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Single-Mode Tunable Laser Emission In The Single-Exciton Regime From Colloidal Nanocrystals, Christos Grivas, Chunyong Li, Peristera Andreakou, Pengfei Wang, Ming Ding, Gilberto Brambilla, Liberato Manna, Pavlos Lagoudakis
Single-Mode Tunable Laser Emission In The Single-Exciton Regime From Colloidal Nanocrystals, Christos Grivas, Chunyong Li, Peristera Andreakou, Pengfei Wang, Ming Ding, Gilberto Brambilla, Liberato Manna, Pavlos Lagoudakis
Articles
Whispering-gallery-mode resonators have been extensively used in conjunction with different materials for the development of a variety of photonic devices. Among the latter, hybrid structures, consisting of dielectric microspheres and colloidal core/shell semiconductor nanocrystals as gain media, have attracted interest for the development of microlasers and studies of cavity quantum electrodynamic effects. Here we demonstrate single-exciton, single-mode, spectrally tuned lasing from ensembles of optical antenna-designed, colloidal core/shell CdSe/CdS quantum rods deposited on silica microspheres. We obtain singleexciton emission by capitalizing on the band structure of the specific core/shell architecture that strongly localizes holes in the core, and the two-dimensional quantum …