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Overcoming Fundamental Barriers In Photovoltaic And Terahertz Generation, Chao Zhou

Open Access Theses

Several fundamental barriers limit the performance of opto-electronic conversion processes below 100%. Two specific examples of current technological interest include photovoltaic conversion of sunlight into electricity (i.e., solar cells), and terahertz generation from optical sources. In particular, solar cells are limited not only by the Carnot limit associated with the second law (approximately 86% at room temperature), but also by radiative recombination, non-reciprocity, carrier thermalization, and sub-bandgap losses. In the case of terahertz generation, the typical process of difference frequency generation relies on two input optical waves with only a small difference between them to generate the desired output; however, …