Engineering Commons^™

Modeling Radionuclide Diffusion Using Moose A Multiscale, Multiphysics Platform, Jonathon Gardner

Theses and Dissertations

Very durable ceramic waste forms have been proposed which offer longterm stability by binding certain radionuclides in their specific crystalline network. Moreover, multiple such ceramic phases can be tailored to contain specific radionuclides generated in the fuel cycle. Many such candidate ceramic forms are in the early stages of development with limited data. Modeling and simulation including modeling of diffusion can inform and provide direction to ongoing fabrication and experimental efforts. Material properties important in modeling can be obtained through laboratory measurement where available and atomistic simulation. Since diffusion occurs over multiple scales and follows multiple pathways, multiscale modeling is …