinski

Publications (YM)

Stainless steel 316L, titanium alloy grade 7, and alloy C22 are currently under consideration as candidate materials for use in various components associated with the spent nuclear fuel package, which must be designed to withstand structural deformation caused by static, thermal, and handling loads. In addition, it has to maintain its integrity in case of accidents, where it may be subjected to high loads over a very short period of time. Mechanical characteristics of these three materials under dynamic loading are not well documented. This paper describes the procedures and results obtained from experiments performed over a range of slow …

Remote Monitoring Of Repository Integrity Using Passive Seismic Arrays, Barbara Luke, Evangelos Yfantis

Publications (YM)

Once radioactive waste is emplaced in the repository, the challenge of monitoring the continued integrity of the excavated openings (e.g., emplacement drifts) escalates tremendously. We envision a seismic monitoring array installed on the surface at Yucca Mountain, which operates automatically to monitor repository opening stability in the long term. The objective is to monitor and validate the structural integrity of the emplacement drifts through identifying and localizing rock falls that could compromise drift access, hinder waste retrievability, and potentially reduce the effective life of waste canisters. Collateral benefits of the system include the ability to address some outstanding uncertainties regarding …

Task 32 Delayed Hydride Cracking Of Spent Fuel Cladding Under Repository Conditions, Ajit K. Roy, Anthony Hechanova, Amy J. Smiecinski

Publications (YM)

The objective of this quality-affecting task is to evaluate the susceptibility of spent nuclear fuel cladding materials (zirconium alloys) to stress corrosion cracking (SCC), delayed hydride cracking (DHC) and localized corrosion (pitting/crevice) in simulated repository environments. During the first year of this project, major efforts were focused on developing the infrastructure for performing the desired testing involving two highly corrosion-resistant alloys namely, zircaloy-2 (Zr-2) and zircaloy-4 (Zr-4) in simulated concentrated acidic water (SAW) and modified SAW (SAWM). Modification of the SAW chemistry was done by adding hydrochloric acid (HC1) to achieve lower pH. The construction of the "Materials Performance Laboratory …

Thermal Transport Eveluations Related To Waste Package Design -- Model Evaluations -- Task 19, Roald Akberov

Publications (YM)

The purpose of the “Thermal Transport Evaluations Related to Waste Package Design” Task # 19 of Cooperative Agreement Number DE-FC28-98NV12081 was to develop a new CFDHT model for heat transfer and fluid flow in the potential rsepository at the Yucca Mountain, Nevada and to study the effects of forced convection during the pre-closure period and natural convection during the postclosure period. The analysis was performed for the drift dimensions shown in Figure 4-1 below. The intended use of the model is to estimate the velocity and temperature distribution as well as the highest temperature in the drift during the pre-closure …

Afci Quarterly Input – Unlv July Through September, 2003, Harry Reid Center For Environmental Studies. Nuclear Science And Technology Division

Transmutation Research Program Reports (TRP)

Quarterly report highlighting research projects and objectives of the Transmutation Research Program at the Nuclear Science & Technology Division, Harry Reid Research Center.

The University of Nevada, Las Vegas supports the AFCI through research and development of technologies for economic and environmentally sound refinement of spent nuclear fuel. The UNLV program has four components: infrastructure, international collaboration, student-based research, and management and program support.

Inside Unlv, Gian Galassi, Jennifer Vaughan, Carol C. Harter, Stephen Rosenbaum

Inside UNLV

No abstract provided.

Design And Evaluation Of Processes For Fuel Fabrication: Quarterly Progress Report #8, Georg F. Mauer

Fuels Campaign (TRP)

The eighth quarter of the project covered the following:

· Mr. Richard Silva continued the development of a simulation model with a Waelischmiller hot cell robot. Rich will continue to develop detailed 3-D process simulation models as his M.Sc. thesis project.

· A paper submitted for ANS for the Winter Annual Meeting on hot cell robotics was accepted for presentation and publication.

· Further advances on Concepts and Methods for Vision-Based Hot Cell Supervision and control, focusing on rule-based object recognition (Ph.D. Student Jae-Kyu Lee)

· Undergraduate student Jamil Renno created simulations of fuel pin assembly (robotic insertion of pellets …

Modeling Corrosion In Oxygen Controlled Lbe Systems With Coupling Of Chemical Kinetics And Hydrodynamics-Task V: Fourth Quarterly Report 06/01/2003-08/30/2003, Samir Moujaes, Yitung Chen

Transmutation Sciences Materials (TRP)

The Lead-Bismuth eutectic (LBE) has been determined from previous experimental studies by the Russians and the European scientific community to be a potential material that can be used as a spallation target and coolant for the TRP proposed application. Properly controlling the oxygen content in LBE can drastically reduce the LBE corrosion to structural steels. However, existing knowledge of material corrosion performance was obtained from point-wise testing with only very sparse experimental data. Scientists have noticed that the concentration of oxygen dissolved in the liquid alloy could control the corrosion rate of steels exposed to Pb or Pb-Bi. At high …

Modeling Corrosion In Oxygen Controlled Lbe Systems With Coupling Of Chemical Kinetics And Hydrodynamics-Task V: Annual Report -Phase Ii 09/01/2002-08/30/2003, Samir Moujaes, Yitung Chen

Transmutation Sciences Materials (TRP)

The Lead-Bismuth eutectic (LBE) has been determined from previous experimental studies by the Russians and the European scientific community to be a potential material that can be used as a spallation target and coolant for the TRP proposed application. Properly controlling the oxygen content in LBE can drastically reduce the LBE corrosion to structural steels. However, existing knowledge of material corrosion performance was obtained from point-wise testing with only very sparse experimental data. Scientists have noticed that the concentration of oxygen dissolved in the liquid alloy could control the corrosion rate of steels exposed to Pb or Pb-Bi. At high …

Development Of A Systems Engineering Model Of The Chemical Separations Process: Quarterly Progress Report 5/16/03- 8/15/03, Yitung Chen, Randy Clarksean, Darrell Pepper

Separations Campaign (TRP)

Two activities are proposed in this Phase I task: the development of a systems engineering model and the refinement of the Argonne code AMUSE (Argonne Model for Universal Solvent Extraction). The detailed systems engineering model is the start of an integrated approach to the analysis of the materials separations associated with the AAA Program. A second portion of the project is to streamline and improve an integral part of the overall systems model, which is the software package AMUSE. AMUSE analyzes the UREX process and other related solvent extraction processes and defines many of the process streams that are integral …

Development Of A Systems Engineering Model Of The Chemical Separations Process, Yitung Chen, Sean Hsieh, Randy Clarksean, Darrell Pepper

Separations Campaign (TRP)

The AFCI program is developing technology for the transmutation of nuclear waste to address many of the long-term disposal issues. An integral part of this program is the proposed chemical separations scheme.

Nearly all issues related to risks to future generations arising from long-term disposal of such spent nuclear fuel is attributable to about 2% of its content. Such 2% is made up primarily of plutonium, neptunium, americium, and curium (the transuranic elements) and long-lived isotopes of iodine and technetium created as products from the fission process in power reactors. When transuranics are removed from discharged fuel destined for disposal, …

Design And Analysis For Melt Casting Metallic Fuel Pins Incorporating Volatile Actinides: Quarterly Progress Report 5/16/03- 8/15/03, Yitung Chen, Randy Clarksean, Darrell Pepper

Fuels Campaign (TRP)

The analysis of mold filling and solidification continues with progress being made for the consideration of these two features within one model. Analysis of the induction heating process of an Induction Skull Melter (ISM) is under study. Efforts are underway to validate the modeling procedure and specific comparisons are being made to previously published work. Few detailed modeling results have been reported by other researchers, making the validations an important part of the overall modeling process. Skin heating depths, power deposition rates, and other process parameters are being evaluated for use in upcoming furnace design simulations. Efforts are beginning on …

Modeling Corrosion In Oxygen Controlled Lbe Systems With Coupling Of Chemical Kinetics And Hydrodynamics - Phase Three, Samir Moujaes, Yitung Chen

Transmutation Sciences Materials (TRP)

The proposed work will combine chemical kinetics and hydrodynamics in target and test-loop lead-bismuth eutectic (LBE) systems to model system corrosion effects. This approach will result in a predicative tool that can be validated with corrosion test data, used to systematically design tests and interpret the results, and provide guidance for optimization in LBE system designs. The task includes two subtasks. The first subtask is to try to develop the necessary predictive tools to be able to predict the levels of oxygen and corrosion products close to the boundary layer through the use of Computational Fluid Dynamics (CFD) modeling. The …

Developing A Sensing System For The Measurement Of Oxygen Concentration In Liquid Pb-Bi Eutectic: Quarterly Progress Report (May. 01 – July 31, 2003), Yingtao Jiang, Bingmei Fu, Woosoon Yim

Transmutation Sciences Materials (TRP)

The report for Y01 has been prepared and submitted. The final part of our apparatus, the N3Si4 stirrer, was received by the end of May. The assembly of the apparatus has almost been completed. The control plan for our apparatus has been revised. To run FLUENT, a high-end Unix-based Sun workstation has been acquired. Plan has been made to ship our apparatus to LANL.

Development Of Advanced High Temperature Heat Exchangers: Proposal, University Of Nevada, Las Vegas. Research Foundation

Publications (NSTD)

A research team led by the University of Nevada, Las Vegas (UNLV) Research Foundation proposes a project to develop advanced high temperature heat exchangers (HTHX) for hydrogen production and electrical energy conversion from advanced nuclear reactor concepts. This project will also support the development of Generation IV reactors. The research team includes researchers from UNLV, General Atomics (GA), Sandia National Laboratories (SNL), The University of California, Berkeley UCB) and Oak Ridge National Laboratory (ORNL).

The proposed project will be administered by the University of Nevada Las Vegas Research Foundation (UNLVRF). UNLVRF will provide the overall contract administration and is the …

Inside Unlv, Gian Galassi, Carol C. Harter, Gene Hall

Inside UNLV

No abstract provided.