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Full-Text Articles in Engineering
Multiple New-Particle Growth Pathways Observed At The Us Doe Southern Great Plains Field Site, Anna L. Hodshire, Michael J. Lawler, Jun Zhao, John Ortega, Coty Jen, Taina Yli-Juuti, Jared F. Brewer, Jack K. Kodros, Kelley C. Barsanti, Dave R. Hanson, Peter H. Mcmurry, James N. Smith, Jeffery R. Pierce
Multiple New-Particle Growth Pathways Observed At The Us Doe Southern Great Plains Field Site, Anna L. Hodshire, Michael J. Lawler, Jun Zhao, John Ortega, Coty Jen, Taina Yli-Juuti, Jared F. Brewer, Jack K. Kodros, Kelley C. Barsanti, Dave R. Hanson, Peter H. Mcmurry, James N. Smith, Jeffery R. Pierce
Civil and Environmental Engineering Faculty Publications and Presentations
New-particle formation (NPF) is a significant source of aerosol particles into the atmosphere. However, these particles are initially too small to have climatic importance and must grow, primarily through net uptake of low volatility species, from diameters ∼ 1 to 30–100 nm in order to potentially impact climate. There are currently uncertainties in the physical and chemical processes associated with the growth of these freshly formed particles that lead to uncertainties in aerosol-climate modeling. Four main pathways for new-particle growth have been identified: condensation of sulfuric-acid vapor (and associated bases when available), condensation of organic vapors, uptake of organic acids …
Model For Acid-Base Chemistry In Nanoparticle Growth (Mabnag), Taina Yli-Juuti, Kelley Barsanti, L. Hildebrandt Ruiz, Antti-Jussi Kieloaho, U. Makkonen, Tuukka Petäjä, Taina Ruuskanen, Markku Kulmala, Ilona Riipinen
Model For Acid-Base Chemistry In Nanoparticle Growth (Mabnag), Taina Yli-Juuti, Kelley Barsanti, L. Hildebrandt Ruiz, Antti-Jussi Kieloaho, U. Makkonen, Tuukka Petäjä, Taina Ruuskanen, Markku Kulmala, Ilona Riipinen
Civil and Environmental Engineering Faculty Publications and Presentations
Climatic effects of newly-formed atmospheric secondary aerosol particles are to a large extent determined by their condensational growth rates. However, all the vapours condensing on atmospheric nanoparticles and growing them to climatically relevant sizes are not identified yet and the effects of particle phase processes on particle growth rates are poorly known. Besides sulfuric acid, organic compounds are known to contribute significantly to atmospheric nanoparticle growth. In this study a particle growth model MABNAG (Model for Acid-Base chemistry in NAnoparticle Growth) was developed to study the effect of salt formation on nanoparticle growth, which has been proposed as a potential …
Identification Of The Biogenic Compounds Responsible For Size-Dependent Nanoparticle Growth, Paul M. Winkler, John Ortega, Thomas Karl, Luca Cappellin, Hans R. Friedli, Kelley Barsanti, Peter H. Mcmurry, James N. Smith
Identification Of The Biogenic Compounds Responsible For Size-Dependent Nanoparticle Growth, Paul M. Winkler, John Ortega, Thomas Karl, Luca Cappellin, Hans R. Friedli, Kelley Barsanti, Peter H. Mcmurry, James N. Smith
Civil and Environmental Engineering Faculty Publications and Presentations
The probability that freshly nucleated nanoparticles can survive to become cloud condensation nuclei is highly sensitive to particle growth rates. Much of the growth of newly formed ambient nanoparticles can be attributed to oxidized organic vapors originating from biogenic precursor gases. In this study we investigated the chemical composition of size-selected biogenic nanoparticles in the size range from 10 to 40 nm. Particles were formed in a flow tube reactor by ozonolysis ofα-pinene and analyzed with a Thermal Desorption Chemical Ionization Mass Spectrometer. While we found similar composition in 10 and 20 nm particles, the relative amounts of …
Thirdhand Tobacco Smoke: Emerging Evidence And Arguments For A Multidisciplinary Research Agenda, Georg E. Matt, Penelope J. Quintana, Hugo Destaillats, Lara A. Gundel, Mohamad Sleiman, Brett C. Singer, Peyton Jacob, Jonathan P. Winickoff, Prue Talbot, Suzaynn Schick, Yinsheng Wang, Bo Hang, Manuela Martins-Green, James F. Pankow, Melbourne F. Hovell, Neal L. Benowitz, Virender K. Rehan, Jonathan M. Samet
Thirdhand Tobacco Smoke: Emerging Evidence And Arguments For A Multidisciplinary Research Agenda, Georg E. Matt, Penelope J. Quintana, Hugo Destaillats, Lara A. Gundel, Mohamad Sleiman, Brett C. Singer, Peyton Jacob, Jonathan P. Winickoff, Prue Talbot, Suzaynn Schick, Yinsheng Wang, Bo Hang, Manuela Martins-Green, James F. Pankow, Melbourne F. Hovell, Neal L. Benowitz, Virender K. Rehan, Jonathan M. Samet
Civil and Environmental Engineering Faculty Publications and Presentations
There is broad consensus regarding the health impact of tobacco use and secondhand smoke exposure, yet considerable ambiguity exists about the nature and consequences of thirdhand smoke (THS). We introduce definitions of THS and THS exposure and review recent findings about constituents, indoor sorption-desorption dynamics, and transformations of THS; distribution and persistence of THS in residential settings; implications for pathways of exposure; potential clinical significance and health effects; and behavioral and policy issues that affect and are affected by THS. Physical and chemical transformations of tobacco smoke pollutants take place over time scales ranging from seconds to months and include …